Permeability and Selectivity of Sulfur Dioxide and Carbon Dioxide in Supported Ionic Liquid Membranes
Permeabilities and selectivities of gases such as carbon dioxide （CO2）, sulfur dioxide （SO2）, nitrogen （N2） and methane （CH4） in six imidazolium-based ionic liquids （[emim][BF4], [bmim][BF4], [bmim][PF6], [banim][BF4], [bmim][Tf2N] and [emim][CF3SO3]） supported on polyethersulfone microfiltration me...
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| Published in | Chinese journal of chemical engineering Vol. 17; no. 4; pp. 594 - 601 |
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| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
2009
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1004-9541 2210-321X |
| DOI | 10.1016/S1004-9541(08)60249-9 |
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| Abstract | Permeabilities and selectivities of gases such as carbon dioxide （CO2）, sulfur dioxide （SO2）, nitrogen （N2） and methane （CH4） in six imidazolium-based ionic liquids （[emim][BF4], [bmim][BF4], [bmim][PF6], [banim][BF4], [bmim][Tf2N] and [emim][CF3SO3]） supported on polyethersulfone microfiltration membranes are investigated in a single gas feed system using nitrogen as the environment and reference component at temperature from 25 to 45℃ and pressure of N2 from 100 to 400 kPa. It is found that SO2 has the highest permeability in the tested supported ionic liquid membranes, being an order of magnitude higher than that of CO2, and about 2 to 3 orders of magnitude larger than those of N2 and CH4. The observed selectivity of SO2 over the two ordinary gas components is also striking. It is shown experimentally that the dissolution and transport of gas components in the supported ionic liquid membranes, as well as the nature of ionic liquids play important roles in the gas permeation. A nonlinear increase of permeation rate with temperature and operation pressure is also observed for all sample gases. By considering the factors that influence the permeabilities and selectivities of CO2 and SO2, it is expected to develop an optimal supported ionic liquid membrane technology for the isolation of acidic gases in the near future. |
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| AbstractList | Permeabilities and selectivities of gases such as carbon dioxide (CO
2), sulfur dioxide (SO
2), nitrogen (N
2) and methane (CH
4) in six imidazolium-based ionic liquids ([emim][BF
4], [bmim][BF
4], [bmim][PF
6], [hmim][BF
4], [bmim][Tf
2N] and [emim][CF
3SO
3]) supported on polyethersulfone microfiltration membranes are investigated in a single gas feed system using nitrogen as the environment and reference component at temperature from 25 to 45°C and pressure of N
2 from 100 to 400 kPa. It is found that SO
2 has the highest permeability in the tested supported ionic liquid membranes, being an order of magnitude higher than that of CO
2, and about 2 to 3 orders of magnitude larger than those of N
2 and CH
4. The observed selectivity of SO
2 over the two ordinary gas components is also striking. It is shown experimentally that the dissolution and transport of gas components in the supported ionic liquid membranes, as well as the nature of ionic liquids play important roles in the gas permeation. A nonlinear increase of permeation rate with temperature and operation pressure is also observed for all sample gases. By considering the factors that influence the permeabilities and selectivities of CO
2 and SO
2, it is expected to develop an optimal supported ionic liquid membrane technology for the isolation of acidic gases in the near future. Permeabilities and selectivities of gases such as carbon dioxide (CO sub(2)), sulfur dioxide (SO sub(2)), nitrogen (N sub(2)) and methane (CH sub(4)) in six imidazolium-based ionic liquids ([emim][BF sub(4)], [bmim][BF sub(4)], [bmim][PF sub(6)], [hmim][BF sub(4)], [bmim][Tf sub(2)N] and [emim][CF sub(3)SO sub(3)]) supported on polyethersulfone microfiltration membranes are investigated in a single gas feed system using nitrogen as the environment and reference component at temperature from 25 to 45 degree C and pressure of N sub(2) from 100 to 400 kPa. It is found that SO sub(2) has the highest permeability in the tested supported ionic liquid membranes, being an order of magnitude higher than that of CO sub(2), and about 2 to 3 orders of magnitude larger than those of N sub(2) and CH sub(4). The observed selectivity of SO sub(2) over the two ordinary gas components is also striking. It is shown experimentally that the dissolution and transport of gas components in the supported ionic liquid membranes, as well as the nature of ionic liquids play important roles in the gas permeation. A nonlinear increase of permeation rate with temperature and operation pressure is also observed for all sample gases. By considering the factors that influence the permeabilities and selectivities of CO sub(2) and SO sub(2), it is expected to develop an optimal supported ionic liquid membrane technology for the isolation of acidic gases in the near future. Permeabilities and selectivities of gases such as carbon dioxide （CO2）, sulfur dioxide （SO2）, nitrogen （N2） and methane （CH4） in six imidazolium-based ionic liquids （[emim][BF4], [bmim][BF4], [bmim][PF6], [banim][BF4], [bmim][Tf2N] and [emim][CF3SO3]） supported on polyethersulfone microfiltration membranes are investigated in a single gas feed system using nitrogen as the environment and reference component at temperature from 25 to 45℃ and pressure of N2 from 100 to 400 kPa. It is found that SO2 has the highest permeability in the tested supported ionic liquid membranes, being an order of magnitude higher than that of CO2, and about 2 to 3 orders of magnitude larger than those of N2 and CH4. The observed selectivity of SO2 over the two ordinary gas components is also striking. It is shown experimentally that the dissolution and transport of gas components in the supported ionic liquid membranes, as well as the nature of ionic liquids play important roles in the gas permeation. A nonlinear increase of permeation rate with temperature and operation pressure is also observed for all sample gases. By considering the factors that influence the permeabilities and selectivities of CO2 and SO2, it is expected to develop an optimal supported ionic liquid membrane technology for the isolation of acidic gases in the near future. |
| Author | 江滢滢 吴有庭 王文婷 李磊 周政 张志炳 |
| AuthorAffiliation | Key Laboratory of Mesoscopic Chemistry of MOE, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210093, China |
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| Cites_doi | 10.1021/ie0704142 10.1002/anie.200353437 10.1021/ie048825v 10.1002/1521-3765(20020816)8:16<3671::AID-CHEM3671>3.0.CO;2-9 10.1016/j.memsci.2006.02.016 10.1021/ja017593d 10.1016/j.memsci.2004.02.033 10.1016/S0376-7388(00)80018-6 10.1021/jp046404l 10.1016/j.jct.2005.07.002 10.1016/S1383-5866(01)00124-1 10.1016/S1383-5866(00)00216-1 10.1016/j.memsci.2006.03.030 10.1021/jp071742i 10.1021/ie060177n 10.1039/b103275p 10.1016/S0022-1139(99)00267-5 10.1021/ic951325x 10.1038/nature04451 10.1081/SS-120001451 10.1016/j.memsci.2006.03.015 |
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| Keywords | ionic liquid supported ionic liquid membrane permeation gas separation acidic gas |
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| Snippet | Permeabilities and selectivities of gases such as carbon dioxide （CO2）, sulfur dioxide （SO2）, nitrogen （N2） and methane （CH4） in six imidazolium-based ionic... Permeabilities and selectivities of gases such as carbon dioxide (CO 2), sulfur dioxide (SO 2), nitrogen (N 2) and methane (CH 4) in six imidazolium-based... Permeabilities and selectivities of gases such as carbon dioxide (CO sub(2)), sulfur dioxide (SO sub(2)), nitrogen (N sub(2)) and methane (CH sub(4)) in six... |
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| SubjectTerms | acidic gas Carbon dioxide Dissolution gas separation ionic liquid Ionic liquids Membranes Permeability Permeation Selectivity Sulfur dioxide supported ionic liquid membrane 二氧化硫 二氧化碳 气体成分 渗透性 离子液体 离子选择性 |
| Title | Permeability and Selectivity of Sulfur Dioxide and Carbon Dioxide in Supported Ionic Liquid Membranes |
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