Enhanced surface decontamination of radioactive Cs by self-generated, strippable hydrogels based on reversible cross-linking
•A self-generated, strippable hydrogel containing adsorbents was developed for surface decontamination.•The hydrogel is composed of polyvinyl alcohol and phenylboronic acid grafted alignate.•The strippable hydrogel effectively removed 137Cs from the various surfaces including a porous cement surface...
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Published in | Journal of hazardous materials Vol. 362; pp. 72 - 81 |
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Main Authors | , , |
Format | Journal Article |
Language | English |
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Elsevier B.V
15.01.2019
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Abstract | •A self-generated, strippable hydrogel containing adsorbents was developed for surface decontamination.•The hydrogel is composed of polyvinyl alcohol and phenylboronic acid grafted alignate.•The strippable hydrogel effectively removed 137Cs from the various surfaces including a porous cement surface.•A new eco-friendly volume-reduction method for radioactive waste was suggested.
A self-generated, strippable hydrogel containing adsorbents was developed to remove the radioactive cesium from surfaces by adsorption for wide-area surface decontamination. Two aqueous polymeric solutions of polyvinyl alcohol (PVA) and phenylboronic-acid-grafted alginate (PBA-Alg) were easily applied to surfaces and subsequently self-generated a hydrogel based on the PBA-diol ester bond. Compared to the strippable coating and chemical gels, the PBA-diol ester bond-based hydrogel was easily peeled off the surfaces without a drying step due to its high elasticity, which is more practical and time saving. The resulting hydrogel displayed high 137Cs removal efficiencies of 91.61% for painted cement, 97.505% for aluminum, 94.05% for stainless steel, and 53.5% for cement, which was 2.3 times higher than that of Decongel due to the presence of the adsorbent in the hydrogel having an excellent Cs distribution coefficient (3.34 × 104 mL/g). Moreover, the volume of radioactive waste generated after the surface decontamination could be reduced by a simple magnetic separation of the adsorbent from the used hydrogel, which can reduce the waste disposal cost. Therefore, our hydrogel system has great potential as a new, cost-effective surface decontaminant in various nuclear industry fields including wide-area environmental remediation after a nuclear accident or terrorist attack. |
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AbstractList | •A self-generated, strippable hydrogel containing adsorbents was developed for surface decontamination.•The hydrogel is composed of polyvinyl alcohol and phenylboronic acid grafted alignate.•The strippable hydrogel effectively removed 137Cs from the various surfaces including a porous cement surface.•A new eco-friendly volume-reduction method for radioactive waste was suggested.
A self-generated, strippable hydrogel containing adsorbents was developed to remove the radioactive cesium from surfaces by adsorption for wide-area surface decontamination. Two aqueous polymeric solutions of polyvinyl alcohol (PVA) and phenylboronic-acid-grafted alginate (PBA-Alg) were easily applied to surfaces and subsequently self-generated a hydrogel based on the PBA-diol ester bond. Compared to the strippable coating and chemical gels, the PBA-diol ester bond-based hydrogel was easily peeled off the surfaces without a drying step due to its high elasticity, which is more practical and time saving. The resulting hydrogel displayed high 137Cs removal efficiencies of 91.61% for painted cement, 97.505% for aluminum, 94.05% for stainless steel, and 53.5% for cement, which was 2.3 times higher than that of Decongel due to the presence of the adsorbent in the hydrogel having an excellent Cs distribution coefficient (3.34 × 104 mL/g). Moreover, the volume of radioactive waste generated after the surface decontamination could be reduced by a simple magnetic separation of the adsorbent from the used hydrogel, which can reduce the waste disposal cost. Therefore, our hydrogel system has great potential as a new, cost-effective surface decontaminant in various nuclear industry fields including wide-area environmental remediation after a nuclear accident or terrorist attack. A self-generated, strippable hydrogel containing adsorbents was developed to remove the radioactive cesium from surfaces by adsorption for wide-area surface decontamination. Two aqueous polymeric solutions of polyvinyl alcohol (PVA) and phenylboronic-acid-grafted alginate (PBA-Alg) were easily applied to surfaces and subsequently self-generated a hydrogel based on the PBA-diol ester bond. Compared to the strippable coating and chemical gels, the PBA-diol ester bond-based hydrogel was easily peeled off the surfaces without a drying step due to its high elasticity, which is more practical and time saving. The resulting hydrogel displayed high Cs removal efficiencies of 91.61% for painted cement, 97.505% for aluminum, 94.05% for stainless steel, and 53.5% for cement, which was 2.3 times higher than that of Decongel due to the presence of the adsorbent in the hydrogel having an excellent Cs distribution coefficient (3.34 × 10 mL/g). Moreover, the volume of radioactive waste generated after the surface decontamination could be reduced by a simple magnetic separation of the adsorbent from the used hydrogel, which can reduce the waste disposal cost. Therefore, our hydrogel system has great potential as a new, cost-effective surface decontaminant in various nuclear industry fields including wide-area environmental remediation after a nuclear accident or terrorist attack. |
Author | Lee, Kune-Woo Park, Chan Woo Yang, Hee-Man |
Author_xml | – sequence: 1 givenname: Hee-Man orcidid: 0000-0001-5554-9947 surname: Yang fullname: Yang, Hee-Man email: hmyang@kaeri.re.kr – sequence: 2 givenname: Chan Woo surname: Park fullname: Park, Chan Woo – sequence: 3 givenname: Kune-Woo surname: Lee fullname: Lee, Kune-Woo |
BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30236944$$D View this record in MEDLINE/PubMed |
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Keywords | Strippable hydrogel Phenylboronic acid-diol ester bond Magnetic separation Radioactive cesium Surface decontamination |
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Snippet | •A self-generated, strippable hydrogel containing adsorbents was developed for surface decontamination.•The hydrogel is composed of polyvinyl alcohol and... A self-generated, strippable hydrogel containing adsorbents was developed to remove the radioactive cesium from surfaces by adsorption for wide-area surface... |
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SubjectTerms | Magnetic separation Phenylboronic acid-diol ester bond Radioactive cesium Strippable hydrogel Surface decontamination |
Title | Enhanced surface decontamination of radioactive Cs by self-generated, strippable hydrogels based on reversible cross-linking |
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