Porous Cobalt–Nickel Hydroxide Nanosheets with Active Cobalt Ions for Overall Water Splitting
Low‐cost and high‐performance catalysts are of great significance for electrochemical water splitting. Here, it is reported that a laser‐synthesized catalyst, porous Co0.75Ni0.25(OH)2 nanosheets, is highly active for catalyzing overall water splitting. The porous nanosheets exhibit low overpotential...
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| Published in | Small (Weinheim an der Bergstrasse, Germany) Vol. 15; no. 8; pp. e1804832 - n/a |
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| Main Authors | , , , , , , , , |
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| Language | English |
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01.02.2019
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| Abstract | Low‐cost and high‐performance catalysts are of great significance for electrochemical water splitting. Here, it is reported that a laser‐synthesized catalyst, porous Co0.75Ni0.25(OH)2 nanosheets, is highly active for catalyzing overall water splitting. The porous nanosheets exhibit low overpotentials for hydrogen evolution reaction (95 mV@10 mA cm−2) and oxygen evolution reaction (235 mV@10 mA cm−2). As both anode and cathode catalysts, the porous nanosheets achieve a current density of 10 mA cm−2 at an external voltage of 1.56 V, which is much lower than that of commercial Ir/C‐Pt/C couple (1.62 V). Experimental and theoretical investigations reveal that numerous Co3+ ions are generated on the pore wall of nanosheets, and the unique atomic structure around Co3+ ions leads to appropriate electronic structure and adsorption energy of intermediates, thus accelerating hydrogen and oxygen evolution.
An ecofriendly technique, laser ablation in liquid, is adopted to produce porous Co0.75Ni0.25(OH)2 nanosheets with numerous Co3+ ions on the pore wall. These Co3+ ions possess moderate adsorption for the intermediates of both hydrogen evolution and oxygen evolution reactions, thus accelerating electrochemical overall water splitting. |
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| AbstractList | Low-cost and high-performance catalysts are of great significance for electrochemical water splitting. Here, it is reported that a laser-synthesized catalyst, porous Co
Ni
(OH)
nanosheets, is highly active for catalyzing overall water splitting. The porous nanosheets exhibit low overpotentials for hydrogen evolution reaction (95 mV@10 mA cm
) and oxygen evolution reaction (235 mV@10 mA cm
). As both anode and cathode catalysts, the porous nanosheets achieve a current density of 10 mA cm
at an external voltage of 1.56 V, which is much lower than that of commercial Ir/C-Pt/C couple (1.62 V). Experimental and theoretical investigations reveal that numerous Co
ions are generated on the pore wall of nanosheets, and the unique atomic structure around Co
ions leads to appropriate electronic structure and adsorption energy of intermediates, thus accelerating hydrogen and oxygen evolution. Low‐cost and high‐performance catalysts are of great significance for electrochemical water splitting. Here, it is reported that a laser‐synthesized catalyst, porous Co0.75Ni0.25(OH)2 nanosheets, is highly active for catalyzing overall water splitting. The porous nanosheets exhibit low overpotentials for hydrogen evolution reaction (95 mV@10 mA cm−2) and oxygen evolution reaction (235 mV@10 mA cm−2). As both anode and cathode catalysts, the porous nanosheets achieve a current density of 10 mA cm−2 at an external voltage of 1.56 V, which is much lower than that of commercial Ir/C‐Pt/C couple (1.62 V). Experimental and theoretical investigations reveal that numerous Co3+ ions are generated on the pore wall of nanosheets, and the unique atomic structure around Co3+ ions leads to appropriate electronic structure and adsorption energy of intermediates, thus accelerating hydrogen and oxygen evolution. An ecofriendly technique, laser ablation in liquid, is adopted to produce porous Co0.75Ni0.25(OH)2 nanosheets with numerous Co3+ ions on the pore wall. These Co3+ ions possess moderate adsorption for the intermediates of both hydrogen evolution and oxygen evolution reactions, thus accelerating electrochemical overall water splitting. Low-cost and high-performance catalysts are of great significance for electrochemical water splitting. Here, it is reported that a laser-synthesized catalyst, porous Co0.75 Ni0.25 (OH)2 nanosheets, is highly active for catalyzing overall water splitting. The porous nanosheets exhibit low overpotentials for hydrogen evolution reaction (95 mV@10 mA cm-2 ) and oxygen evolution reaction (235 mV@10 mA cm-2 ). As both anode and cathode catalysts, the porous nanosheets achieve a current density of 10 mA cm-2 at an external voltage of 1.56 V, which is much lower than that of commercial Ir/C-Pt/C couple (1.62 V). Experimental and theoretical investigations reveal that numerous Co3+ ions are generated on the pore wall of nanosheets, and the unique atomic structure around Co3+ ions leads to appropriate electronic structure and adsorption energy of intermediates, thus accelerating hydrogen and oxygen evolution.Low-cost and high-performance catalysts are of great significance for electrochemical water splitting. Here, it is reported that a laser-synthesized catalyst, porous Co0.75 Ni0.25 (OH)2 nanosheets, is highly active for catalyzing overall water splitting. The porous nanosheets exhibit low overpotentials for hydrogen evolution reaction (95 mV@10 mA cm-2 ) and oxygen evolution reaction (235 mV@10 mA cm-2 ). As both anode and cathode catalysts, the porous nanosheets achieve a current density of 10 mA cm-2 at an external voltage of 1.56 V, which is much lower than that of commercial Ir/C-Pt/C couple (1.62 V). Experimental and theoretical investigations reveal that numerous Co3+ ions are generated on the pore wall of nanosheets, and the unique atomic structure around Co3+ ions leads to appropriate electronic structure and adsorption energy of intermediates, thus accelerating hydrogen and oxygen evolution. Low‐cost and high‐performance catalysts are of great significance for electrochemical water splitting. Here, it is reported that a laser‐synthesized catalyst, porous Co0.75Ni0.25(OH)2 nanosheets, is highly active for catalyzing overall water splitting. The porous nanosheets exhibit low overpotentials for hydrogen evolution reaction (95 mV@10 mA cm−2) and oxygen evolution reaction (235 mV@10 mA cm−2). As both anode and cathode catalysts, the porous nanosheets achieve a current density of 10 mA cm−2 at an external voltage of 1.56 V, which is much lower than that of commercial Ir/C‐Pt/C couple (1.62 V). Experimental and theoretical investigations reveal that numerous Co3+ ions are generated on the pore wall of nanosheets, and the unique atomic structure around Co3+ ions leads to appropriate electronic structure and adsorption energy of intermediates, thus accelerating hydrogen and oxygen evolution. Low‐cost and high‐performance catalysts are of great significance for electrochemical water splitting. Here, it is reported that a laser‐synthesized catalyst, porous Co 0.75 Ni 0.25 (OH) 2 nanosheets, is highly active for catalyzing overall water splitting. The porous nanosheets exhibit low overpotentials for hydrogen evolution reaction (95 mV@10 mA cm −2 ) and oxygen evolution reaction (235 mV@10 mA cm −2 ). As both anode and cathode catalysts, the porous nanosheets achieve a current density of 10 mA cm −2 at an external voltage of 1.56 V, which is much lower than that of commercial Ir/C‐Pt/C couple (1.62 V). Experimental and theoretical investigations reveal that numerous Co 3+ ions are generated on the pore wall of nanosheets, and the unique atomic structure around Co 3+ ions leads to appropriate electronic structure and adsorption energy of intermediates, thus accelerating hydrogen and oxygen evolution. |
| Author | Feng, Yi Li, Zhe Shen, Gu‐Rong Zou, Chengqin Liu, Hui Du, Xi‐Wen Dong, Cun‐Ku Wang, Xiao Wu, De‐Yao |
| Author_xml | – sequence: 1 givenname: Xiao surname: Wang fullname: Wang, Xiao organization: Tianjin University – sequence: 2 givenname: Zhe surname: Li fullname: Li, Zhe organization: Tianjin University – sequence: 3 givenname: De‐Yao surname: Wu fullname: Wu, De‐Yao organization: Tianjin University – sequence: 4 givenname: Gu‐Rong surname: Shen fullname: Shen, Gu‐Rong organization: Tianjin University – sequence: 5 givenname: Chengqin surname: Zou fullname: Zou, Chengqin organization: Tianjin University – sequence: 6 givenname: Yi surname: Feng fullname: Feng, Yi organization: Tianjin University – sequence: 7 givenname: Hui surname: Liu fullname: Liu, Hui email: cry5501@163.com organization: Tianjin University – sequence: 8 givenname: Cun‐Ku surname: Dong fullname: Dong, Cun‐Ku email: ckdong@tju.edu.cn organization: Tianjin University – sequence: 9 givenname: Xi‐Wen orcidid: 0000-0002-2811-147X surname: Du fullname: Du, Xi‐Wen email: xwdu@tju.edu.cn organization: Tianjin University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30714319$$D View this record in MEDLINE/PubMed |
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| Keywords | porous nanosheets trivalent cobalt ions cobalt-nickel hydroxide overall water splitting |
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| Snippet | Low‐cost and high‐performance catalysts are of great significance for electrochemical water splitting. Here, it is reported that a laser‐synthesized catalyst,... Low-cost and high-performance catalysts are of great significance for electrochemical water splitting. Here, it is reported that a laser-synthesized catalyst,... |
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| SubjectTerms | Atomic structure Catalysis Catalysts Chemical synthesis Cobalt cobalt–nickel hydroxide Electronic structure Hydrogen evolution reactions Iridium Nanosheets Nanotechnology overall water splitting Oxygen evolution reactions porous nanosheets trivalent cobalt ions Water splitting |
| Title | Porous Cobalt–Nickel Hydroxide Nanosheets with Active Cobalt Ions for Overall Water Splitting |
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