Non‐Solvating and Low‐Dielectricity Cosolvent for Anion‐Derived Solid Electrolyte Interphases in Lithium Metal Batteries
Lithium (Li) metal anodes hold great promise for next‐generation high‐energy‐density batteries, while the insufficient fundamental understanding of the complex solid electrolyte interphase (SEI) is the major obstacle for the full demonstration of their potential in working batteries. The characteris...
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| Published in | Angewandte Chemie International Edition Vol. 60; no. 20; pp. 11442 - 11447 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
10.05.2021
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Lithium (Li) metal anodes hold great promise for next‐generation high‐energy‐density batteries, while the insufficient fundamental understanding of the complex solid electrolyte interphase (SEI) is the major obstacle for the full demonstration of their potential in working batteries. The characteristics of SEI highly depend on the inner solvation structure of lithium ions (Li+). Herein, we clarify the critical significance of cosolvent properties on both Li+ solvation structure and the SEI formation on working Li metal anodes. Non‐solvating and low‐dielectricity (NL) cosolvents intrinsically enhance the interaction between anion and Li+ by affording a low dielectric environment. The abundant positively charged anion–cation aggregates generated as the introduction of NL cosolvents are preferentially brought to the negatively charged Li anode surface, inducing an anion‐derived inorganic‐rich SEI. A solvent diagram is further built to illustrate that a solvent with both proper relative binding energy toward Li+ and dielectric constant is suitable as NL cosolvent.
The introduction of cosolvents with non‐solvating and low‐dielectricity (NL) properties can intrinsically enhance the interaction between anion and Li+ and regulate the solvation structures in electrolytes, which favors an upgraded anion‐derived solid electrolyte interphase (SEI) on lithium metal anodes. |
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| AbstractList | Lithium (Li) metal anodes hold great promise for next‐generation high‐energy‐density batteries, while the insufficient fundamental understanding of the complex solid electrolyte interphase (SEI) is the major obstacle for the full demonstration of their potential in working batteries. The characteristics of SEI highly depend on the inner solvation structure of lithium ions (Li+). Herein, we clarify the critical significance of cosolvent properties on both Li+ solvation structure and the SEI formation on working Li metal anodes. Non‐solvating and low‐dielectricity (NL) cosolvents intrinsically enhance the interaction between anion and Li+ by affording a low dielectric environment. The abundant positively charged anion–cation aggregates generated as the introduction of NL cosolvents are preferentially brought to the negatively charged Li anode surface, inducing an anion‐derived inorganic‐rich SEI. A solvent diagram is further built to illustrate that a solvent with both proper relative binding energy toward Li+ and dielectric constant is suitable as NL cosolvent. Lithium (Li) metal anodes hold great promise for next‐generation high‐energy‐density batteries, while the insufficient fundamental understanding of the complex solid electrolyte interphase (SEI) is the major obstacle for the full demonstration of their potential in working batteries. The characteristics of SEI highly depend on the inner solvation structure of lithium ions (Li + ). Herein, we clarify the critical significance of cosolvent properties on both Li + solvation structure and the SEI formation on working Li metal anodes. Non‐solvating and low‐dielectricity (NL) cosolvents intrinsically enhance the interaction between anion and Li + by affording a low dielectric environment. The abundant positively charged anion–cation aggregates generated as the introduction of NL cosolvents are preferentially brought to the negatively charged Li anode surface, inducing an anion‐derived inorganic‐rich SEI. A solvent diagram is further built to illustrate that a solvent with both proper relative binding energy toward Li + and dielectric constant is suitable as NL cosolvent. Lithium (Li) metal anodes hold great promise for next‐generation high‐energy‐density batteries, while the insufficient fundamental understanding of the complex solid electrolyte interphase (SEI) is the major obstacle for the full demonstration of their potential in working batteries. The characteristics of SEI highly depend on the inner solvation structure of lithium ions (Li+). Herein, we clarify the critical significance of cosolvent properties on both Li+ solvation structure and the SEI formation on working Li metal anodes. Non‐solvating and low‐dielectricity (NL) cosolvents intrinsically enhance the interaction between anion and Li+ by affording a low dielectric environment. The abundant positively charged anion–cation aggregates generated as the introduction of NL cosolvents are preferentially brought to the negatively charged Li anode surface, inducing an anion‐derived inorganic‐rich SEI. A solvent diagram is further built to illustrate that a solvent with both proper relative binding energy toward Li+ and dielectric constant is suitable as NL cosolvent. The introduction of cosolvents with non‐solvating and low‐dielectricity (NL) properties can intrinsically enhance the interaction between anion and Li+ and regulate the solvation structures in electrolytes, which favors an upgraded anion‐derived solid electrolyte interphase (SEI) on lithium metal anodes. Lithium (Li) metal anodes hold great promise for next-generation high-energy-density batteries, while the insufficient fundamental understanding of the complex solid electrolyte interphase (SEI) is the major obstacle for the full demonstration of their potential in working batteries. The characteristics of SEI highly depend on the inner solvation structure of lithium ions (Li ). Herein, we clarify the critical significance of cosolvent properties on both Li solvation structure and the SEI formation on working Li metal anodes. Non-solvating and low-dielectricity (NL) cosolvents intrinsically enhance the interaction between anion and Li by affording a low dielectric environment. The abundant positively charged anion-cation aggregates generated as the introduction of NL cosolvents are preferentially brought to the negatively charged Li anode surface, inducing an anion-derived inorganic-rich SEI. A solvent diagram is further built to illustrate that a solvent with both proper relative binding energy toward Li and dielectric constant is suitable as NL cosolvent. Lithium (Li) metal anodes hold great promise for next-generation high-energy-density batteries, while the insufficient fundamental understanding of the complex solid electrolyte interphase (SEI) is the major obstacle for the full demonstration of their potential in working batteries. The characteristics of SEI highly depend on the inner solvation structure of lithium ions (Li+ ). Herein, we clarify the critical significance of cosolvent properties on both Li+ solvation structure and the SEI formation on working Li metal anodes. Non-solvating and low-dielectricity (NL) cosolvents intrinsically enhance the interaction between anion and Li+ by affording a low dielectric environment. The abundant positively charged anion-cation aggregates generated as the introduction of NL cosolvents are preferentially brought to the negatively charged Li anode surface, inducing an anion-derived inorganic-rich SEI. A solvent diagram is further built to illustrate that a solvent with both proper relative binding energy toward Li+ and dielectric constant is suitable as NL cosolvent.Lithium (Li) metal anodes hold great promise for next-generation high-energy-density batteries, while the insufficient fundamental understanding of the complex solid electrolyte interphase (SEI) is the major obstacle for the full demonstration of their potential in working batteries. The characteristics of SEI highly depend on the inner solvation structure of lithium ions (Li+ ). Herein, we clarify the critical significance of cosolvent properties on both Li+ solvation structure and the SEI formation on working Li metal anodes. Non-solvating and low-dielectricity (NL) cosolvents intrinsically enhance the interaction between anion and Li+ by affording a low dielectric environment. The abundant positively charged anion-cation aggregates generated as the introduction of NL cosolvents are preferentially brought to the negatively charged Li anode surface, inducing an anion-derived inorganic-rich SEI. A solvent diagram is further built to illustrate that a solvent with both proper relative binding energy toward Li+ and dielectric constant is suitable as NL cosolvent. |
| Author | Huang, Jia‐Qi Xu, Rui Xiao, Ye Yao, Yu‐Xing Yao, Nan Xie, Jin Ding, Jun‐Fan Chen, Xiang Yan, Chong |
| Author_xml | – sequence: 1 givenname: Jun‐Fan orcidid: 0000-0002-9042-0193 surname: Ding fullname: Ding, Jun‐Fan organization: Beijing Institute of Technology – sequence: 2 givenname: Rui orcidid: 0000-0001-6439-8706 surname: Xu fullname: Xu, Rui organization: Beijing Institute of Technology – sequence: 3 givenname: Nan orcidid: 0000-0003-1965-2917 surname: Yao fullname: Yao, Nan organization: Tsinghua University – sequence: 4 givenname: Xiang orcidid: 0000-0002-7686-6308 surname: Chen fullname: Chen, Xiang organization: Tsinghua University – sequence: 5 givenname: Ye orcidid: 0000-0001-9118-8931 surname: Xiao fullname: Xiao, Ye organization: Beijing Institute of Technology – sequence: 6 givenname: Yu‐Xing orcidid: 0000-0001-6350-1206 surname: Yao fullname: Yao, Yu‐Xing organization: Tsinghua University – sequence: 7 givenname: Chong orcidid: 0000-0001-9521-4981 surname: Yan fullname: Yan, Chong organization: Tsinghua University – sequence: 8 givenname: Jin orcidid: 0000-0002-4235-7441 surname: Xie fullname: Xie, Jin organization: Tsinghua University – sequence: 9 givenname: Jia‐Qi orcidid: 0000-0001-7394-9186 surname: Huang fullname: Huang, Jia‐Qi email: jqhuang@bit.edu.cn organization: Beijing Institute of Technology |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/33655631$$D View this record in MEDLINE/PubMed |
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| Copyright | 2021 Wiley‐VCH GmbH 2021 Wiley-VCH GmbH. |
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| Snippet | Lithium (Li) metal anodes hold great promise for next‐generation high‐energy‐density batteries, while the insufficient fundamental understanding of the complex... Lithium (Li) metal anodes hold great promise for next-generation high-energy-density batteries, while the insufficient fundamental understanding of the complex... |
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| SubjectTerms | Anions anion–cation interaction Anodes cation solvation Dielectric constant Electrolytes Lithium Lithium ions lithium metal batteries low-dielectricity cosolvent solid electrolyte interphase Solid electrolytes Solvation Solvents |
| Title | Non‐Solvating and Low‐Dielectricity Cosolvent for Anion‐Derived Solid Electrolyte Interphases in Lithium Metal Batteries |
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