Films from soft-core/hard-shell hydrophobic latexes: Structure and thermomechanical properties

Structured latexes provide a promising route to hard coatings without the use of coalescing aids. We studied the thermomechanical properties of films from structured soft‐core/hard‐shell hydrophobic latexes. We found that the mechanical properties of these films were closely related to their very pa...

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Published inJournal of polymer science. Part B, Polymer physics Vol. 38; no. 23; pp. 2989 - 3000
Main Authors Domingues Dos Santos, Fabrice, Fabre, Pascale, Drujon, Xavier, Meunier, Gilles, Leibler, Ludwik
Format Journal Article
LanguageEnglish
Published New York John Wiley & Sons, Inc 01.12.2000
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Abstract Structured latexes provide a promising route to hard coatings without the use of coalescing aids. We studied the thermomechanical properties of films from structured soft‐core/hard‐shell hydrophobic latexes. We found that the mechanical properties of these films were closely related to their very particular organization. When the rigid phase was continuous, whatever its volume fraction, the films exhibited a high elastic modulus. An analysis of the viscoelastic properties of the films provided a good method for obtaining information about the interphase between the hard shell and soft core of the latex particles. By varying the film structure through annealing or the particle composition (core/shell ratio, core crosslinking, etc.), we were able to tune the mechanical properties of the films. © 2000 John Wiley & Sons, Inc. J Polym Sci B: Polym Phys 38: 2989–3000, 2000
AbstractList Structured latexes provide a promising route to hard coatings without the use of coalescing aids. We studied the thermomechanical properties of films from structured soft‐core/hard‐shell hydrophobic latexes. We found that the mechanical properties of these films were closely related to their very particular organization. When the rigid phase was continuous, whatever its volume fraction, the films exhibited a high elastic modulus. An analysis of the viscoelastic properties of the films provided a good method for obtaining information about the interphase between the hard shell and soft core of the latex particles. By varying the film structure through annealing or the particle composition (core/shell ratio, core crosslinking, etc.), we were able to tune the mechanical properties of the films. © 2000 John Wiley & Sons, Inc. J Polym Sci B: Polym Phys 38: 2989–3000, 2000
Structured latexes provide a promising route to hard coatings without the use of coalescing aids. We studied the thermomechanical properties of films from structured sort-core/hard-!1hell hydrophobic latexes. We found that the mechanical properties of these films were closely related to their very particular organization. When the rigid phase was continuous, whatever its volume fraction, the films exhibited a high elastic modulus. An analysis of the viscoelastic properties of the films provided a good method for obtaining information about the interphase between the hard shell and sort core of the latex particles. By varying the film structure through annealing or the particle composition (corelshell ratio, core crosslinking, etc.), we were able to tune the mechanical properties of the films.
Author Domingues Dos Santos, Fabrice
Fabre, Pascale
Leibler, Ludwik
Meunier, Gilles
Drujon, Xavier
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Issue 23
Keywords Dynamic mechanical properties
Butyl acrylate polymer
Film
Morphology
Internal structure
Methyl methacrylate polymer
Property structure relationship
Experimental study
Latex
Thermomechanical analysis
thermomechanical properties
latex films
structure
interphase
core-shell
Language English
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PublicationTitle Journal of polymer science. Part B, Polymer physics
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Snippet Structured latexes provide a promising route to hard coatings without the use of coalescing aids. We studied the thermomechanical properties of films from...
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SubjectTerms Applied sciences
core-shell
Exact sciences and technology
Forms of application and semi-finished materials
interphase
latex films
Physics
Polymer industry, paints, wood
Sheets and films
structure
Technology of polymers
thermomechanical properties
Title Films from soft-core/hard-shell hydrophobic latexes: Structure and thermomechanical properties
URI https://api.istex.fr/ark:/67375/WNG-BNDWRSN6-R/fulltext.pdf
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https://hal.science/hal-03555328
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