Structural study of the Ag(1 1 0) c(2 × 2)–Sb phase by low energy electron diffraction
This work concerns the deposition of Sb on the (1 1 0) clean surface of silver. Two structured phases have been observed: an Ag(1 1 0)(4 × 1)–Sb, with a Sb coverage of about 1.0 ML and an Ag(1 1 0) c(2 × 2)–Sb, with half the coverage of the first one. The structural determination of the Ag(1 1 0) c(...
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Published in | Surface science Vol. 572; no. 2; pp. 337 - 346 |
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Main Authors | , , , , , , |
Format | Journal Article |
Language | English |
Published |
Lausanne
Elsevier B.V
20.11.2004
Amsterdam Elsevier Science New York, NY |
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Abstract | This work concerns the deposition of Sb on the (1
1
0) clean surface of silver. Two structured phases have been observed: an Ag(1
1
0)(4
×
1)–Sb, with a Sb coverage of about 1.0
ML and an Ag(1
1
0)
c(2
×
2)–Sb, with half the coverage of the first one. The structural determination of the Ag(1
1
0)
c(2
×
2)–Sb phase has been performed by a standard LEED analysis and the results obtained indicate the presence of substitutional Sb atoms in the first atomic layer. The presence of the Sb substitutional atoms promotes an expansion in the first interlayer distance without any change in the surface thermal vibrational behaviour. Based on results obtained by this study and previously published ones, the substitutional site seems to be most energetically favourable for Sb atoms, in any of the low index surfaces of silver. |
---|---|
AbstractList | Sb plays the role of a surfactant in the homo-epitaxy growth of Ag on Ag(111), changing the growth mode from islanding to layer-on-layer. This work concerns the deposition of Sb on the (110) clean surface of silver. Two structured phases have been observed: an Ag(110)(4 x 1)-Sb, with a Sb coverage of about 1.0 ML and an Ag(110)c(2 x 2)-Sb, with half the coverage of the first one. The structural determination of the Ag(110)c(2 x 2)-Sb phase has been performed by a standard LEED analysis and the results obtained indicate the presence of substitutional Sb atoms in the first atomic layer. The presence of the Sb substitutional atoms promotes an expansion in the first interlayer distance without any change in the surface thermal vibrational behaviour. Based on results obtained by this study and previously published ones, the substitutional site seems to be most energetically favourable for Sb atoms, in any of the low index surfaces of silver. This work concerns the deposition of Sb on the (1 1 0) clean surface of silver. Two structured phases have been observed: an Ag(1 1 0)(4 × 1)–Sb, with a Sb coverage of about 1.0 ML and an Ag(1 1 0) c(2 × 2)–Sb, with half the coverage of the first one. The structural determination of the Ag(1 1 0) c(2 × 2)–Sb phase has been performed by a standard LEED analysis and the results obtained indicate the presence of substitutional Sb atoms in the first atomic layer. The presence of the Sb substitutional atoms promotes an expansion in the first interlayer distance without any change in the surface thermal vibrational behaviour. Based on results obtained by this study and previously published ones, the substitutional site seems to be most energetically favourable for Sb atoms, in any of the low index surfaces of silver. |
Author | Paniago, R. de Carvalho, V.E. Landers, R. de Siervo, A. de Castilho, C.M.C. Nascimento, V.B. Soares, E.A. |
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Cites_doi | 10.1016/S0039-6028(98)00509-3 10.1088/0953-8984/12/35/304 10.1103/PhysRevB.68.245408 10.1016/S0169-4332(03)00627-5 10.1016/S0039-6028(02)01488-7 10.1088/0953-8984/14/4/301 10.1063/1.1733573 10.1016/0039-6028(86)90777-6 10.1016/0039-6028(95)00401-7 10.3390/i3020087 10.1088/0022-3719/13/5/024 10.1103/PhysRevB.61.7706 10.1103/PhysRevB.61.13983 10.1103/PhysRevLett.68.3335 10.1103/PhysRevLett.72.3843 10.1016/S0039-6028(96)01139-9 10.1063/1.1725697 10.1088/0953-8984/10/39/004 10.1016/j.susc.2003.12.027 10.1016/0022-1902(73)80357-4 |
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Keywords | Silver Low energy electron diffraction (LEED) Antimony Surface structure, morphology, roughness, and topography and topography; Low energy electron diffraction (LEED) morphology Transition elements Roughness LEED Surface topography Coverage rate Antimony; Silver; Surface structure Surface structure |
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References | Nascimento, Soares, de Carvalho, Lopes, Paniago, de Castilho (bib28) 2003; 68 E.A. Soares, A. de Siervo, R. Landers, Universidade Estadual de Campinas—UNICAMP (private communication) Slater (bib17) 1964; 39 Slater (bib18) 1965 Ghosh, Biswas (bib21) 2002; 3 Soares, Bittencourt, Nascimento, de Carvalho, de Castilho, McConville, de Carvalho, Woodruff (bib6) 2000; 61 Van Hove, Weinberg, Chan (bib25) 1986 Woodruff, Robinson (bib29) 2000; 12 Loucks (bib24) 1976 Brown, Quinn, Woodruff (bib30) 2000; 61 Pendry (bib26) 1980; 13 Kittel (bib22) 1986 Woodruff, Robinson (bib31) 2003; 219 Jiang, Zhou, Qiu, Cao (bib4) 1998; 10 Vrijmoeth, van der Vegt, Meyer, Vlieg, Behm (bib2) 1994; 72 de Vries, Huisman, Goedtkindt, Zwanenburg, Bennet, Robinson, Vlieg (bib7) 1998; 414 Campbell (bib15) 1986; 167 A. Barbieri, M.A. Van Hove (private communication) , Quinn, Bittencourt, Brown, Woodruff, Noakes, Bailey (bib33) 2002; 14 van der Vegt, Huisman, Howes, Vlieg (bib3) 1995; 330 Clementi, Raimondi, Reinhardt (bib14) 1963; 38 Soares, Bittencourt, Lopes, de Carvalho, Woodruff (bib32) 2004; 550 Quinn, Brown, Woodruff, Bailey, Noakes (bib8) 2002; 511 Zachariasen (bib16) 1973; 35 V.B. Nascimento, Dr. Thesis, Universidade Federal de Minas Gerais, Brazil (in Portuguese) Press, Flannery, Teukolsky, Vetterling (bib27) 1989 van der Vegt, van Pinxteren, Lohmeier, Vlieg, Thornton (bib1) 1992; 68 Noakes, Hutt, McConville, Woodruff (bib5) 1997; 372 van der Vegt (10.1016/j.susc.2004.09.005_bib1) 1992; 68 Zachariasen (10.1016/j.susc.2004.09.005_bib16) 1973; 35 Kittel (10.1016/j.susc.2004.09.005_bib22) 1986 Quinn (10.1016/j.susc.2004.09.005_bib33) 2002; 14 Quinn (10.1016/j.susc.2004.09.005_bib8) 2002; 511 Press (10.1016/j.susc.2004.09.005_bib27) 1989 Campbell (10.1016/j.susc.2004.09.005_bib15) 1986; 167 10.1016/j.susc.2004.09.005_bib20 Nascimento (10.1016/j.susc.2004.09.005_bib28) 2003; 68 Woodruff (10.1016/j.susc.2004.09.005_bib31) 2003; 219 Jiang (10.1016/j.susc.2004.09.005_bib4) 1998; 10 10.1016/j.susc.2004.09.005_bib23 Vrijmoeth (10.1016/j.susc.2004.09.005_bib2) 1994; 72 10.1016/j.susc.2004.09.005_bib9 10.1016/j.susc.2004.09.005_bib19 Clementi (10.1016/j.susc.2004.09.005_bib14) 1963; 38 van der Vegt (10.1016/j.susc.2004.09.005_bib3) 1995; 330 Pendry (10.1016/j.susc.2004.09.005_bib26) 1980; 13 Ghosh (10.1016/j.susc.2004.09.005_bib21) 2002; 3 Soares (10.1016/j.susc.2004.09.005_bib32) 2004; 550 10.1016/j.susc.2004.09.005_bib10 10.1016/j.susc.2004.09.005_bib11 Slater (10.1016/j.susc.2004.09.005_bib17) 1964; 39 Brown (10.1016/j.susc.2004.09.005_bib30) 2000; 61 Noakes (10.1016/j.susc.2004.09.005_bib5) 1997; 372 10.1016/j.susc.2004.09.005_bib12 10.1016/j.susc.2004.09.005_bib13 Van Hove (10.1016/j.susc.2004.09.005_bib25) 1986 Woodruff (10.1016/j.susc.2004.09.005_bib29) 2000; 12 Soares (10.1016/j.susc.2004.09.005_bib6) 2000; 61 de Vries (10.1016/j.susc.2004.09.005_bib7) 1998; 414 Loucks (10.1016/j.susc.2004.09.005_bib24) 1976 Slater (10.1016/j.susc.2004.09.005_bib18) 1965 |
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Snippet | This work concerns the deposition of Sb on the (1
1
0) clean surface of silver. Two structured phases have been observed: an Ag(1
1
0)(4
×
1)–Sb, with a Sb... Sb plays the role of a surfactant in the homo-epitaxy growth of Ag on Ag(111), changing the growth mode from islanding to layer-on-layer. This work concerns... |
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SubjectTerms | Antimony Condensed matter: electronic structure, electrical, magnetic, and optical properties Condensed matter: structure, mechanical and thermal properties Cross-disciplinary physics: materials science; rheology Exact sciences and technology Low energy electron diffraction (LEED) Physics Silver Surface structure, morphology, roughness, and topography |
Title | Structural study of the Ag(1 1 0) c(2 × 2)–Sb phase by low energy electron diffraction |
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