Plasmonic polyaniline/gold nanorods hybrid composites for selective NIR photodetection: Synthesis and characterization

In this study, we present the development of polyaniline/gold nanorod nanocomposites and the effect of the nanorods' aspect ratio and concentration on the overall electrical conductivity of nanocomposite systems. The electrical characterization showed that at the same atomic gold concentration,...

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Published inComposites. Part B, Engineering Vol. 149; pp. 178 - 187
Main Authors Abdelrasoul, Gaser N., Pignatelli, Francesca, Liakos, Ioannis, Cingolani, Roberto, Athanassiou, Athanassia
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 15.09.2018
Subjects
Gold nanorods
Nanocomposites
Photodetectors
Polyaniline
Polyaniline/gold nanorods composites
Photodetectors
Gold nanorods
Polyaniline/gold nanorods composites
Nanocomposites
Polyaniline
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Abstract In this study, we present the development of polyaniline/gold nanorod nanocomposites and the effect of the nanorods' aspect ratio and concentration on the overall electrical conductivity of nanocomposite systems. The electrical characterization showed that at the same atomic gold concentration, the conductivity of the nanocomposites increased by about 14% after increasing the gold nanorods' aspect ratio from 2.9 to 3.8. Furthermore, the conductivity of the nanocomposites increases linearly with the concentration of atomic gold, keeping the nanorods' aspect ratio stable, due to increasing the metallic content. The interaction between polyaniline and gold nanorods was investigated by FTIR, micro Raman, and XPS spectroscopic techniques, indicating the delocalization of the charges across the polymer chains induced by the incorporation of the nanorods. The interaction most likely occurs through the imine nitrogen of the polymer's backbone. The homogenous distribution of the gold nanorods in the polyaniline matrix was verified by TEM. Furthermore, the selective photosensitivity of the developed nanocomposites to NIR light was examined, and an increase in their current density was detected when the nanocomposites were irradiated at the wavelength that coincides with the longitudinal plasmonic resonance absorption of the incorporated nanorods. We foresee applications of the developed nanocomposites in numerous optoelectronic sectors.
AbstractList In this study, we present the development of polyaniline/gold nanorod nanocomposites and the effect of the nanorods' aspect ratio and concentration on the overall electrical conductivity of nanocomposite systems. The electrical characterization showed that at the same atomic gold concentration, the conductivity of the nanocomposites increased by about 14% after increasing the gold nanorods' aspect ratio from 2.9 to 3.8. Furthermore, the conductivity of the nanocomposites increases linearly with the concentration of atomic gold, keeping the nanorods' aspect ratio stable, due to increasing the metallic content. The interaction between polyaniline and gold nanorods was investigated by FTIR, micro Raman, and XPS spectroscopic techniques, indicating the delocalization of the charges across the polymer chains induced by the incorporation of the nanorods. The interaction most likely occurs through the imine nitrogen of the polymer's backbone. The homogenous distribution of the gold nanorods in the polyaniline matrix was verified by TEM. Furthermore, the selective photosensitivity of the developed nanocomposites to NIR light was examined, and an increase in their current density was detected when the nanocomposites were irradiated at the wavelength that coincides with the longitudinal plasmonic resonance absorption of the incorporated nanorods. We foresee applications of the developed nanocomposites in numerous optoelectronic sectors.
Author Pignatelli, Francesca
Athanassiou, Athanassia
Liakos, Ioannis
Cingolani, Roberto
Abdelrasoul, Gaser N.
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Keywords Photodetectors
Gold nanorods
Polyaniline/gold nanorods composites
Nanocomposites
Polyaniline
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Snippet In this study, we present the development of polyaniline/gold nanorod nanocomposites and the effect of the nanorods' aspect ratio and concentration on the...
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SubjectTerms Gold nanorods
Nanocomposites
Photodetectors
Polyaniline
Polyaniline/gold nanorods composites
Title Plasmonic polyaniline/gold nanorods hybrid composites for selective NIR photodetection: Synthesis and characterization
URI https://dx.doi.org/10.1016/j.compositesb.2018.05.015
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