Decontamination of real textile industrial effluent by strong oxidant species electrogenerated on diamond electrode: Viability and disadvantages of this electrochemical technology
[Display omitted] ► Electrogenerated strong oxidants on BDD surface improve the color and COD removals. ► Active chlorine species can generate organochlorinated compounds at the end of treatment. ► Chloroform is a recalcitrant and persistent by-product formed. ► Catalytic alternative processes to el...
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| Published in | Applied catalysis. B, Environmental Vol. 130-131; pp. 112 - 120 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
07.02.2013
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
► Electrogenerated strong oxidants on BDD surface improve the color and COD removals. ► Active chlorine species can generate organochlorinated compounds at the end of treatment. ► Chloroform is a recalcitrant and persistent by-product formed. ► Catalytic alternative processes to eliminate organic pollutants from industrial effluents.
In a previous work [1], the treatment of dye solutions containing Remazol Red BR (RRB) and Novacron Blue C-D (NB) by anodic oxidation using boron doped diamond anode (BDD) demonstrated that the electrochemical treatment is an efficient alternative for removing color and chemical oxygen demand (COD) and this technology can be used for depuration of real effluents. More recently, these assumptions have been confirmed by oxidizing electrochemically a real textile effluent using BDD anode [2]. Then, as a further development of the research carried out in these previous studies [1,2], in the present work, it has been considered appropriate to extend the investigation to the anodic oxidation, using BDD anode, of a specific real effluent discharged by Brazilian textile industry, adding Na2SO4 or NaCl salts in order to verify the applicability of this treatment producing in situ strong oxidant species (peroxodisulfates or active chlorine, respectively).
In this study, we also attempt to discuss critical evidence about the viability of peroxodisulfates or active chlorine. Results obtained in this research clearly demonstrated that the effect of the electrogenerated strong oxidant species, peroxodisulfates or active chlorine, depends on electrocatalytic mechanism followed on BDD surface, improving the color and COD removal. However, there is a limit of NaCl for treating real effluents avoiding the formation of organochloride compounds; and it is a subject of critical importance, from the environmental point of view, to apply this alternative treatment. |
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| AbstractList | In a previous work [1], the treatment of dye solutions containing Remazol Red BR (RRB) and Novacron Blue C-D (NB) by anodic oxidation using boron doped diamond anode (BDD) demonstrated that the electrochemical treatment is an efficient alternative for removing color and chemical oxygen demand (COD) and this technology can be used for depuration of real effluents. More recently, these assumptions have been confirmed by oxidizing electrochemically a real textile effluent using BDD anode [2]. Then, as a further development of the research carried out in these previous studies 0005 and 0010, in the present work, it has been considered appropriate to extend the investigation to the anodic oxidation, using BDD anode, of a specific real effluent discharged by Brazilian textile industry, adding Na sub(2)SO sub(4) or NaCl salts in order to verify the applicability of this treatment producing in situ strong oxidant species (peroxodisulfates or active chlorine, respectively). In this study, we also attempt to discuss critical evidence about the viability of peroxodisulfates or active chlorine. Results obtained in this research clearly demonstrated that the effect of the electrogenerated strong oxidant species, peroxodisulfates or active chlorine, depends on electrocatalytic mechanism followed on BDD surface, improving the color and COD removal. However, there is a limit of NaCl for treating real effluents avoiding the formation of organochloride compounds; and it is a subject of critical importance, from the environmental point of view, to apply this alternative treatment. [Display omitted] ► Electrogenerated strong oxidants on BDD surface improve the color and COD removals. ► Active chlorine species can generate organochlorinated compounds at the end of treatment. ► Chloroform is a recalcitrant and persistent by-product formed. ► Catalytic alternative processes to eliminate organic pollutants from industrial effluents. In a previous work [1], the treatment of dye solutions containing Remazol Red BR (RRB) and Novacron Blue C-D (NB) by anodic oxidation using boron doped diamond anode (BDD) demonstrated that the electrochemical treatment is an efficient alternative for removing color and chemical oxygen demand (COD) and this technology can be used for depuration of real effluents. More recently, these assumptions have been confirmed by oxidizing electrochemically a real textile effluent using BDD anode [2]. Then, as a further development of the research carried out in these previous studies [1,2], in the present work, it has been considered appropriate to extend the investigation to the anodic oxidation, using BDD anode, of a specific real effluent discharged by Brazilian textile industry, adding Na2SO4 or NaCl salts in order to verify the applicability of this treatment producing in situ strong oxidant species (peroxodisulfates or active chlorine, respectively). In this study, we also attempt to discuss critical evidence about the viability of peroxodisulfates or active chlorine. Results obtained in this research clearly demonstrated that the effect of the electrogenerated strong oxidant species, peroxodisulfates or active chlorine, depends on electrocatalytic mechanism followed on BDD surface, improving the color and COD removal. However, there is a limit of NaCl for treating real effluents avoiding the formation of organochloride compounds; and it is a subject of critical importance, from the environmental point of view, to apply this alternative treatment. In a previous work [1], the treatment of dye solutions containing Remazol Red BR (RRB) and Novacron Blue C-D (NB) by anodic oxidation using boron doped diamond anode (BDD) demonstrated that the electrochemical treatment is an efficient alternative for removing color and chemical oxygen demand (COD) and this technology can be used for depuration of real effluents. More recently, these assumptions have been confirmed by oxidizing electrochemically a real textile effluent using BDD anode [2]. Then, as a further development of the research carried out in these previous studies [1,2], in the present work, it has been considered appropriate to extend the investigation to the anodic oxidation, using BDD anode, of a specific real effluent discharged by Brazilian textile industry, adding Na2SO4 or NaCl salts in order to verify the applicability of this treatment producing in situ strong oxidant species (peroxodisulfates or active chlorine, respectively). In this study, we also attempt to discuss critical evidence about the viability of peroxodisulfates or active chlorine. Results obtained in this research clearly demonstrated that the effect of the electrogenerated strong oxidant species, peroxodisulfates or active chlorine, depends on electrocatalytic mechanism followed on BDD surface, improving the color and COD removal. However, there is a limit of NaCl for treating real effluents avoiding the formation of organochloride compounds; and it is a subject of critical importance, from the environmental point of view, to apply this alternative treatment. |
| Author | Vieira de Melo, Jailson Peralta-Hernandez, Juan M. Ribeiro da Silva, Djalma Sales Solano, Aline Maria Costa de Araújo, Cynthia K. Martínez-Huitle, Carlos A. |
| Author_xml | – sequence: 1 givenname: Aline Maria surname: Sales Solano fullname: Sales Solano, Aline Maria organization: Universidade Federal do Rio Grande do Norte, Instituto de Química, Lagoa Nova CEP 59078-970, Natal, RN, Brazil – sequence: 2 givenname: Cynthia K. surname: Costa de Araújo fullname: Costa de Araújo, Cynthia K. organization: Universidade Federal do Rio Grande do Norte, Instituto de Química, Lagoa Nova CEP 59078-970, Natal, RN, Brazil – sequence: 3 givenname: Jailson surname: Vieira de Melo fullname: Vieira de Melo, Jailson organization: Universidade Federal do Rio Grande do Norte, Instituto de Química, Lagoa Nova CEP 59078-970, Natal, RN, Brazil – sequence: 4 givenname: Juan M. surname: Peralta-Hernandez fullname: Peralta-Hernandez, Juan M. organization: Centro de Innovación Aplicada en Tecnologías Competitivas(CIATEC), Departamento de Investigación Ambiental Omega-201, Fraccionamiento Industrial Delta, León, 37545, Guanajuato, México – sequence: 5 givenname: Djalma surname: Ribeiro da Silva fullname: Ribeiro da Silva, Djalma organization: Universidade Federal do Rio Grande do Norte, Instituto de Química, Lagoa Nova CEP 59078-970, Natal, RN, Brazil – sequence: 6 givenname: Carlos A. surname: Martínez-Huitle fullname: Martínez-Huitle, Carlos A. email: carlosmh@quimica.ufrn.br organization: Universidade Federal do Rio Grande do Norte, Instituto de Química, Lagoa Nova CEP 59078-970, Natal, RN, Brazil |
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| Keywords | Decolorization Organic matter Active chlorine Strong oxidant species Real effluent Diamond electrode Peroxodisulfates |
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► Electrogenerated strong oxidants on BDD surface improve the color and COD removals. ► Active chlorine species can generate... In a previous work [1], the treatment of dye solutions containing Remazol Red BR (RRB) and Novacron Blue C-D (NB) by anodic oxidation using boron doped diamond... |
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| SubjectTerms | Active chlorine Decolorization Diamond electrode Organic matter Peroxodisulfates Real effluent Strong oxidant species |
| Title | Decontamination of real textile industrial effluent by strong oxidant species electrogenerated on diamond electrode: Viability and disadvantages of this electrochemical technology |
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