Irradiation growth of zirconium single crystals

Irradiation growth of zirconium single crystals has been studied during neutron irradiation at 353 K and 553 K at fluences up to 2× 10 25 n/m 2. The results may be summarized as follows: (a) there was an expansion parallel to the a-axis and a c-axis contraction; (b) the growth strains were small (~1...

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Published inJournal of nuclear materials Vol. 101; no. 1; pp. 28 - 37
Main Authors Carpenter, G.J.C., Murgatroyd, R.A., Rogerson, A., Watters, J.F.
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.10.1981
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Abstract Irradiation growth of zirconium single crystals has been studied during neutron irradiation at 353 K and 553 K at fluences up to 2× 10 25 n/m 2. The results may be summarized as follows: (a) there was an expansion parallel to the a-axis and a c-axis contraction; (b) the growth strains were small (~10 −4), (c) growth saturated at fluences less than ~5× 10 24 n/m 2, (d) the growth behaviour was only weakly dependent on temperature for the range studied, (e) there was a calculated volume increase of the same order as the growth strain, and (f) single crystals prepared from stock of iodide and zone-refined purity showed similar growth behaviour at 553 K. The a-axis expansion is attributed to the annihilation of an excess of interstitials at < a>-type dislocations and interstitial loops. The c-axis contraction may be caused by: (1) elastic relaxation around vacancies or small vacancy clusters, (2) non-linear elastic effects at the dislocation cores of small 〈 a〉-type loops, or (3) sub-microscopic vacancy loops with 〈 c〉-component Burgers vectors. Comparison with data from polycrystalline zirconium confirms that grain boundaries can play an important role in the irradiation growth of zirconium.
AbstractList Irradiation growth of zirconium single crystals has been studied during neutron irradiation at 353 K and 553 K at fluences up to 2× 10 25 n/m 2. The results may be summarized as follows: (a) there was an expansion parallel to the a-axis and a c-axis contraction; (b) the growth strains were small (~10 −4), (c) growth saturated at fluences less than ~5× 10 24 n/m 2, (d) the growth behaviour was only weakly dependent on temperature for the range studied, (e) there was a calculated volume increase of the same order as the growth strain, and (f) single crystals prepared from stock of iodide and zone-refined purity showed similar growth behaviour at 553 K. The a-axis expansion is attributed to the annihilation of an excess of interstitials at < a>-type dislocations and interstitial loops. The c-axis contraction may be caused by: (1) elastic relaxation around vacancies or small vacancy clusters, (2) non-linear elastic effects at the dislocation cores of small 〈 a〉-type loops, or (3) sub-microscopic vacancy loops with 〈 c〉-component Burgers vectors. Comparison with data from polycrystalline zirconium confirms that grain boundaries can play an important role in the irradiation growth of zirconium.
Irradiation growth of Zr single crystals has been studied during neutron irradiation at 353 and 553 deg K at fluences up to 2 x 10 exp 25 n/m exp 2 . The results may be summarized as follows: there was an expansion parallel to the a -axis and a c -axis contraction, the growth strains were small ( approx 10 exp --4 ); growth saturated at fluences < approx 5 x 10 exp 24 n/m exp 2 ; the growth behavior was only weakly dependent on temp. for the range studied; there was a calculated volume increase of the same order as the growth strain; and single crystals prepared from stock of iodide and zone-refined purity showed similar growth behavior at 553 deg K. The a -axis expansion is attributed to the annihilation of an excess of interstitials at < a > -type dislocations and interstitial loops. The c -axis contraction may be caused by: elastic relaxation around vacancies or small vacancy clusters; nonlinear elastic effects at the dislocation cores of small < a > -type loops; or submicroscopic vacancy loops with < c > -component Burgers vectors. 38 ref.--AA
Author Watters, J.F.
Murgatroyd, R.A.
Carpenter, G.J.C.
Rogerson, A.
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Snippet Irradiation growth of zirconium single crystals has been studied during neutron irradiation at 353 K and 553 K at fluences up to 2× 10 25 n/m 2. The results...
Irradiation growth of Zr single crystals has been studied during neutron irradiation at 353 and 553 deg K at fluences up to 2 x 10 exp 25 n/m exp 2 . The...
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Title Irradiation growth of zirconium single crystals
URI https://dx.doi.org/10.1016/0022-3115(81)90441-4
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