Recent Progress of Hybrid Solid‐State Electrolytes for Lithium Batteries
Conventional liquid electrolytes for lithium batteries usually suffer from irreversible decomposition and safety concerns. Solid state electrolytes (SSEs) have been considered as the key for advanced lithium batteries with improved energy density and safety, whereas challenges remain for polymer and...
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| Published in | Chemistry : a European journal Vol. 24; no. 69; pp. 18293 - 18306 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
10.12.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Conventional liquid electrolytes for lithium batteries usually suffer from irreversible decomposition and safety concerns. Solid state electrolytes (SSEs) have been considered as the key for advanced lithium batteries with improved energy density and safety, whereas challenges remain for polymer and inorganic SSEs. Recently, hybrid solid‐state electrolytes (HSSEs) that integrate the merits of different electrolyte systems have been under intensive study. Herein, we summarize the recent progress of HSSEs with different compositions and structures. The design principle of each type of HSSEs are discussed, as well as their ionic conducting mechanism, electrochemical performance and effects of compositional/structural control. Finally, challenges and perspectives are provided for the future development of HSSEs and solid‐state lithium batteries.
Hybrid solid‐state electrolytes (HSSEs) are keys to the development of lithium batteries with enhanced energy density and safety. This Minireview summarizes the recent development of HSSEs and discusses their design principles, performance and ionic conducting mechanism. |
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| AbstractList | Conventional liquid electrolytes for lithium batteries usually suffer from irreversible decomposition and safety concerns. Solid state electrolytes (SSEs) have been considered as the key for advanced lithium batteries with improved energy density and safety, whereas challenges remain for polymer and inorganic SSEs. Recently, hybrid solid‐state electrolytes (HSSEs) that integrate the merits of different electrolyte systems have been under intensive study. Herein, we summarize the recent progress of HSSEs with different compositions and structures. The design principle of each type of HSSEs are discussed, as well as their ionic conducting mechanism, electrochemical performance and effects of compositional/structural control. Finally, challenges and perspectives are provided for the future development of HSSEs and solid‐state lithium batteries.
Hybrid solid‐state electrolytes (HSSEs) are keys to the development of lithium batteries with enhanced energy density and safety. This Minireview summarizes the recent development of HSSEs and discusses their design principles, performance and ionic conducting mechanism. Conventional liquid electrolytes for lithium batteries usually suffer from irreversible decomposition and safety concerns. Solid state electrolytes (SSEs) have been considered as the key for advanced lithium batteries with improved energy density and safety, whereas challenges remain for polymer and inorganic SSEs. Recently, hybrid solid‐state electrolytes (HSSEs) that integrate the merits of different electrolyte systems have been under intensive study. Herein, we summarize the recent progress of HSSEs with different compositions and structures. The design principle of each type of HSSEs are discussed, as well as their ionic conducting mechanism, electrochemical performance and effects of compositional/structural control. Finally, challenges and perspectives are provided for the future development of HSSEs and solid‐state lithium batteries. Conventional liquid electrolytes for lithium batteries usually suffer from irreversible decomposition and safety concerns. Solid state electrolytes (SSEs) have been considered as the key for advanced lithium batteries with improved energy density and safety, whereas challenges remain for polymer and inorganic SSEs. Recently, hybrid solid-state electrolytes (HSSEs) that integrate the merits of different electrolyte systems have been under intensive study. Herein, we summarize the recent progress of HSSEs with different compositions and structures. The design principle of each type of HSSEs are discussed, as well as their ionic conducting mechanism, electrochemical performance and effects of compositional/structural control. Finally, challenges and perspectives are provided for the future development of HSSEs and solid-state lithium batteries.Conventional liquid electrolytes for lithium batteries usually suffer from irreversible decomposition and safety concerns. Solid state electrolytes (SSEs) have been considered as the key for advanced lithium batteries with improved energy density and safety, whereas challenges remain for polymer and inorganic SSEs. Recently, hybrid solid-state electrolytes (HSSEs) that integrate the merits of different electrolyte systems have been under intensive study. Herein, we summarize the recent progress of HSSEs with different compositions and structures. The design principle of each type of HSSEs are discussed, as well as their ionic conducting mechanism, electrochemical performance and effects of compositional/structural control. Finally, challenges and perspectives are provided for the future development of HSSEs and solid-state lithium batteries. |
| Author | Liu, Xiaoyan Li, Xinru Li, Hexing Wu, Hao Bin |
| Author_xml | – sequence: 1 givenname: Xiaoyan surname: Liu fullname: Liu, Xiaoyan organization: Shanghai Normal University – sequence: 2 givenname: Xinru surname: Li fullname: Li, Xinru organization: University of California – sequence: 3 givenname: Hexing surname: Li fullname: Li, Hexing organization: Shanghai Normal University – sequence: 4 givenname: Hao Bin orcidid: 0000-0002-0725-6442 surname: Wu fullname: Wu, Hao Bin email: hbwu@zju.edu.cn organization: Zhejiang University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30221404$$D View this record in MEDLINE/PubMed |
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| Keywords | hybrid materials lithium metal anode ionic conductivity solid lithium batteries solid-state electrolyte |
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| Snippet | Conventional liquid electrolytes for lithium batteries usually suffer from irreversible decomposition and safety concerns. Solid state electrolytes (SSEs) have... |
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| SubjectTerms | Batteries Chemistry Electrochemical analysis Electrochemistry Electrolytes Flux density hybrid materials ionic conductivity Lithium Lithium batteries lithium metal anode Molten salt electrolytes Polymers Product design Safety Solid electrolytes solid lithium batteries solid-state electrolyte |
| Title | Recent Progress of Hybrid Solid‐State Electrolytes for Lithium Batteries |
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