Anthropogenic influences on riverine fluxes of dissolved inorganic carbon to the oceans
Bicarbonate (HCO3−), the predominant form of dissolved inorganic carbon in natural waters, originates mostly from watershed mineral weathering. On time scales of decades to centuries, riverine fluxes of HCO3− to the oceans and subsequent reactions affect atmospheric CO2, global climate and ocean pH....
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| Published in | Limnology and oceanography letters Vol. 3; no. 3; pp. 143 - 155 |
|---|---|
| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Hoboken
John Wiley & Sons, Inc
01.06.2018
Wiley |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Bicarbonate (HCO3−), the predominant form of dissolved inorganic carbon in natural waters, originates mostly from watershed mineral weathering. On time scales of decades to centuries, riverine fluxes of HCO3− to the oceans and subsequent reactions affect atmospheric CO2, global climate and ocean pH. This review summarizes controls on the production of HCO3− from chemical weathering and its transport into river systems. The availability of minerals and weathering agents (carbonic, sulfuric, and nitric acids) in the weathering zone interact to control HCO3− production, and water throughput controls HCO3− transport into rivers. Human influences on HCO3− fluxes include climate warming, acid precipitation, mining, concrete use, and agricultural fertilization and liming. We currently cannot evaluate the net result of human influences on a global scale but HCO3− fluxes are clearly increasing in some major rivers as shown here for much of the United States. This increase could be partly a return to pre‐industrial HCO3− fluxes as anthropogenic acidification has been mitigated in the United States, but elsewhere around the world anthropogenic acidification could be leading to decreased concentrations and fluxes. |
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| AbstractList | Bicarbonate (HCO3−), the predominant form of dissolved inorganic carbon in natural waters, originates mostly from watershed mineral weathering. On time scales of decades to centuries, riverine fluxes of HCO3− to the oceans and subsequent reactions affect atmospheric CO2, global climate and ocean pH. This review summarizes controls on the production of HCO3− from chemical weathering and its transport into river systems. The availability of minerals and weathering agents (carbonic, sulfuric, and nitric acids) in the weathering zone interact to control HCO3− production, and water throughput controls HCO3− transport into rivers. Human influences on HCO3− fluxes include climate warming, acid precipitation, mining, concrete use, and agricultural fertilization and liming. We currently cannot evaluate the net result of human influences on a global scale but HCO3− fluxes are clearly increasing in some major rivers as shown here for much of the United States. This increase could be partly a return to pre‐industrial HCO3− fluxes as anthropogenic acidification has been mitigated in the United States, but elsewhere around the world anthropogenic acidification could be leading to decreased concentrations and fluxes. Abstract Bicarbonate (HCO3−), the predominant form of dissolved inorganic carbon in natural waters, originates mostly from watershed mineral weathering. On time scales of decades to centuries, riverine fluxes of HCO3− to the oceans and subsequent reactions affect atmospheric CO2, global climate and ocean pH. This review summarizes controls on the production of HCO3− from chemical weathering and its transport into river systems. The availability of minerals and weathering agents (carbonic, sulfuric, and nitric acids) in the weathering zone interact to control HCO3− production, and water throughput controls HCO3− transport into rivers. Human influences on HCO3− fluxes include climate warming, acid precipitation, mining, concrete use, and agricultural fertilization and liming. We currently cannot evaluate the net result of human influences on a global scale but HCO3− fluxes are clearly increasing in some major rivers as shown here for much of the United States. This increase could be partly a return to pre‐industrial HCO3− fluxes as anthropogenic acidification has been mitigated in the United States, but elsewhere around the world anthropogenic acidification could be leading to decreased concentrations and fluxes. Bicarbonate ( ), the predominant form of dissolved inorganic carbon in natural waters, originates mostly from watershed mineral weathering. On time scales of decades to centuries, riverine fluxes of to the oceans and subsequent reactions affect atmospheric CO 2 , global climate and ocean pH. This review summarizes controls on the production of from chemical weathering and its transport into river systems. The availability of minerals and weathering agents (carbonic, sulfuric, and nitric acids) in the weathering zone interact to control production, and water throughput controls transport into rivers. Human influences on fluxes include climate warming, acid precipitation, mining, concrete use, and agricultural fertilization and liming. We currently cannot evaluate the net result of human influences on a global scale but fluxes are clearly increasing in some major rivers as shown here for much of the United States. This increase could be partly a return to pre‐industrial fluxes as anthropogenic acidification has been mitigated in the United States, but elsewhere around the world anthropogenic acidification could be leading to decreased concentrations and fluxes. |
| Author | Raymond, Peter A. Hamilton, Stephen K. |
| Author_xml | – sequence: 1 givenname: Peter A. orcidid: 0000-0002-8564-7860 surname: Raymond fullname: Raymond, Peter A. email: peter.raymond@yale.edu organization: Yale School of Forestry and Environmental Studies, Yale University – sequence: 2 givenname: Stephen K. orcidid: 0000-0002-4702-9017 surname: Hamilton fullname: Hamilton, Stephen K. organization: Michigan State University, Hickory Corners |
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| Copyright | 2018 The Author. Limnology and Oceanography Letters published by Wiley Periodicals, Inc. on behalf of Association for the Sciences of Limnology and Oceanography 2018. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. |
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| Snippet | Bicarbonate (HCO3−), the predominant form of dissolved inorganic carbon in natural waters, originates mostly from watershed mineral weathering. On time scales... Bicarbonate ( ), the predominant form of dissolved inorganic carbon in natural waters, originates mostly from watershed mineral weathering. On time scales of... Abstract Bicarbonate (HCO3−), the predominant form of dissolved inorganic carbon in natural waters, originates mostly from watershed mineral weathering. On... |
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| SubjectTerms | Acidification Acids Alkalinity Anthropogenic factors Aquatic ecosystems Biogeochemistry Calcification Carbon cycle Carbon dioxide Chemistry Climate change Dissolved inorganic carbon Global warming Hydrologic cycle Liming Minerals Mining Natural waters Oceans Precipitation River systems Rivers Seawater Sediments Water treatment Watersheds Weathering Weathering zone |
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| Title | Anthropogenic influences on riverine fluxes of dissolved inorganic carbon to the oceans |
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