Flexible, low-density polymer crosslinked silica aerogels
Polymerization of a di-isocyanate with the amine-modified surface of a sol–gel derived mesoporous silica network crosslinks the nanoparticles of the silica skeleton, and reinforces the otherwise fragile framework. Systematically adjusting the processing variables affecting density produce aerogels w...
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| Published in | Polymer (Guilford) Vol. 47; no. 16; pp. 5754 - 5761 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Oxford
Elsevier Ltd
26.07.2006
Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Polymerization of a di-isocyanate with the amine-modified surface of a sol–gel derived mesoporous silica network crosslinks the nanoparticles of the silica skeleton, and reinforces the otherwise fragile framework. Systematically adjusting the processing variables affecting density produce aerogels whose macroscopic properties could be controlled, and are attributed to changing nanoscale morphology. Aerogels crosslinked using the smallest amount of silica studied exhibit as much as a 40-fold increase in strength over the corresponding non-crosslinked framework, and are flexible. |
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| AbstractList | Polymerization of a di-isocyanate with the amine-modified surface of a sol-gel derived mesoporous silica network crosslinks the nanopar-ticles of the silica skeleton, and reinforces the otherwise fragile framework. Systematically adjusting the processing variables affecting density produce aerogels whose macroscopic properties could be controlled, and are attributed to changing nanoscale morphology. Aerogels crosslinked using the smallest amount of silica studied exhibit as much as a 40-fold increase in strength over the corresponding non-crosslinked framework, and are flexible. Polymerization of a di-isocyanate with the amine-modified surface of a sol–gel derived mesoporous silica network crosslinks the nanoparticles of the silica skeleton, and reinforces the otherwise fragile framework. Systematically adjusting the processing variables affecting density produce aerogels whose macroscopic properties could be controlled, and are attributed to changing nanoscale morphology. Aerogels crosslinked using the smallest amount of silica studied exhibit as much as a 40-fold increase in strength over the corresponding non-crosslinked framework, and are flexible. |
| Author | Meador, Mary Ann B. Fabrizio, Eve F. Leventis, Nicholas Capadona, Lynn A. Vassilaras, Plousia Alunni, Antonella |
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| Keywords | Mesoporous Di-isocyanates Polymer crosslinked aerogels Molecular structure Aerogel Hybrid material Mechanical properties Urea polymer Experimental study Polyaddition Silica Bending strength Organic diisocyanate Sol gel process Preparation Concentration effect Lattice structure Silicon polymer |
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| Snippet | Polymerization of a di-isocyanate with the amine-modified surface of a sol–gel derived mesoporous silica network crosslinks the nanoparticles of the silica... Polymerization of a di-isocyanate with the amine-modified surface of a sol-gel derived mesoporous silica network crosslinks the nanopar-ticles of the silica... |
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| SubjectTerms | Applied sciences Composites Di-isocyanates Exact sciences and technology Forms of application and semi-finished materials Mesoporous Polymer crosslinked aerogels Polymer industry, paints, wood Technology of polymers |
| Title | Flexible, low-density polymer crosslinked silica aerogels |
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