Thermodynamic calculation of intermetallic compounds in AZ91 alloy containing calcium
Based on the Miedema model and Chou model, the activities of different solute components in Mg-Al-Zn, Mg-Ca-Zn and Mg-Al-Ca ternary systems were calculated. The results show that the variety of zinc content has little influence on the activity of Al or Ca, and the interaction of Zn and Al or Ca can...
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| Published in | Transactions of Nonferrous Metals Society of China Vol. 16; no. 2; pp. 392 - 396 |
|---|---|
| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
01.04.2006
College of Materials Science and Engineering, Beijing University of Technology, Beijing 100022, China |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1003-6326 |
| DOI | 10.1016/S1003-6326(06)60067-8 |
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| Abstract | Based on the Miedema model and Chou model, the activities of different solute components in Mg-Al-Zn, Mg-Ca-Zn and Mg-Al-Ca ternary systems were calculated. The results show that the variety of zinc content has little influence on the activity of Al or Ca, and the interaction of Zn and Al or Ca can be neglected when the mass fraction of Zn is lower than 2% in the AZ91 alloy containing calcium （noted as Mg-Al-Zn-Ca system）. Therefore, the possible intermetallic compounds in the Mg-Al-Zn-Ca system can be predicted by directly calculating the Gibbs flee energies of the reactions in Mg-Al-Ca system. The calculated Gibbs flee energies in the Mg-Al-Ca system indicate that Al2Ca phase can take priority of depositing, which agrees with the experimental results in references. The consistency of calculation and experiment proves that the intermetallic compounds in the Mg-Al-Zn-Ca system can be predicted by the Miedema model and Chou model. |
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| AbstractList | Based on the Miedema model and Chou model, the activities of different solute components in Mg-Al-Zn, Mg-Ca-Zn and Mg-Al-Ca ternary systems were calculated. The results show that the variety of zinc content has little influence on the activity of Al or Ca, and the interaction of Zn and Al or Ca can be neglected when the mass fraction of Zn is lower than 2% in the AZ91 alloy containing calcium （noted as Mg-Al-Zn-Ca system）. Therefore, the possible intermetallic compounds in the Mg-Al-Zn-Ca system can be predicted by directly calculating the Gibbs flee energies of the reactions in Mg-Al-Ca system. The calculated Gibbs flee energies in the Mg-Al-Ca system indicate that Al2Ca phase can take priority of depositing, which agrees with the experimental results in references. The consistency of calculation and experiment proves that the intermetallic compounds in the Mg-Al-Zn-Ca system can be predicted by the Miedema model and Chou model. Based on the Miedema model and Chou model, the activities of different solute components in Mg-Al-Zn, Mg-Ca-Zn and Mg-Al-Ca ternary systems were calculated. The results show that the variety of zinc content has little influence on the activity of Al or Ca, and the interaction of Zn and Al or Ca can be neglected when the mass fraction of Zn is lower than 2% in the AZ91 alloy containing calcium (noted as Mg-Al-Zn-Ca system). Therefore, the possible intermetallic compounds in the Mg-Al-Zn-Ca system can be predicted by directly calculating the Gibbs free energies of the reactions in Mg-Al-Ca system. The calculated Gibbs free energies in the Mg-Al-Ca system indicate that Al 2Ca phase can take priority of depositing, which agrees with the experimental results in references. The consistency of calculation and experiment proves that the intermetallic compounds in the Mg-Al-Zn-Ca system can be predicted by the Miedema model and Chou model. TG29; Based on the Miedema model and Chou model, the activities of different solute components in Mg-Al-Zn, Mg-Ca-Zn and Mg-Al-Ca ternary systems were calculated. The results show that the variety of zinc content has little influence on the activity of Al or Ca, and the interaction of Zn and Al or Ca can be neglected when the mass fraction of Zn is lower than 2% in the AZ91 alloy containing calcium (noted as Mg-Al-Zn-Ca system). Therefore, the possible intermetallic compounds in the Mg-Al-Zn-Ca system can be predicted by directly calculating the Gibbs free energies of the reactions in Mg-Al-Ca system. The calculated Gibbs free energies in the Mg-Al-Ca system indicate that Al2Ca phase can take priority of depositing, which agrees with the experimental results in references. The consistency of calculation and experiment proves that the intermetallic compounds in the Mg-Al-Zn-Ca system can be predicted by the Miedema model and Chou model. Based on the Miedema model and Chou model, the activities of different solute components in Mg-Al-Zn, Mg-Ca-Zn and Mg-Al-Ca ternary systems were calculated. The results show that the variety of zinc content has little influence on the activity of Al or Ca, and the interaction of Zn and Al or Ca can be neglected when the mass fraction of Zn is lower than 2% in the AZ91 alloy containing calcium (noted as Mg-Al-Zn-Ca system). Therefore, the possible intermetallic compounds in the Mg-Al-Zn-Ca system can be predicted by directly calculating the Gibbs free energies of the reactions in Mg-Al-Ca system. The calculated Gibbs free energies in the Mg-Al-Ca system indicate that Al(2)Ca phase can take priority of depositing, which agrees with the experimental results in references. The consistency of calculation and experiment proves that the intermetallic compounds in the Mg-Al-Zn-Ca system can be predicted by the Miedema model and Chou model. |
| Author | 吴玉锋 杜文博 聂祚仁 曹林锋 左铁镛 |
| AuthorAffiliation | College of Materials Science and Engineering, Beijing University of Technology, Beijing 100022, China |
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| Cites_doi | 10.1016/S0921-5093(02)00551-8 10.1016/S0921-5093(99)00604-8 10.1016/S0254-0584(02)00312-7 10.1023/A:1016567421956 10.1007/s11661-005-0154-8 |
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| Keywords | AZ91 alloy Mg-Ca-Zn alloy Gibbs free energy Mg-Al-Ca alloy Chou model Al 2Ca Mg-Al-Zn alloy Miedema model Al2Ca |
| Language | English |
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| Notes | Al2Ca AZ91 alloy; Mg-Al-Zn alloy; Mg-Ca-Zn alloy; Mg-Al-Ca alloy; Al2Ca; Miedema model; Chou model; Gibbs freeenergy AZ91 alloy Mg-Ca-Zn alloy Mg-Al-Ca alloy 43-1239/TG Chou model Gibbs freeenergy Mg-Al-Zn alloy Miedema model TG146.22 ObjectType-Article-2 SourceType-Scholarly Journals-1 ObjectType-Feature-1 content type line 23 |
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| Snippet | Based on the Miedema model and Chou model, the activities of different solute components in Mg-Al-Zn, Mg-Ca-Zn and Mg-Al-Ca ternary systems were calculated.... TG29; Based on the Miedema model and Chou model, the activities of different solute components in Mg-Al-Zn, Mg-Ca-Zn and Mg-Al-Ca ternary systems were... |
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| SubjectTerms | Al 2Ca Al2Ca AZ91 alloy AZ91合金 Chou model Gibbs free energy Mg-Al-Ca Mg-Al-Ca alloy Mg-Al-Zn Mg-Al-Zn alloy Mg-Ca-Zn Mg-Ca-Zn alloy Miedema model 热力学计算 金属间化合物 镁合金 |
| Title | Thermodynamic calculation of intermetallic compounds in AZ91 alloy containing calcium |
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