Rare earth modified Ni-Si catalysts for hydrogen production from methane decomposition
Different rare earth （RE=La, Ce, Pr, Nd, Sm, Y） and Cu modified nickel catalysts for hydrogen production from meth-ane decomposition were synthesized by a sol-gel process and method. The catalysts were characterized or analyzed through Brumauer-Emmett-Teller （BET）, X-ray diffraction （XRD）, scanning...
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| Published in | Journal of rare earths Vol. 32; no. 8; pp. 709 - 714 |
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| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.08.2014
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1002-0721 2509-4963 |
| DOI | 10.1016/S1002-0721(14)60130-7 |
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| Abstract | Different rare earth （RE=La, Ce, Pr, Nd, Sm, Y） and Cu modified nickel catalysts for hydrogen production from meth-ane decomposition were synthesized by a sol-gel process and method. The catalysts were characterized or analyzed through Brumauer-Emmett-Teller （BET）, X-ray diffraction （XRD）, scanning electron microscopy （SEM）, transmission electron microscopy （TEM） techniques. And the hydrogen production performance was also evaluated by a fixed-bed and micro-reaction technique with CH4→C＋H2 as a probe reaction. The results showed that rare earth modification had played a great role for nickel catalysts, for example, smaller nickel particles, good thermal stability, high activity, etc. La was the best additive among rare earth modification. The SEM of rare earth modified catalysts showed ordered flower-like structure and rare earth modification made the nickel particles move to the surface of catalysts. In addition, the SEM of nano-carbons was also changed by rare earth modification with long, narrow nano-carbon fibers or tubes obtained. Solid carbon formation was prevented by rare earth modification. |
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| AbstractList | Different rare earth (RE=La, Ce, Pr, Nd, Sm, Y) and Cu modified nickel catalysts for hydrogen production from methane decomposition were synthesized by a sol-gel process and method. The catalysts were characterized or analyzed through Brumauer-Emmett-Teller (BET), X-ray diffraction (XRD), scanning electron microscopy (SEM), transmission electron microscopy (TEM) techniques. And the hydrogen production performance was also evaluated by a fixed-bed and micro-reaction technique with CH sub(4) arrow right C+H sub(2) as a probe reaction. The results showed that rare earth modification had played a great role for nickel catalysts, for example, smaller nickel particles, good thermal stability, high activity, etc. La was the best additive among rare earth modification. The SEM of rare earth modified catalysts showed ordered flower-like structure and rare earth modification made the nickel particles move to the surface of catalysts. In addition, the SEM of nano-carbons was also changed by rare earth modification with long, narrow nano-carbon fibers or tubes obtained. Solid carbon formation was prevented by rare earth modification. Different rare earth (RE=La, Ce, Pr, Nd, Sm, Y) and Cu modified nickel catalysts for hydrogen production from methane decomposition were synthesized by a sol-gel process and method. The catalysts were characterized or analyzed through Brumauer-Emmett-Teller (BET), X-ray diffraction (XRD), scanning electron microscopy (SEM), transmission electron microscopy (TEM) techniques. And the hydrogen production performance was also evaluated by a fixed-bed and micro-reaction technique with CH4→C+H2 as a probe reaction. The results showed that rare earth modification had played a great role for nickel catalysts, for example, smaller nickel particles, good thermal stability, high activity, etc. La was the best additive among rare earth modification. The SEM of rare earth modified catalysts showed ordered flower-like structure and rare earth modification made the nickel particles move to the surface of catalysts. In addition, the SEM of nano-carbons was also changed by rare earth modification with long, narrow nano-carbon fibers or tubes obtained. Solid carbon formation was prevented by rare earth modification. SEM of rare earth and Cu modified catalysts Different rare earth （RE=La, Ce, Pr, Nd, Sm, Y） and Cu modified nickel catalysts for hydrogen production from meth-ane decomposition were synthesized by a sol-gel process and method. The catalysts were characterized or analyzed through Brumauer-Emmett-Teller （BET）, X-ray diffraction （XRD）, scanning electron microscopy （SEM）, transmission electron microscopy （TEM） techniques. And the hydrogen production performance was also evaluated by a fixed-bed and micro-reaction technique with CH4→C＋H2 as a probe reaction. The results showed that rare earth modification had played a great role for nickel catalysts, for example, smaller nickel particles, good thermal stability, high activity, etc. La was the best additive among rare earth modification. The SEM of rare earth modified catalysts showed ordered flower-like structure and rare earth modification made the nickel particles move to the surface of catalysts. In addition, the SEM of nano-carbons was also changed by rare earth modification with long, narrow nano-carbon fibers or tubes obtained. Solid carbon formation was prevented by rare earth modification. |
| Author | 于瀛 崔梅生 李明来 赵娜 龙志奇 施用晞 |
| AuthorAffiliation | National Engineering Research Center for Rare Earth Materials, General Research Institute for Nonferrous Metals, and Grirem Advanced Materials Co., Ltd., Beijing 100088, China Science College, Beijing University of Chemical Technology, Beijing 100029, China |
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| Cites_doi | 10.1016/j.cattod.2006.05.075 10.1163/156856706777346525 10.1016/j.molcata.2006.10.044 10.1016/j.cattod.2006.05.085 10.1016/S1381-1169(01)00358-2 10.1016/j.jpowsour.2007.01.058 10.1016/j.apcata.2004.04.016 10.1016/j.ijhydene.2004.03.033 10.1016/S1003-9953(07)60002-4 |
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| Keywords | Ni-Si catalyst rare earth modification hydrogen production methane decomposition |
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| Notes | 11-2788/TF Different rare earth （RE=La, Ce, Pr, Nd, Sm, Y） and Cu modified nickel catalysts for hydrogen production from meth-ane decomposition were synthesized by a sol-gel process and method. The catalysts were characterized or analyzed through Brumauer-Emmett-Teller （BET）, X-ray diffraction （XRD）, scanning electron microscopy （SEM）, transmission electron microscopy （TEM） techniques. And the hydrogen production performance was also evaluated by a fixed-bed and micro-reaction technique with CH4→C＋H2 as a probe reaction. The results showed that rare earth modification had played a great role for nickel catalysts, for example, smaller nickel particles, good thermal stability, high activity, etc. La was the best additive among rare earth modification. The SEM of rare earth modified catalysts showed ordered flower-like structure and rare earth modification made the nickel particles move to the surface of catalysts. In addition, the SEM of nano-carbons was also changed by rare earth modification with long, narrow nano-carbon fibers or tubes obtained. Solid carbon formation was prevented by rare earth modification. YU Ying , CUI Meisheng, LI Minglai , ZHAO Na , LONG Zhiqi , SHI Yongxi（1. National Engineering Research Center for Rare Earth Materials, General Research Institute for Nonferrous Metals, and Grirem Advanced Materials Co., Ltd., Beijing 100088, China; 2. Science College, Beijing University of Chemical Technology, Beijing 100029, China） rare earth modification; Ni-Si catalyst; hydrogen production; methane decomposition ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
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| SubjectTerms | Catalysis Catalysts Hydrogen production Methane methane decomposition Nanostructure Ni-Si catalyst Nickel Rare earth metals rare earth modification Scanning electron microscopy SEM分析 产氢 分解 扫描电子显微镜 甲烷 稀土改性 透射电子显微镜 镍催化剂 |
| Title | Rare earth modified Ni-Si catalysts for hydrogen production from methane decomposition |
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