Controllable Modular Growth of Hierarchical MOF‐on‐MOF Architectures
Fabrication of hybrid MOF‐on‐MOF heteroarchitectures can create novel and multifunctional platforms to achieve desired properties. However, only MOFs with similar crystallographic parameters can be hybridized by the classical epitaxial growth method (EGM), which largely suppressed its applications....
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| Published in | Angewandte Chemie International Edition Vol. 56; no. 49; pp. 15658 - 15662 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
04.12.2017
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Fabrication of hybrid MOF‐on‐MOF heteroarchitectures can create novel and multifunctional platforms to achieve desired properties. However, only MOFs with similar crystallographic parameters can be hybridized by the classical epitaxial growth method (EGM), which largely suppressed its applications. A general strategy, called internal extended growth method (IEGM), is demonstrated for the feasible assembly of MOFs with distinct crystallographic parameters in an MOF matrix. Various MOFs with diverse functions could be introduced in a modular MOF matrix to form 3D core–satellite pluralistic hybrid system. The number of different MOF crystals interspersed could be varied on demand. More importantly, the different MOF crystals distributed in individual domains could be used to further incorporate functional units or enhance target functions.
A general strategy, the internal extended growth method (IEGM), was applied to design modular hierarchically structured MOF composites, thereby overcoming the limitation of lattice matching. The number of MOF crystals interspersed and the size of the MOF matrix can be well‐controlled. IEGM can optimize the design of novel multicompositional MOFs systems with great flexibility. TTIP=Ti(OiPr4), BDC=benzenedicarboxylic acid. |
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| AbstractList | Fabrication of hybrid MOF-on-MOF heteroarchitectures can create novel and multifunctional platforms to achieve desired properties. However, only MOFs with similar crystallographic parameters can be hybridized by the classical epitaxial growth method (EGM), which largely suppressed its applications. A general strategy, called internal extended growth method (IEGM), is demonstrated for the feasible assembly of MOFs with distinct crystallographic parameters in an MOF matrix. Various MOFs with diverse functions could be introduced in a modular MOF matrix to form 3D core-satellite pluralistic hybrid system. The number of different MOF crystals interspersed could be varied on demand. More importantly, the different MOF crystals distributed in individual domains could be used to further incorporate functional units or enhance target functions. Fabrication of hybrid MOF‐on‐MOF heteroarchitectures can create novel and multifunctional platforms to achieve desired properties. However, only MOFs with similar crystallographic parameters can be hybridized by the classical epitaxial growth method (EGM), which largely suppressed its applications. A general strategy, called internal extended growth method (IEGM), is demonstrated for the feasible assembly of MOFs with distinct crystallographic parameters in an MOF matrix. Various MOFs with diverse functions could be introduced in a modular MOF matrix to form 3D core–satellite pluralistic hybrid system. The number of different MOF crystals interspersed could be varied on demand. More importantly, the different MOF crystals distributed in individual domains could be used to further incorporate functional units or enhance target functions. A general strategy, the internal extended growth method (IEGM), was applied to design modular hierarchically structured MOF composites, thereby overcoming the limitation of lattice matching. The number of MOF crystals interspersed and the size of the MOF matrix can be well‐controlled. IEGM can optimize the design of novel multicompositional MOFs systems with great flexibility. TTIP=Ti(OiPr4), BDC=benzenedicarboxylic acid. Fabrication of hybrid MOF-on-MOF heteroarchitectures can create novel and multifunctional platforms to achieve desired properties. However, only MOFs with similar crystallographic parameters can be hybridized by the classical epitaxial growth method (EGM), which largely suppressed its applications. A general strategy, called internal extended growth method (IEGM), is demonstrated for the feasible assembly of MOFs with distinct crystallographic parameters in an MOF matrix. Various MOFs with diverse functions could be introduced in a modular MOF matrix to form 3D core-satellite pluralistic hybrid system. The number of different MOF crystals interspersed could be varied on demand. More importantly, the different MOF crystals distributed in individual domains could be used to further incorporate functional units or enhance target functions.Fabrication of hybrid MOF-on-MOF heteroarchitectures can create novel and multifunctional platforms to achieve desired properties. However, only MOFs with similar crystallographic parameters can be hybridized by the classical epitaxial growth method (EGM), which largely suppressed its applications. A general strategy, called internal extended growth method (IEGM), is demonstrated for the feasible assembly of MOFs with distinct crystallographic parameters in an MOF matrix. Various MOFs with diverse functions could be introduced in a modular MOF matrix to form 3D core-satellite pluralistic hybrid system. The number of different MOF crystals interspersed could be varied on demand. More importantly, the different MOF crystals distributed in individual domains could be used to further incorporate functional units or enhance target functions. |
| Author | Chen, Wei Gu, Yifan Li, Fengting Kitagawa, Susumu Li, Liangchun Wu, Yi‐nan |
| Author_xml | – sequence: 1 givenname: Yifan surname: Gu fullname: Gu, Yifan organization: Tongji University – sequence: 2 givenname: Yi‐nan surname: Wu fullname: Wu, Yi‐nan organization: Tongji University – sequence: 3 givenname: Liangchun surname: Li fullname: Li, Liangchun organization: Tongji University – sequence: 4 givenname: Wei surname: Chen fullname: Chen, Wei organization: Tongji University – sequence: 5 givenname: Fengting surname: Li fullname: Li, Fengting email: fengting@tongji.edu.cn organization: Tongji University – sequence: 6 givenname: Susumu surname: Kitagawa fullname: Kitagawa, Susumu email: kitagawa@iCeMS.kyoto-u.ac.jp organization: Kyoto University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29048720$$D View this record in MEDLINE/PubMed |
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| ContentType | Journal Article |
| Copyright | 2017 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim. |
| Copyright_xml | – notice: 2017 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim – notice: 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim. |
| DBID | AAYXX CITATION NPM 7TM K9. 7X8 |
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| SubjectTerms | Crystallography Crystals Epitaxial growth Fabrication functionalization Hybrid systems Hybridization metal–organic frameworks modular growth nanostructures synthesis design |
| Title | Controllable Modular Growth of Hierarchical MOF‐on‐MOF Architectures |
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