Ag3PO4/reduced graphite oxide sheets nanocomposites with highly enhanced visible light photocatalytic activity and stability
[Display omitted] ► Ag3PO4/RGOs nanocomposites were firstly prepared by a facile approach. ► The composite shows high photocatalytic activity for organic dyes degradation. ► The composite exhibits enhanced photocatalytic and structural stability. ► RGOs could improve the stability of easily photocor...
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| Published in | Applied catalysis. B, Environmental Vol. 132-133; pp. 45 - 53 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Kidlington
Elsevier B.V
27.03.2013
Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
► Ag3PO4/RGOs nanocomposites were firstly prepared by a facile approach. ► The composite shows high photocatalytic activity for organic dyes degradation. ► The composite exhibits enhanced photocatalytic and structural stability. ► RGOs could improve the stability of easily photocorroded photocatalysts.
A series of Ag3PO4 and reduced graphite oxide sheets (RGOs) nanocomposites have been fabricated by a facile chemical precipitation approach in N,N-dimethylformamide (DMF) solvent without any hard/soft templates. The as-prepared Ag3PO4/RGOs composites were characterized by X-ray diffraction pattern (XRD), Fourier transform infrared spectra (FTIR), Raman spectroscopy, field emission scanning electron microscopy (SEM), transmission electron microscopy (TEM), and ultraviolet–visible (UV–vis) diffuse reflectance spectroscopy (DRS). It is found that the nano-sized Ag3PO4 particles are deposited on the surfaces of RGOs. The Ag3PO4/RGOs nanocomposites exhibit enhanced photocatalytic activity for the photodegradation of organic methyl orange (MO) and methylene blue (MB) under visible light irradiation. The photocatalytic rate of Ag3PO4/2.1wt% RGOs nanocomposite is 3 and 2 times of that of pure Ag3PO4 nanoparticles for the degradation of MO and MB, respectively. Furthermore, the photocatalytic and structural stability of Ag3PO4 is greatly enhanced. It is suggested that RGOs can be used as protective coatings that partially inhibit the photocorrosion of Ag3PO4. Overall, this work could provide a new approach to the improvement not only in the photocatalytic activity but also the stability of photocorrosion catalysts. |
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| AbstractList | [Display omitted]
► Ag3PO4/RGOs nanocomposites were firstly prepared by a facile approach. ► The composite shows high photocatalytic activity for organic dyes degradation. ► The composite exhibits enhanced photocatalytic and structural stability. ► RGOs could improve the stability of easily photocorroded photocatalysts.
A series of Ag3PO4 and reduced graphite oxide sheets (RGOs) nanocomposites have been fabricated by a facile chemical precipitation approach in N,N-dimethylformamide (DMF) solvent without any hard/soft templates. The as-prepared Ag3PO4/RGOs composites were characterized by X-ray diffraction pattern (XRD), Fourier transform infrared spectra (FTIR), Raman spectroscopy, field emission scanning electron microscopy (SEM), transmission electron microscopy (TEM), and ultraviolet–visible (UV–vis) diffuse reflectance spectroscopy (DRS). It is found that the nano-sized Ag3PO4 particles are deposited on the surfaces of RGOs. The Ag3PO4/RGOs nanocomposites exhibit enhanced photocatalytic activity for the photodegradation of organic methyl orange (MO) and methylene blue (MB) under visible light irradiation. The photocatalytic rate of Ag3PO4/2.1wt% RGOs nanocomposite is 3 and 2 times of that of pure Ag3PO4 nanoparticles for the degradation of MO and MB, respectively. Furthermore, the photocatalytic and structural stability of Ag3PO4 is greatly enhanced. It is suggested that RGOs can be used as protective coatings that partially inhibit the photocorrosion of Ag3PO4. Overall, this work could provide a new approach to the improvement not only in the photocatalytic activity but also the stability of photocorrosion catalysts. A series of Ag3PO4 and reduced graphite oxide sheets (RGOs) nanocomposites have been fabricated by a facile chemical precipitation approach in N,N-dimethylformamide (DMF) solvent without any hard/soft templates. The as-prepared Ag3PO4/RGOs composites were characterized by X-ray diffraction pattern (XRD), Fourier transform infrared spectra (FTIR), Raman spectroscopy, field emission scanning electron microscopy (SEM), transmission electron microscopy (TEM), and ultravioletavisible (UV-vis) diffuse reflectance spectroscopy (DRS). It is found that the nano-sized Ag3PO4 particles are deposited on the surfaces of RGOs. The Ag3PO4/RGOs nanocomposites exhibit enhanced photocatalytic activity for the photodegradation of organic methyl orange (MO) and methylene blue (MB) under visible light irradiation. The photocatalytic rate of Ag3PO4/2.1 wt% RGOs nanocomposite is 3 and 2 times of that of pure Ag3PO4 nanoparticles for the degradation of MO and MB, respectively. Furthermore, the photocatalytic and structural stability of Ag3PO4 is greatly enhanced. It is suggested that RGOs can be used as protective coatings that partially inhibit the photocorrosion of Ag3PO4. Overall, this work could provide a new approach to the improvement not only in the photocatalytic activity but also the stability of photocorrosion catalysts. |
| Author | Dong, Pengyu Li, Fenghua Xin, Shuangyu Wang, Yuhua Cao, Baocheng Guo, Linna Zhang, Jia |
| Author_xml | – sequence: 1 givenname: Pengyu surname: Dong fullname: Dong, Pengyu – sequence: 2 givenname: Yuhua surname: Wang fullname: Wang, Yuhua email: wyh@lzu.edu.cn – sequence: 3 givenname: Baocheng surname: Cao fullname: Cao, Baocheng – sequence: 4 givenname: Shuangyu surname: Xin fullname: Xin, Shuangyu – sequence: 5 givenname: Linna surname: Guo fullname: Guo, Linna – sequence: 6 givenname: Jia surname: Zhang fullname: Zhang, Jia – sequence: 7 givenname: Fenghua surname: Li fullname: Li, Fenghua |
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| Keywords | Silver orthophosphate Nanocomposite Stability Photocatalysis Reduced graphite oxide sheets Silver Heterogeneous catalysis Graphite oxide Graphite Silver phosphate Transition metal Environmental protection |
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► Ag3PO4/RGOs nanocomposites were firstly prepared by a facile approach. ► The composite shows high photocatalytic activity for organic dyes... A series of Ag3PO4 and reduced graphite oxide sheets (RGOs) nanocomposites have been fabricated by a facile chemical precipitation approach in... |
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| SubjectTerms | Catalysis Chemistry Exact sciences and technology General and physical chemistry Graphite Nanocomposite Nanocomposites Nanostructure Oxides Photocatalysis Photochemistry Physical chemistry of induced reactions (with radiations, particles and ultrasonics) Reduced graphite oxide sheets Scanning electron microscopy Silver orthophosphate Stability Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry |
| Title | Ag3PO4/reduced graphite oxide sheets nanocomposites with highly enhanced visible light photocatalytic activity and stability |
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