Hydrolytic degradation of polylactic acid (PLA) and its composites
Biodegradable polymers are seen as a potential solution to the environmental problems generated by plastic waste. In particular, the renewable aliphatic polyesters of poly(hydroxyacid)-type homopolymers and copolymers consisting of polylactic acid (PLA), poly(glycolic acid) (PGA), and poly(e-caprola...
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| Published in | Renewable & sustainable energy reviews Vol. 79; pp. 1346 - 1352 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
01.11.2017
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Biodegradable polymers are seen as a potential solution to the environmental problems generated by plastic waste. In particular, the renewable aliphatic polyesters of poly(hydroxyacid)-type homopolymers and copolymers consisting of polylactic acid (PLA), poly(glycolic acid) (PGA), and poly(e-caprolactone) (PCL) constitute the most promising bioresorbable materials for applications in biomedical and consumer applications. Among those polymers, PLA has attracted particular attention as a substitute for conventional petroleum-based plastics. PLA is synthesized by the fermentation of renewable agricultural sources, including corn, cellulose, and other polysaccharides. Although some of its characteristics are disadvantageous (e.g., poor melt properties, mechanical brittleness, low heat resistance, and slow crystallization), there exist potential routes to resolve these shortcomings. These include copolymerization, blending, plasticization modification, or the addition of reinforcing phases (e.g., chitosan (Cs), cellulose, and starch). In this review, we discuss the degradation mechanisms of PLA and its modified form in the environment, current issues that hinder the achievement of good Cs/PLA combination, and ways to overcome some of these problems. Furthermore, our discussion is extended to cover the subjects of hydrolytic degradation and weathering effects with different Cs/PLA blends. |
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| AbstractList | Biodegradable polymers are seen as a potential solution to the environmental problems generated by plastic waste. In particular, the renewable aliphatic polyesters of poly(hydroxyacid)-type homopolymers and copolymers consisting of polylactic acid (PLA), poly(glycolic acid) (PGA), and poly(e-caprolactone) (PCL) constitute the most promising bioresorbable materials for applications in biomedical and consumer applications. Among those polymers, PLA has attracted particular attention as a substitute for conventional petroleum-based plastics. PLA is synthesized by the fermentation of renewable agricultural sources, including corn, cellulose, and other polysaccharides. Although some of its characteristics are disadvantageous (e.g., poor melt properties, mechanical brittleness, low heat resistance, and slow crystallization), there exist potential routes to resolve these shortcomings. These include copolymerization, blending, plasticization modification, or the addition of reinforcing phases (e.g., chitosan (Cs), cellulose, and starch). In this review, we discuss the degradation mechanisms of PLA and its modified form in the environment, current issues that hinder the achievement of good Cs/PLA combination, and ways to overcome some of these problems. Furthermore, our discussion is extended to cover the subjects of hydrolytic degradation and weathering effects with different Cs/PLA blends. |
| Author | Elsawy, Moataz A. Deep, Akash Kim, Ki-Hyun Park, Jae-Woo |
| Author_xml | – sequence: 1 givenname: Moataz A. surname: Elsawy fullname: Elsawy, Moataz A. organization: Polymer laboratory, Petrochemical Department, Egyptian Petroleum Research Institute, Nasr City 11727, Cairo, Egypt – sequence: 2 givenname: Ki-Hyun surname: Kim fullname: Kim, Ki-Hyun email: kkim61@hanyang.ac.kr organization: Department of Civil and Environmental Engineering, Hanyang University, 222, Wangsimni-Ro, Seoul 04763, Korea – sequence: 3 givenname: Jae-Woo surname: Park fullname: Park, Jae-Woo organization: Department of Civil and Environmental Engineering, Hanyang University, 222, Wangsimni-Ro, Seoul 04763, Korea – sequence: 4 givenname: Akash surname: Deep fullname: Deep, Akash email: dr.akashdeep@csio.res.in organization: Central Scientific Instruments Organisation (CSIR-CSIO), Sector 30C, Chandigarh 160030, India |
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