Viscosity investigation of natural gas hydrate slurries with anti-agglomerants additives
•Viscosity of natural gas hydrates slurry is investigated with anti-agglomerants.•Hydrates slurry viscosity model is developed based on Einstein effective medium theory.•Empirical correlations for non-Newtonian coefficient is extracted from experimental data.•Aggregation and broken of hydrates parti...
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| Published in | Fuel (Guildford) Vol. 185; pp. 323 - 338 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
01.12.2016
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| Subjects | |
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| Abstract | •Viscosity of natural gas hydrates slurry is investigated with anti-agglomerants.•Hydrates slurry viscosity model is developed based on Einstein effective medium theory.•Empirical correlations for non-Newtonian coefficient is extracted from experimental data.•Aggregation and broken of hydrates particles was considered by four dimensionless parameters.
The viscosity of natural gas hydrates slurry in high-pressure hydrates slurry rheological measurement system is investigated, which is meaningful for hydrates risk management to solve flow assurance issues in deep-water offshore field. Based on an appropriate stirring speed and time, a relatively uniform and stable hydrates slurry were formed from a water-in-oil emulsion to study the hydrates formation and slurry viscosity under different water cuts, bath temperatures and AAs concentrations. The influence of water cut on hydrates formation and hydrates slurry viscosity is much more significant than that of bath temperature and AAs concentration. Results indicate that the hydrates volume fraction, the continuous liquid phase viscosity and the dispersion degree of hydrates particles in the slurry are the critical factors to affect the viscosity of natural gas hydrates slurry. Considering both of aggregation and breakage of hydrates particles, a natural gas hydrates slurry viscosity semi-empirical model is developed based on the Einstein effective medium theory. The key parameter non-Newtonian coefficient K of this model is determined by several empirical correlations according to the experimental conditions and fluid properties. The consistence of predicted and experimental data demonstrates the feasibility of this model. |
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| AbstractList | •Viscosity of natural gas hydrates slurry is investigated with anti-agglomerants.•Hydrates slurry viscosity model is developed based on Einstein effective medium theory.•Empirical correlations for non-Newtonian coefficient is extracted from experimental data.•Aggregation and broken of hydrates particles was considered by four dimensionless parameters.
The viscosity of natural gas hydrates slurry in high-pressure hydrates slurry rheological measurement system is investigated, which is meaningful for hydrates risk management to solve flow assurance issues in deep-water offshore field. Based on an appropriate stirring speed and time, a relatively uniform and stable hydrates slurry were formed from a water-in-oil emulsion to study the hydrates formation and slurry viscosity under different water cuts, bath temperatures and AAs concentrations. The influence of water cut on hydrates formation and hydrates slurry viscosity is much more significant than that of bath temperature and AAs concentration. Results indicate that the hydrates volume fraction, the continuous liquid phase viscosity and the dispersion degree of hydrates particles in the slurry are the critical factors to affect the viscosity of natural gas hydrates slurry. Considering both of aggregation and breakage of hydrates particles, a natural gas hydrates slurry viscosity semi-empirical model is developed based on the Einstein effective medium theory. The key parameter non-Newtonian coefficient K of this model is determined by several empirical correlations according to the experimental conditions and fluid properties. The consistence of predicted and experimental data demonstrates the feasibility of this model. |
| Author | Wu, Hai-Hao Wang, Wei Gong, Jing Wang, Lin-Yan Yu, Da Liu, Hui-Shu Chai, Shuai Lv, Xiaofang Shi, Bo-Hui |
| Author_xml | – sequence: 1 givenname: Bo-Hui surname: Shi fullname: Shi, Bo-Hui email: bh.shi@cup.edu.cn organization: National Engineering Laboratory for Pipeline Safety/MOE Key Laboratory of Petroleum Engineering/Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, China University of Petroleum-Beijing, Changping, Beijing 102249, China – sequence: 2 givenname: Shuai surname: Chai fullname: Chai, Shuai organization: National Engineering Laboratory for Pipeline Safety/MOE Key Laboratory of Petroleum Engineering/Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, China University of Petroleum-Beijing, Changping, Beijing 102249, China – sequence: 3 givenname: Lin-Yan surname: Wang fullname: Wang, Lin-Yan organization: CNPC Research Institute of Safety & Environment Technology, Beijing Huayou Senior Engineering Supervision Co. Ltd, Langfang, Hebei 065000, China – sequence: 4 givenname: Xiaofang surname: Lv fullname: Lv, Xiaofang organization: Jiangsu Key Laboratory of Oil and Gas Storage & Transportation Technology, School of Petroleum Engineering, Changzhou University, Changzhou 213016, China – sequence: 5 givenname: Hui-Shu surname: Liu fullname: Liu, Hui-Shu organization: Department of Military Petroleum Supply Engineering, Logistical Engineering University, Shapingba, Chongqing 401311, China – sequence: 6 givenname: Hai-Hao surname: Wu fullname: Wu, Hai-Hao organization: National Engineering Laboratory for Pipeline Safety/MOE Key Laboratory of Petroleum Engineering/Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, China University of Petroleum-Beijing, Changping, Beijing 102249, China – sequence: 7 givenname: Wei surname: Wang fullname: Wang, Wei organization: National Engineering Laboratory for Pipeline Safety/MOE Key Laboratory of Petroleum Engineering/Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, China University of Petroleum-Beijing, Changping, Beijing 102249, China – sequence: 8 givenname: Da surname: Yu fullname: Yu, Da organization: National Engineering Laboratory for Pipeline Safety/MOE Key Laboratory of Petroleum Engineering/Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, China University of Petroleum-Beijing, Changping, Beijing 102249, China – sequence: 9 givenname: Jing surname: Gong fullname: Gong, Jing email: ydgj@cup.edu.cn organization: National Engineering Laboratory for Pipeline Safety/MOE Key Laboratory of Petroleum Engineering/Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, China University of Petroleum-Beijing, Changping, Beijing 102249, China |
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| Keywords | Viscosity Einstein effective medium theory Natural gas hydrates Hydrates slurry Anti-agglomerants |
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| SubjectTerms | Anti-agglomerants Einstein effective medium theory Hydrates slurry Natural gas hydrates Viscosity |
| Title | Viscosity investigation of natural gas hydrate slurries with anti-agglomerants additives |
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