Dopant‐Free Squaraine‐Based Polymeric Hole‐Transporting Materials with Comprehensive Passivation Effects for Efficient All‐Inorganic Perovskite Solar Cells
Development of high‐performance dopant‐free hole‐transporting materials (HTMs) with comprehensive passivation effects is highly desirable for all‐inorganic perovskite solar cells (PVSCs). Squaraines (SQs) could be a candidate for dopant‐free HTMs as they are natural passivators for perovskites. One...
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| Published in | Angewandte Chemie International Edition Vol. 58; no. 49; pp. 17724 - 17730 |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
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Germany
Wiley Subscription Services, Inc
02.12.2019
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| Edition | International ed. in English |
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| Abstract | Development of high‐performance dopant‐free hole‐transporting materials (HTMs) with comprehensive passivation effects is highly desirable for all‐inorganic perovskite solar cells (PVSCs). Squaraines (SQs) could be a candidate for dopant‐free HTMs as they are natural passivators for perovskites. One major limitation of SQs is their relatively low hole mobility. Herein we demonstrate that polymerizing SQs into pseudo two dimensional (2D) p–π conjugated polymers could overcome this problem. By rationally using N,N‐diarylanilinosquaraines as the comonomers, the resulting polysquaraine HTMs not only exhibit suitable energy levels and efficient passivation effects, but also achieve very high hole mobility close to 0.01 cm−2 V−1 s−1. Thus as dopant‐free HTMs for α‐CsPbI2Br‐based all‐inorganic PVSCs, the best PCE reached is 15.5 %, outperforming those of the doped‐Spiro‐OMeTAD (14.4 %) based control devices and among the best for all‐inorganic PVSCs.
Squaring the hole: Using N,N‐diarylanilinosquaraines as the comonomers gives polysquaraine hole‐transporting materials (HTMs) that have very high hole mobility. As a dopant‐free HTM for α‐CsPbI2Br‐based all‐inorganic perovskite solar cells, the power conversion efficiency (PCE) can reach 15.5 %, among the best for all‐inorganic PVSCs. |
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| AbstractList | Development of high-performance dopant-free hole-transporting materials (HTMs) with comprehensive passivation effects is highly desirable for all-inorganic perovskite solar cells (PVSCs). Squaraines (SQs) could be a candidate for dopant-free HTMs as they are natural passivators for perovskites. One major limitation of SQs is their relatively low hole mobility. Herein we demonstrate that polymerizing SQs into pseudo two dimensional (2D) p-π conjugated polymers could overcome this problem. By rationally using N,N-diarylanilinosquaraines as the comonomers, the resulting polysquaraine HTMs not only exhibit suitable energy levels and efficient passivation effects, but also achieve very high hole mobility close to 0.01 cm-2 V-1 s-1 . Thus as dopant-free HTMs for α-CsPbI2 Br-based all-inorganic PVSCs, the best PCE reached is 15.5 %, outperforming those of the doped-Spiro-OMeTAD (14.4 %) based control devices and among the best for all-inorganic PVSCs.Development of high-performance dopant-free hole-transporting materials (HTMs) with comprehensive passivation effects is highly desirable for all-inorganic perovskite solar cells (PVSCs). Squaraines (SQs) could be a candidate for dopant-free HTMs as they are natural passivators for perovskites. One major limitation of SQs is their relatively low hole mobility. Herein we demonstrate that polymerizing SQs into pseudo two dimensional (2D) p-π conjugated polymers could overcome this problem. By rationally using N,N-diarylanilinosquaraines as the comonomers, the resulting polysquaraine HTMs not only exhibit suitable energy levels and efficient passivation effects, but also achieve very high hole mobility close to 0.01 cm-2 V-1 s-1 . Thus as dopant-free HTMs for α-CsPbI2 Br-based all-inorganic PVSCs, the best PCE reached is 15.5 %, outperforming those of the doped-Spiro-OMeTAD (14.4 %) based control devices and among the best for all-inorganic PVSCs. Development of high‐performance dopant‐free hole‐transporting materials (HTMs) with comprehensive passivation effects is highly desirable for all‐inorganic perovskite solar cells (PVSCs). Squaraines (SQs) could be a candidate for dopant‐free HTMs as they are natural passivators for perovskites. One major limitation of SQs is their relatively low hole mobility. Herein we demonstrate that polymerizing SQs into pseudo two dimensional (2D) p–π conjugated polymers could overcome this problem. By rationally using N,N‐diarylanilinosquaraines as the comonomers, the resulting polysquaraine HTMs not only exhibit suitable energy levels and efficient passivation effects, but also achieve very high hole mobility close to 0.01 cm−2 V−1 s−1. Thus as dopant‐free HTMs for α‐CsPbI2Br‐based all‐inorganic PVSCs, the best PCE reached is 15.5 %, outperforming those of the doped‐Spiro‐OMeTAD (14.4 %) based control devices and among the best for all‐inorganic PVSCs. Development of high‐performance dopant‐free hole‐transporting materials (HTMs) with comprehensive passivation effects is highly desirable for all‐inorganic perovskite solar cells (PVSCs). Squaraines (SQs) could be a candidate for dopant‐free HTMs as they are natural passivators for perovskites. One major limitation of SQs is their relatively low hole mobility. Herein we demonstrate that polymerizing SQs into pseudo two dimensional (2D) p–π conjugated polymers could overcome this problem. By rationally using N,N‐diarylanilinosquaraines as the comonomers, the resulting polysquaraine HTMs not only exhibit suitable energy levels and efficient passivation effects, but also achieve very high hole mobility close to 0.01 cm −2 V −1 s −1 . Thus as dopant‐free HTMs for α‐CsPbI 2 Br‐based all‐inorganic PVSCs, the best PCE reached is 15.5 %, outperforming those of the doped‐Spiro‐OMeTAD (14.4 %) based control devices and among the best for all‐inorganic PVSCs. Development of high-performance dopant-free hole-transporting materials (HTMs) with comprehensive passivation effects is highly desirable for all-inorganic perovskite solar cells (PVSCs). Squaraines (SQs) could be a candidate for dopant-free HTMs as they are natural passivators for perovskites. One major limitation of SQs is their relatively low hole mobility. Herein we demonstrate that polymerizing SQs into pseudo two dimensional (2D) p-π conjugated polymers could overcome this problem. By rationally using N,N-diarylanilinosquaraines as the comonomers, the resulting polysquaraine HTMs not only exhibit suitable energy levels and efficient passivation effects, but also achieve very high hole mobility close to 0.01 cm V s . Thus as dopant-free HTMs for α-CsPbI Br-based all-inorganic PVSCs, the best PCE reached is 15.5 %, outperforming those of the doped-Spiro-OMeTAD (14.4 %) based control devices and among the best for all-inorganic PVSCs. Development of high‐performance dopant‐free hole‐transporting materials (HTMs) with comprehensive passivation effects is highly desirable for all‐inorganic perovskite solar cells (PVSCs). Squaraines (SQs) could be a candidate for dopant‐free HTMs as they are natural passivators for perovskites. One major limitation of SQs is their relatively low hole mobility. Herein we demonstrate that polymerizing SQs into pseudo two dimensional (2D) p–π conjugated polymers could overcome this problem. By rationally using N,N‐diarylanilinosquaraines as the comonomers, the resulting polysquaraine HTMs not only exhibit suitable energy levels and efficient passivation effects, but also achieve very high hole mobility close to 0.01 cm−2 V−1 s−1. Thus as dopant‐free HTMs for α‐CsPbI2Br‐based all‐inorganic PVSCs, the best PCE reached is 15.5 %, outperforming those of the doped‐Spiro‐OMeTAD (14.4 %) based control devices and among the best for all‐inorganic PVSCs. Squaring the hole: Using N,N‐diarylanilinosquaraines as the comonomers gives polysquaraine hole‐transporting materials (HTMs) that have very high hole mobility. As a dopant‐free HTM for α‐CsPbI2Br‐based all‐inorganic perovskite solar cells, the power conversion efficiency (PCE) can reach 15.5 %, among the best for all‐inorganic PVSCs. |
| Author | Li, Zhen Han, Mengmeng Xiao, Qi Xiong, Bijin Zhu, Zonglong Li, Zhong'an Tian, Jingjing Wang, Jing Yip, Hin‐Lap Xue, Qifan |
| Author_xml | – sequence: 1 givenname: Qi surname: Xiao fullname: Xiao, Qi organization: Huazhong University of Science and Technology – sequence: 2 givenname: Jingjing surname: Tian fullname: Tian, Jingjing organization: South China University of Technology – sequence: 3 givenname: Qifan surname: Xue fullname: Xue, Qifan email: qfxue@scut.edu.cn organization: South China University of Technology – sequence: 4 givenname: Jing surname: Wang fullname: Wang, Jing organization: City University of Hong Kong – sequence: 5 givenname: Bijin surname: Xiong fullname: Xiong, Bijin organization: Huazhong University of Science and Technology – sequence: 6 givenname: Mengmeng surname: Han fullname: Han, Mengmeng organization: Wuhan University – sequence: 7 givenname: Zhen surname: Li fullname: Li, Zhen organization: Wuhan University – sequence: 8 givenname: Zonglong surname: Zhu fullname: Zhu, Zonglong organization: City University of Hong Kong – sequence: 9 givenname: Hin‐Lap surname: Yip fullname: Yip, Hin‐Lap email: msangusyip@scut.edu.cn organization: South China University of Technology – sequence: 10 givenname: Zhong'an orcidid: 0000-0001-9294-8939 surname: Li fullname: Li, Zhong'an email: lizha@hust.edu.cn organization: Huazhong University of Science and Technology |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31560144$$D View this record in MEDLINE/PubMed |
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| Keywords | passivation polysquaraines hole-transporting materials dopant-free all-inorganic perovskite solar cells |
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| Snippet | Development of high‐performance dopant‐free hole‐transporting materials (HTMs) with comprehensive passivation effects is highly desirable for all‐inorganic... Development of high-performance dopant-free hole-transporting materials (HTMs) with comprehensive passivation effects is highly desirable for all-inorganic... |
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| SubjectTerms | all-inorganic perovskite solar cells dopant-free Dopants Energy levels Hole mobility hole-transporting materials Mobility passivation Passivity Perovskites Photovoltaic cells Polymers polysquaraines Solar cells Transportation |
| Title | Dopant‐Free Squaraine‐Based Polymeric Hole‐Transporting Materials with Comprehensive Passivation Effects for Efficient All‐Inorganic Perovskite Solar Cells |
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