Robust, stretchable and photothermal self-healing polyurethane elastomer based on furan-modified polydopamine nanoparticles
The realization of high strengthen, large ductility, and multiple-responding for self-healing composites is an urgent problem to be solved for expanding practical applications in industry. Herein, a simple stagey was proposed to prepare multiple-responding self-healing composites, which possess outs...
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| Published in | Polymer (Guilford) Vol. 190; p. 122219 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Kidlington
Elsevier Ltd
02.03.2020
Elsevier BV |
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| Online Access | Get full text |
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| Abstract | The realization of high strengthen, large ductility, and multiple-responding for self-healing composites is an urgent problem to be solved for expanding practical applications in industry. Herein, a simple stagey was proposed to prepare multiple-responding self-healing composites, which possess outstanding both tensile strengths also ductility, by utilizing furfuryl-modified polydopamine particles (F-PDAPs) as crosslinkers in maleimide-terminated polyurethane (m-PU) based on Diels-Alder reaction. Due to the excellent photo-thermal effect of F-PDAPs and the existence of DA bonds, the composites exhibited excellent healing efficiency under NIR (91.83%) and thermal (92.54%) initiation, in particular, could locally and specifically repair any crack under near-infrared light conditions. Furthermore, the tensile strength of composite materials was reached up to 34.26 MPa with a high breaking strain of 800%. Besides, the composites exhibited outstanding adhesive strength that could be healed via thermally induced. Such excellent comprehensive performance gives the composite materials an opportunity to have great potential in the fields of coatings, binders, etc.
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•The self-healing composites possess outstanding tensile strengths also ductility.•The composites can realize specifically healing under NIR irradiation.•The composites have good adhesive strength that can be healed by thermal-induced. |
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| AbstractList | The realization of high strengthen, large ductility, and multiple-responding for self-healing composites is an urgent problem to be solved for expanding practical applications in industry. Herein, a simple stagey was proposed to prepare multiple-responding self-healing composites, which possess outstanding both tensile strengths also ductility, by utilizing furfuryl-modified polydopamine particles (F-PDAPs) as crosslinkers in maleimide-terminated polyurethane (m-PU) based on Diels-Alder reaction. Due to the excellent photo-thermal effect of F-PDAPs and the existence of DA bonds, the composites exhibited excellent healing efficiency under NIR (91.83%) and thermal (92.54%) initiation, in particular, could locally and specifically repair any crack under near-infrared light conditions. Furthermore, the tensile strength of composite materials was reached up to 34.26 MPa with a high breaking strain of 800%. Besides, the composites exhibited outstanding adhesive strength that could be healed via thermally induced. Such excellent comprehensive performance gives the composite materials an opportunity to have great potential in the fields of coatings, binders, etc. The realization of high strengthen, large ductility, and multiple-responding for self-healing composites is an urgent problem to be solved for expanding practical applications in industry. Herein, a simple stagey was proposed to prepare multiple-responding self-healing composites, which possess outstanding both tensile strengths also ductility, by utilizing furfuryl-modified polydopamine particles (F-PDAPs) as crosslinkers in maleimide-terminated polyurethane (m-PU) based on Diels-Alder reaction. Due to the excellent photo-thermal effect of F-PDAPs and the existence of DA bonds, the composites exhibited excellent healing efficiency under NIR (91.83%) and thermal (92.54%) initiation, in particular, could locally and specifically repair any crack under near-infrared light conditions. Furthermore, the tensile strength of composite materials was reached up to 34.26 MPa with a high breaking strain of 800%. Besides, the composites exhibited outstanding adhesive strength that could be healed via thermally induced. Such excellent comprehensive performance gives the composite materials an opportunity to have great potential in the fields of coatings, binders, etc. [Display omitted] •The self-healing composites possess outstanding tensile strengths also ductility.•The composites can realize specifically healing under NIR irradiation.•The composites have good adhesive strength that can be healed by thermal-induced. |
| ArticleNumber | 122219 |
| Author | Zhou, Mi Cheng, Xu Yang, Shiwen Wang, Haibo Yan, Bin Du, Zongliang Du, Xiaosheng |
| Author_xml | – sequence: 1 givenname: Shiwen surname: Yang fullname: Yang, Shiwen organization: College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065, PR China – sequence: 2 givenname: Xiaosheng orcidid: 0000-0001-8239-4303 surname: Du fullname: Du, Xiaosheng organization: College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065, PR China – sequence: 3 givenname: Zongliang surname: Du fullname: Du, Zongliang organization: College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065, PR China – sequence: 4 givenname: Mi surname: Zhou fullname: Zhou, Mi organization: College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065, PR China – sequence: 5 givenname: Xu surname: Cheng fullname: Cheng, Xu organization: College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065, PR China – sequence: 6 givenname: Haibo orcidid: 0000-0001-5321-8888 surname: Wang fullname: Wang, Haibo email: whb6985@scu.edu.cn organization: College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065, PR China – sequence: 7 givenname: Bin surname: Yan fullname: Yan, Bin email: yanbinscu@126.com organization: College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065, PR China |
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| SubjectTerms | Adhesive strength Binders Composite materials Crack initiation Crosslinking Diels-Alder reactions Ductility Elastomers Industrial applications Infrared radiation Mechanical enhancement Multiple stimuli Nanoparticles Polyurethane Polyurethane resins Self healing materials Self-healing Temperature effects Tensile strength |
| Title | Robust, stretchable and photothermal self-healing polyurethane elastomer based on furan-modified polydopamine nanoparticles |
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