The Comparability of Pt to Pt‐Ru in Catalyzing the Hydrogen Oxidation Reaction for Alkaline Polymer Electrolyte Fuel Cells Operated at 80 °C
The Pt‐catalyzed hydrogen oxidation reaction (HOR) for alkaline polymer electrolyte fuel cells (APEFCs) has been one of the focus subjects in current fuel‐cell research. The Pt catalyst is inferior for HOR in alkaline solutions, and alloying with Ru is an effective promotion strategy. APEFCs with Pt...
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| Published in | Angewandte Chemie International Edition Vol. 58; no. 5; pp. 1442 - 1446 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
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Wiley Subscription Services, Inc
28.01.2019
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| Edition | International ed. in English |
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| Abstract | The Pt‐catalyzed hydrogen oxidation reaction (HOR) for alkaline polymer electrolyte fuel cells (APEFCs) has been one of the focus subjects in current fuel‐cell research. The Pt catalyst is inferior for HOR in alkaline solutions, and alloying with Ru is an effective promotion strategy. APEFCs with Pt‐Ru anodes have provided a performance benchmark over 1 W cm−2 at 60 °C. The Pt anode is now found to be in fact as good as the Pt‐Ru anode for APEFCs operated at elevated conditions. At 80 °C with appropriate gas back‐pressure, the cell with a Pt anode exhibits a peak power density of about 1.9 W cm−2, which is very close to that with a Pt‐Ru anode. Even by decreasing the anode Pt loading to 0.1 mg cm−2, over 1.5 W cm−2 can still be achieved at 80 °C. This finding alters the previous understanding about the Pt catalyzed HOR in alkaline media and casts a new light on the development of practical and high‐power APFEC technology.
Alkaline polymer electrolyte fuel cells (APEFCs) with Pt‐Ru anodes have provided a performance benchmark over 1 W cm−2 at 60 °C. The Pt anode (gray) is now found to be as good as the Pt‐Ru anode (red) for APEFCs operated at elevated conditions. At T=80 °C with appropriate gas back‐pressure p, the cell with a Pt anode exhibits a peak power density of about 1.9 W cm−2, which is very close to that with a Pt‐Ru anode. |
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| AbstractList | The Pt-catalyzed hydrogen oxidation reaction (HOR) for alkaline polymer electrolyte fuel cells (APEFCs) has been one of the focus subjects in current fuel-cell research. The Pt catalyst is inferior for HOR in alkaline solutions, and alloying with Ru is an effective promotion strategy. APEFCs with Pt-Ru anodes have provided a performance benchmark over 1 W cm
at 60 °C. The Pt anode is now found to be in fact as good as the Pt-Ru anode for APEFCs operated at elevated conditions. At 80 °C with appropriate gas back-pressure, the cell with a Pt anode exhibits a peak power density of about 1.9 W cm
, which is very close to that with a Pt-Ru anode. Even by decreasing the anode Pt loading to 0.1 mg cm
, over 1.5 W cm
can still be achieved at 80 °C. This finding alters the previous understanding about the Pt catalyzed HOR in alkaline media and casts a new light on the development of practical and high-power APFEC technology. The Pt‐catalyzed hydrogen oxidation reaction (HOR) for alkaline polymer electrolyte fuel cells (APEFCs) has been one of the focus subjects in current fuel‐cell research. The Pt catalyst is inferior for HOR in alkaline solutions, and alloying with Ru is an effective promotion strategy. APEFCs with Pt‐Ru anodes have provided a performance benchmark over 1 W cm−2 at 60 °C. The Pt anode is now found to be in fact as good as the Pt‐Ru anode for APEFCs operated at elevated conditions. At 80 °C with appropriate gas back‐pressure, the cell with a Pt anode exhibits a peak power density of about 1.9 W cm−2, which is very close to that with a Pt‐Ru anode. Even by decreasing the anode Pt loading to 0.1 mg cm−2, over 1.5 W cm−2 can still be achieved at 80 °C. This finding alters the previous understanding about the Pt catalyzed HOR in alkaline media and casts a new light on the development of practical and high‐power APFEC technology. The Pt‐catalyzed hydrogen oxidation reaction (HOR) for alkaline polymer electrolyte fuel cells (APEFCs) has been one of the focus subjects in current fuel‐cell research. The Pt catalyst is inferior for HOR in alkaline solutions, and alloying with Ru is an effective promotion strategy. APEFCs with Pt‐Ru anodes have provided a performance benchmark over 1 W cm−2 at 60 °C. The Pt anode is now found to be in fact as good as the Pt‐Ru anode for APEFCs operated at elevated conditions. At 80 °C with appropriate gas back‐pressure, the cell with a Pt anode exhibits a peak power density of about 1.9 W cm−2, which is very close to that with a Pt‐Ru anode. Even by decreasing the anode Pt loading to 0.1 mg cm−2, over 1.5 W cm−2 can still be achieved at 80 °C. This finding alters the previous understanding about the Pt catalyzed HOR in alkaline media and casts a new light on the development of practical and high‐power APFEC technology. Alkaline polymer electrolyte fuel cells (APEFCs) with Pt‐Ru anodes have provided a performance benchmark over 1 W cm−2 at 60 °C. The Pt anode (gray) is now found to be as good as the Pt‐Ru anode (red) for APEFCs operated at elevated conditions. At T=80 °C with appropriate gas back‐pressure p, the cell with a Pt anode exhibits a peak power density of about 1.9 W cm−2, which is very close to that with a Pt‐Ru anode. The Pt-catalyzed hydrogen oxidation reaction (HOR) for alkaline polymer electrolyte fuel cells (APEFCs) has been one of the focus subjects in current fuel-cell research. The Pt catalyst is inferior for HOR in alkaline solutions, and alloying with Ru is an effective promotion strategy. APEFCs with Pt-Ru anodes have provided a performance benchmark over 1 W cm-2 at 60 °C. The Pt anode is now found to be in fact as good as the Pt-Ru anode for APEFCs operated at elevated conditions. At 80 °C with appropriate gas back-pressure, the cell with a Pt anode exhibits a peak power density of about 1.9 W cm-2 , which is very close to that with a Pt-Ru anode. Even by decreasing the anode Pt loading to 0.1 mg cm-2 , over 1.5 W cm-2 can still be achieved at 80 °C. This finding alters the previous understanding about the Pt catalyzed HOR in alkaline media and casts a new light on the development of practical and high-power APFEC technology.The Pt-catalyzed hydrogen oxidation reaction (HOR) for alkaline polymer electrolyte fuel cells (APEFCs) has been one of the focus subjects in current fuel-cell research. The Pt catalyst is inferior for HOR in alkaline solutions, and alloying with Ru is an effective promotion strategy. APEFCs with Pt-Ru anodes have provided a performance benchmark over 1 W cm-2 at 60 °C. The Pt anode is now found to be in fact as good as the Pt-Ru anode for APEFCs operated at elevated conditions. At 80 °C with appropriate gas back-pressure, the cell with a Pt anode exhibits a peak power density of about 1.9 W cm-2 , which is very close to that with a Pt-Ru anode. Even by decreasing the anode Pt loading to 0.1 mg cm-2 , over 1.5 W cm-2 can still be achieved at 80 °C. This finding alters the previous understanding about the Pt catalyzed HOR in alkaline media and casts a new light on the development of practical and high-power APFEC technology. The Pt‐catalyzed hydrogen oxidation reaction (HOR) for alkaline polymer electrolyte fuel cells (APEFCs) has been one of the focus subjects in current fuel‐cell research. The Pt catalyst is inferior for HOR in alkaline solutions, and alloying with Ru is an effective promotion strategy. APEFCs with Pt‐Ru anodes have provided a performance benchmark over 1 W cm −2 at 60 °C. The Pt anode is now found to be in fact as good as the Pt‐Ru anode for APEFCs operated at elevated conditions. At 80 °C with appropriate gas back‐pressure, the cell with a Pt anode exhibits a peak power density of about 1.9 W cm −2 , which is very close to that with a Pt‐Ru anode. Even by decreasing the anode Pt loading to 0.1 mg cm −2 , over 1.5 W cm −2 can still be achieved at 80 °C. This finding alters the previous understanding about the Pt catalyzed HOR in alkaline media and casts a new light on the development of practical and high‐power APFEC technology. |
| Author | Wang, Yingming Peng, Hanqing Zhuang, Lin Xiao, Li Li, Qihao Lu, Juntao |
| Author_xml | – sequence: 1 givenname: Qihao surname: Li fullname: Li, Qihao organization: Wuhan University – sequence: 2 givenname: Hanqing surname: Peng fullname: Peng, Hanqing organization: Wuhan University – sequence: 3 givenname: Yingming surname: Wang fullname: Wang, Yingming organization: Wuhan University – sequence: 4 givenname: Li surname: Xiao fullname: Xiao, Li email: chem.lily@whu.edu.cn organization: Wuhan University – sequence: 5 givenname: Juntao surname: Lu fullname: Lu, Juntao organization: Wuhan University – sequence: 6 givenname: Lin orcidid: 0000-0002-5642-6735 surname: Zhuang fullname: Zhuang, Lin email: lzhuang@whu.edu.cn organization: Wuhan University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30548378$$D View this record in MEDLINE/PubMed |
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| Keywords | fuel cells temperature platinum hydrogen oxidation reaction alkaline polymer electrolyte |
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| Snippet | The Pt‐catalyzed hydrogen oxidation reaction (HOR) for alkaline polymer electrolyte fuel cells (APEFCs) has been one of the focus subjects in current fuel‐cell... The Pt-catalyzed hydrogen oxidation reaction (HOR) for alkaline polymer electrolyte fuel cells (APEFCs) has been one of the focus subjects in current fuel-cell... |
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| SubjectTerms | alkaline polymer electrolyte Anode effect Electrolytes Electrolytic cells Fuel cells Fuel technology hydrogen oxidation reaction Oxidation platinum Polymers Proton exchange membrane fuel cells Ruthenium temperature |
| Title | The Comparability of Pt to Pt‐Ru in Catalyzing the Hydrogen Oxidation Reaction for Alkaline Polymer Electrolyte Fuel Cells Operated at 80 °C |
| URI | https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.201812662 https://www.ncbi.nlm.nih.gov/pubmed/30548378 https://www.proquest.com/docview/2168819665 https://www.proquest.com/docview/2157656096 |
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