A Dual‐Ligand Porous Coordination Polymer Chemiresistor with Modulated Conductivity and Porosity
Single‐ligand‐based electronically conductive porous coordination polymers/metal–organic frameworks (EC‐PCPs/MOFs) fail to meet the requirements of numerous electronic applications owing to their limited tunability in terms of both conductivity and topology. In this study, a new 2D π‐conjugated EC‐M...
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| Published in | Angewandte Chemie International Edition Vol. 59; no. 1; pp. 172 - 176 |
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| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
02.01.2020
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Single‐ligand‐based electronically conductive porous coordination polymers/metal–organic frameworks (EC‐PCPs/MOFs) fail to meet the requirements of numerous electronic applications owing to their limited tunability in terms of both conductivity and topology. In this study, a new 2D π‐conjugated EC‐MOF containing copper units with mixed trigonal ligands was developed: Cu3(HHTP)(THQ) (HHTP=2,3,6,7,10,11‐hexahydrotriphenylene, THQ=tetrahydroxy‐1,4‐quinone). The modulated conductivity (σ≈2.53×10−5 S cm−1 with an activation energy of 0.30 eV) and high porosity (ca. 441.2 m2 g−1) of the Cu3(HHTP)(THQ) semiconductive nanowires provided an appropriate resistance baseline and highly accessible areas for the development of an excellent chemiresistive gas sensor.
Makes sense: As two ligands offer more opportunity than one to tune MOF conductivity and topology, a 2D π‐conjugated copper‐based electronically conductive MOF with two different trigonal organic ligands was developed (see structure). The semiconductivity and high porosity of the resulting nanowires provided a low conductivity baseline and highly accessible surface areas, thus resulting in excellent room‐temperature chemiresistive sensing properties. |
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| AbstractList | Single‐ligand‐based electronically conductive porous coordination polymers/metal–organic frameworks (EC‐PCPs/MOFs) fail to meet the requirements of numerous electronic applications owing to their limited tunability in terms of both conductivity and topology. In this study, a new 2D π‐conjugated EC‐MOF containing copper units with mixed trigonal ligands was developed: Cu3(HHTP)(THQ) (HHTP=2,3,6,7,10,11‐hexahydrotriphenylene, THQ=tetrahydroxy‐1,4‐quinone). The modulated conductivity (σ≈2.53×10−5 S cm−1 with an activation energy of 0.30 eV) and high porosity (ca. 441.2 m2 g−1) of the Cu3(HHTP)(THQ) semiconductive nanowires provided an appropriate resistance baseline and highly accessible areas for the development of an excellent chemiresistive gas sensor.
Makes sense: As two ligands offer more opportunity than one to tune MOF conductivity and topology, a 2D π‐conjugated copper‐based electronically conductive MOF with two different trigonal organic ligands was developed (see structure). The semiconductivity and high porosity of the resulting nanowires provided a low conductivity baseline and highly accessible surface areas, thus resulting in excellent room‐temperature chemiresistive sensing properties. Single‐ligand‐based electronically conductive porous coordination polymers/metal–organic frameworks (EC‐PCPs/MOFs) fail to meet the requirements of numerous electronic applications owing to their limited tunability in terms of both conductivity and topology. In this study, a new 2D π‐conjugated EC‐MOF containing copper units with mixed trigonal ligands was developed: Cu3(HHTP)(THQ) (HHTP=2,3,6,7,10,11‐hexahydrotriphenylene, THQ=tetrahydroxy‐1,4‐quinone). The modulated conductivity (σ≈2.53×10−5 S cm−1 with an activation energy of 0.30 eV) and high porosity (ca. 441.2 m2 g−1) of the Cu3(HHTP)(THQ) semiconductive nanowires provided an appropriate resistance baseline and highly accessible areas for the development of an excellent chemiresistive gas sensor. Single-ligand-based electronically conductive porous coordination polymers/metal-organic frameworks (EC-PCPs/MOFs) fail to meet the requirements of numerous electronic applications owing to their limited tunability in terms of both conductivity and topology. In this study, a new 2D π-conjugated EC-MOF containing copper units with mixed trigonal ligands was developed: Cu (HHTP)(THQ) (HHTP=2,3,6,7,10,11-hexahydrotriphenylene, THQ=tetrahydroxy-1,4-quinone). The modulated conductivity (σ≈2.53×10 S cm with an activation energy of 0.30 eV) and high porosity (ca. 441.2 m g ) of the Cu (HHTP)(THQ) semiconductive nanowires provided an appropriate resistance baseline and highly accessible areas for the development of an excellent chemiresistive gas sensor. Single-ligand-based electronically conductive porous coordination polymers/metal-organic frameworks (EC-PCPs/MOFs) fail to meet the requirements of numerous electronic applications owing to their limited tunability in terms of both conductivity and topology. In this study, a new 2D π-conjugated EC-MOF containing copper units with mixed trigonal ligands was developed: Cu3 (HHTP)(THQ) (HHTP=2,3,6,7,10,11-hexahydrotriphenylene, THQ=tetrahydroxy-1,4-quinone). The modulated conductivity (σ≈2.53×10-5 S cm-1 with an activation energy of 0.30 eV) and high porosity (ca. 441.2 m2 g-1 ) of the Cu3 (HHTP)(THQ) semiconductive nanowires provided an appropriate resistance baseline and highly accessible areas for the development of an excellent chemiresistive gas sensor.Single-ligand-based electronically conductive porous coordination polymers/metal-organic frameworks (EC-PCPs/MOFs) fail to meet the requirements of numerous electronic applications owing to their limited tunability in terms of both conductivity and topology. In this study, a new 2D π-conjugated EC-MOF containing copper units with mixed trigonal ligands was developed: Cu3 (HHTP)(THQ) (HHTP=2,3,6,7,10,11-hexahydrotriphenylene, THQ=tetrahydroxy-1,4-quinone). The modulated conductivity (σ≈2.53×10-5 S cm-1 with an activation energy of 0.30 eV) and high porosity (ca. 441.2 m2 g-1 ) of the Cu3 (HHTP)(THQ) semiconductive nanowires provided an appropriate resistance baseline and highly accessible areas for the development of an excellent chemiresistive gas sensor. Single‐ligand‐based electronically conductive porous coordination polymers/metal–organic frameworks (EC‐PCPs/MOFs) fail to meet the requirements of numerous electronic applications owing to their limited tunability in terms of both conductivity and topology. In this study, a new 2D π‐conjugated EC‐MOF containing copper units with mixed trigonal ligands was developed: Cu 3 (HHTP)(THQ) (HHTP=2,3,6,7,10,11‐hexahydrotriphenylene, THQ=tetrahydroxy‐1,4‐quinone). The modulated conductivity ( σ ≈2.53×10 −5 S cm −1 with an activation energy of 0.30 eV) and high porosity (ca. 441.2 m 2 g −1 ) of the Cu 3 (HHTP)(THQ) semiconductive nanowires provided an appropriate resistance baseline and highly accessible areas for the development of an excellent chemiresistive gas sensor. |
| Author | Otake, Kenichi Tsujimoto, Masahiko Sakaki, Shigeyoshi Yao, Ming‐Shui Wu, Ai‐Qian Zheng, Jia‐Jia Kitagawa, Susumu Zhang, Gen Xu, Gang Horike, Satoshi Nagarkar, Sanjog S. |
| Author_xml | – sequence: 1 givenname: Ming‐Shui orcidid: 0000-0003-1604-2611 surname: Yao fullname: Yao, Ming‐Shui organization: Kyoto University – sequence: 2 givenname: Jia‐Jia surname: Zheng fullname: Zheng, Jia‐Jia organization: Kyoto University – sequence: 3 givenname: Ai‐Qian surname: Wu fullname: Wu, Ai‐Qian organization: Chinese Academy of Sciences – sequence: 4 givenname: Gang surname: Xu fullname: Xu, Gang organization: Chinese Academy of Sciences – sequence: 5 givenname: Sanjog S. surname: Nagarkar fullname: Nagarkar, Sanjog S. organization: Kyoto University – sequence: 6 givenname: Gen surname: Zhang fullname: Zhang, Gen organization: Kyoto University – sequence: 7 givenname: Masahiko surname: Tsujimoto fullname: Tsujimoto, Masahiko organization: Kyoto University – sequence: 8 givenname: Shigeyoshi surname: Sakaki fullname: Sakaki, Shigeyoshi organization: Kyoto University – sequence: 9 givenname: Satoshi surname: Horike fullname: Horike, Satoshi organization: Kyoto University – sequence: 10 givenname: Kenichi orcidid: 0000-0002-7904-5003 surname: Otake fullname: Otake, Kenichi email: ootake.kenichi.8a@kyoto-u.ac.jp organization: Kyoto University – sequence: 11 givenname: Susumu orcidid: 0000-0001-6956-9543 surname: Kitagawa fullname: Kitagawa, Susumu email: kitagawa@icems.kyoto-u.ac.jp organization: Kyoto University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31595640$$D View this record in MEDLINE/PubMed |
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| Keywords | nanowires porous coordination polymers semiconductors gas sensors metal-organic frameworks |
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| Snippet | Single‐ligand‐based electronically conductive porous coordination polymers/metal–organic frameworks (EC‐PCPs/MOFs) fail to meet the requirements of numerous... Single-ligand-based electronically conductive porous coordination polymers/metal-organic frameworks (EC-PCPs/MOFs) fail to meet the requirements of numerous... |
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| SubjectTerms | Conductivity Coordination polymers Gas sensors Ligands Metal-organic frameworks Nanotechnology Nanowires Organic chemistry Polymers Porosity porous coordination polymers Quinones semiconductors Topology |
| Title | A Dual‐Ligand Porous Coordination Polymer Chemiresistor with Modulated Conductivity and Porosity |
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