On the design of new europium heteroaromatic carboxylates for OLED application
The approach to the directed synthesis of lanthanide aromatic carboxylates – precursors to the electroluminescent materials, - was proposed, namely the conjugation length increase and heteroatom introduction in the appropriate position in combination with the neutral ligand introduction. This result...
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| Published in | Dyes and pigments Vol. 170; p. 107604 |
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| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
01.11.2019
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The approach to the directed synthesis of lanthanide aromatic carboxylates – precursors to the electroluminescent materials, - was proposed, namely the conjugation length increase and heteroatom introduction in the appropriate position in combination with the neutral ligand introduction. This resulted in the isolation of a series of new lanthanide complexes, among which the highest electroluminescence efficiency was obtained for mixed-ligand europium benzothiazole-2-carboxylate with bathophenanthroline in a solution-processed OLED. The peculiarities of energy transfer processes allowed obtaining luminescence thermometer materials based on this system, which demontrated the sensitivity of 2.8%/K in the physiological range.
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•New benzoxazolates and benzothiazolates of some lanthanides were obtained.•Complex properties are mainly independent on the second (O or S) heteroatom nature.•Mixed-ligand europium benzothiazolate with batophenanthroline was successfully used in solution-based OLED.•Bimetallic terbium-europium benzothiazolate demonstrates temperature-dependent luminescence with high sensitivity (2.8%/K). |
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| AbstractList | The approach to the directed synthesis of lanthanide aromatic carboxylates – precursors to the electroluminescent materials, - was proposed, namely the conjugation length increase and heteroatom introduction in the appropriate position in combination with the neutral ligand introduction. This resulted in the isolation of a series of new lanthanide complexes, among which the highest electroluminescence efficiency was obtained for mixed-ligand europium benzothiazole-2-carboxylate with bathophenanthroline in a solution-processed OLED. The peculiarities of energy transfer processes allowed obtaining luminescence thermometer materials based on this system, which demontrated the sensitivity of 2.8%/K in the physiological range.
[Display omitted]
•New benzoxazolates and benzothiazolates of some lanthanides were obtained.•Complex properties are mainly independent on the second (O or S) heteroatom nature.•Mixed-ligand europium benzothiazolate with batophenanthroline was successfully used in solution-based OLED.•Bimetallic terbium-europium benzothiazolate demonstrates temperature-dependent luminescence with high sensitivity (2.8%/K). |
| ArticleNumber | 107604 |
| Author | Goloveshkin, Alexander S. Vashchenko, Andrey A. Averin, Alexey A. Kozhevnikova (Khudoleeva), Vladislava Yu Medvedko, Alexey V. Schepers, Ute Koshelev, Daniil S. Tsymbarenko, Dmitry M. Meschkov, Anna Vatsadze, Sergey Z. Utochnikova, Valentina V. Chikineva, Tatyana Yu |
| Author_xml | – sequence: 1 givenname: Daniil S. surname: Koshelev fullname: Koshelev, Daniil S. email: valentina@inorg.chem.msu.ru organization: Faculty of Materials Science, M.V. Lomonosov Moscow State University, 1/73 Leninskye Gory, Moscow, 119991, Russia – sequence: 2 givenname: Tatyana Yu surname: Chikineva fullname: Chikineva, Tatyana Yu organization: Faculty of Materials Science, M.V. Lomonosov Moscow State University, 1/73 Leninskye Gory, Moscow, 119991, Russia – sequence: 3 givenname: Vladislava Yu surname: Kozhevnikova (Khudoleeva) fullname: Kozhevnikova (Khudoleeva), Vladislava Yu organization: Faculty of Materials Science, M.V. Lomonosov Moscow State University, 1/73 Leninskye Gory, Moscow, 119991, Russia – sequence: 4 givenname: Alexey V. surname: Medvedko fullname: Medvedko, Alexey V. organization: Department of Chemistry, M.V. Lomonosov Moscow State University, 1/3 Leninskye Gory, Moscow, 119991, Russia – sequence: 5 givenname: Andrey A. surname: Vashchenko fullname: Vashchenko, Andrey A. organization: P.N. Lebedev Physical Institute, Leninsky Prosp. 53, Moscow, 119992, Russia – sequence: 6 givenname: Alexander S. surname: Goloveshkin fullname: Goloveshkin, Alexander S. organization: A. N. Nesmeyanov Institute of Organoelement Compounds, Vavilova Str., 28, Moscow, 117312, Russia – sequence: 7 givenname: Dmitry M. surname: Tsymbarenko fullname: Tsymbarenko, Dmitry M. organization: Department of Chemistry, M.V. Lomonosov Moscow State University, 1/3 Leninskye Gory, Moscow, 119991, Russia – sequence: 8 givenname: Alexey A. surname: Averin fullname: Averin, Alexey A. organization: A. N. Frumkin Institute of Physical Chemistry and Electrochemistry, Leninsky Prosp. 31/5 P.2, Moscow, 119071, Russia – sequence: 9 givenname: Anna surname: Meschkov fullname: Meschkov, Anna organization: Institute of Functional Interfaces, Karlsruhe Institute of Technology, Karlsruhe, Germany – sequence: 10 givenname: Ute surname: Schepers fullname: Schepers, Ute organization: Institute of Functional Interfaces, Karlsruhe Institute of Technology, Karlsruhe, Germany – sequence: 11 givenname: Sergey Z. surname: Vatsadze fullname: Vatsadze, Sergey Z. organization: Department of Chemistry, M.V. Lomonosov Moscow State University, 1/3 Leninskye Gory, Moscow, 119991, Russia – sequence: 12 givenname: Valentina V. surname: Utochnikova fullname: Utochnikova, Valentina V. organization: Faculty of Materials Science, M.V. Lomonosov Moscow State University, 1/73 Leninskye Gory, Moscow, 119991, Russia |
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| Keywords | OLED Lanthanides Benzothiazole Carboxylates Luminescence Benzoxazole |
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| Title | On the design of new europium heteroaromatic carboxylates for OLED application |
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