Synthesis, Characterization, and Environmental Applications of Cu-Ni-Doped Bismuth Molybdate

Bismuthoxide-based catalysts gained attention for photocatalytic remediation of environmental pollutants owing to their low cost, feasibility, stability, small, and tunable band gap. In the present work, bismuth molybdate was modified via transition metal doping to achieve maximum catalytic efficien...

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Published inNanomaterials and nanotechnology Vol. 2023; pp. 1 - 17
Main Authors Sehar, Kashaf, Saeed, Muhammad, Murtaza, Maida, Zahra, Manzar, Waseem, Amir
Format Journal Article
LanguageEnglish
Published London Hindawi 2023
John Wiley & Sons, Inc
Wiley
Subjects
Bismuth
Catalysts
Caustic soda
Chemical synthesis
Chemicals
Comparative studies
Copper
Dyes
Efficiency
Electrons
Energy gap
Heavy metals
Malachite green
Methods
Mineralization
Nickel
Nitrates
Oxidation
Performance degradation
Photocatalysis
Photodegradation
Pollutants
Raman spectroscopy
Rate constants
Rhodamine
Spectrophotometry
Transition metals
Online AccessGet full text
ISSN1847-9804
1847-9804
DOI10.1155/2023/9793804

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Abstract Bismuthoxide-based catalysts gained attention for photocatalytic remediation of environmental pollutants owing to their low cost, feasibility, stability, small, and tunable band gap. In the present work, bismuth molybdate was modified via transition metal doping to achieve maximum catalytic efficiency. This aim was accomplished by synthesizing novel Cu2+ and Ni2+ codoped bismuth molybdate (CuNi/Bi2MoO6, Cu/Bi2MoO6, and Ni/Bi2MoO6) which were utilized for heavy metal reduction and dyes degradation. Pure bismuth molybdate was also fabricated for comparative studies. All the prepared samples were characterized by XRD, Raman spectroscopy, SEM, and EDX. Optical studies for band gap calculations were carried out by UV-Visible spectrophotometry and decrease in band gap was observed in doped materials. Pseudo-first-order kinetic studies were performed to find the rate constants and regression values for Cr(VI) reduction and degradation of rhodamine B and malachite green using CuNi/Bi2MoO6. Codoped bismuth molybdate exhibited more than 95% photocatalytic performance for Cr(VI) reduction and degradation of rhodamine B and malachite green dyes. Reusability of catalyst was confirmed up to six cycles. Considering its catalytic proficiency, CuNi/Bi2MoO6 is anticipated to be utilized for more environment friendly applications in future.
AbstractList Bismuthoxide-based catalysts gained attention for photocatalytic remediation of environmental pollutants owing to their low cost, feasibility, stability, small, and tunable band gap. In the present work, bismuth molybdate was modified via transition metal doping to achieve maximum catalytic efficiency. This aim was accomplished by synthesizing novel Cu2+ and Ni2+ codoped bismuth molybdate (CuNi/Bi2MoO6, Cu/Bi2MoO6, and Ni/Bi2MoO6) which were utilized for heavy metal reduction and dyes degradation. Pure bismuth molybdate was also fabricated for comparative studies. All the prepared samples were characterized by XRD, Raman spectroscopy, SEM, and EDX. Optical studies for band gap calculations were carried out by UV-Visible spectrophotometry and decrease in band gap was observed in doped materials. Pseudo-first-order kinetic studies were performed to find the rate constants and regression values for Cr(VI) reduction and degradation of rhodamine B and malachite green using CuNi/Bi2MoO6. Codoped bismuth molybdate exhibited more than 95% photocatalytic performance for Cr(VI) reduction and degradation of rhodamine B and malachite green dyes. Reusability of catalyst was confirmed up to six cycles. Considering its catalytic proficiency, CuNi/Bi2MoO6 is anticipated to be utilized for more environment friendly applications in future.
Author Sehar, Kashaf
Saeed, Muhammad
Zahra, Manzar
Waseem, Amir
Murtaza, Maida
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CitedBy_id crossref_primary_10_3390_ijms252313104
crossref_primary_10_1016_j_cattod_2025_115238
crossref_primary_10_1016_j_dwt_2024_100589
crossref_primary_10_1080_1536383X_2024_2399243
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Copyright Copyright © 2023 Kashaf Sehar et al.
Copyright © 2023 Kashaf Sehar et al. This is an open access article distributed under the Creative Commons Attribution License (the “License”), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. https://creativecommons.org/licenses/by/4.0
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Snippet Bismuthoxide-based catalysts gained attention for photocatalytic remediation of environmental pollutants owing to their low cost, feasibility, stability,...
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SubjectTerms Bismuth
Catalysts
Caustic soda
Chemical synthesis
Chemicals
Comparative studies
Copper
Dyes
Efficiency
Electrons
Energy gap
Heavy metals
Malachite green
Methods
Mineralization
Nickel
Nitrates
Oxidation
Performance degradation
Photocatalysis
Photodegradation
Pollutants
Raman spectroscopy
Rate constants
Rhodamine
Spectrophotometry
Transition metals
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Title Synthesis, Characterization, and Environmental Applications of Cu-Ni-Doped Bismuth Molybdate
URI https://dx.doi.org/10.1155/2023/9793804
https://www.proquest.com/docview/3107126558
https://doaj.org/article/d0d7eda5e4bb4e02b250e05f64464407
Volume 2023
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