A supramolecular strategy based on molecular dipole moments for high-quality covalent organic frameworks
A supramolecular strategy based on strong molecular dipole moments is presented to gain access to covalent organic framework structures with high crystallinity and porosity. Antiparallel alignment of the molecules within the pore walls is proposed to lead to reinforced columnar stacking, thus afford...
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| Published in | Chemical communications (Cambridge, England) Vol. 52; no. 51; pp. 7986 - 7989 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
CAMBRIDGE
Royal Soc Chemistry
01.01.2016
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| Subjects | |
| Online Access | Get full text |
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| Abstract | A supramolecular strategy based on strong molecular dipole moments is presented to gain access to covalent organic framework structures with high crystallinity and porosity. Antiparallel alignment of the molecules within the pore walls is proposed to lead to reinforced columnar stacking, thus affording a high-quality material. As a proof of principle, a novel pyrene dione building block was prepared and reacted with hexahydroxytriphenylene to form a boronic ester-linked covalent organic framework. We anticipate the strategy presented herein to be valuable for producing highly defined COF structures.
Attractive intermolecular interactions of building blocks with strong dipole moments result in a COF with high crystallinity and large surface area. |
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| AbstractList | A supramolecular strategy based on strongmolecular dipole moments is presented to gain access to covalent organic framework structures with high crystallinity and porosity. Antiparallel alignment of the molecules within the pore walls is proposed to lead to reinforced columnar stacking, thus affording a high-quality material. As a proof of principle, a novel pyrene dione building block was prepared and reacted with hexahydroxytriphenylene to form a boronic ester-linked covalent organic framework. We anticipate the strategy presented herein to be valuable for producing highly defined COF structures. A supramolecular strategy based on strong molecular dipole moments is presented to gain access to covalent organic framework structures with high crystallinity and porosity. Antiparallel alignment of the molecules within the pore walls is proposed to lead to reinforced columnar stacking, thus affording a high-quality material. As a proof of principle, a novel pyrene dione building block was prepared and reacted with hexahydroxytriphenylene to form a boronic ester-linked covalent organic framework. We anticipate the strategy presented herein to be valuable for producing highly defined COF structures. A supramolecular strategy based on strong molecular dipole moments is presented to gain access to covalent organic framework structures with high crystallinity and porosity. Antiparallel alignment of the molecules within the pore walls is proposed to lead to reinforced columnar stacking, thus affording a high-quality material. As a proof of principle, a novel pyrene dione building block was prepared and reacted with hexahydroxytriphenylene to form a boronic ester-linked covalent organic framework. We anticipate the strategy presented herein to be valuable for producing highly defined COF structures. Attractive intermolecular interactions of building blocks with strong dipole moments result in a COF with high crystallinity and large surface area. |
| Author | Guldris, Noelia Mafra, Luís Rotter, Julian M Salonen, Laura M Stroppa, Daniel G Medina, Dana D Rodríguez-Abreu, Carlos Carbó-Argibay, Enrique Goesten, Maarten G |
| AuthorAffiliation | Department of Chemistry University of Aveiro International Iberian Nanotechnology Laboratory (INL) CICECO - Aveiro Institute of Materials Ludwig-Maximilians-University Munich (LMU) Department of Chemistry and Center for NanoScience (CeNS) Inorganic Materials Chemistry Eindhoven University of Technology |
| AuthorAffiliation_xml | – sequence: 0 name: Department of Chemistry – sequence: 0 name: University of Aveiro – sequence: 0 name: International Iberian Nanotechnology Laboratory (INL) – sequence: 0 name: Ludwig-Maximilians-University Munich (LMU) – sequence: 0 name: Inorganic Materials Chemistry – sequence: 0 name: Department of Chemistry and Center for NanoScience (CeNS) – sequence: 0 name: CICECO - Aveiro Institute of Materials – sequence: 0 name: Eindhoven University of Technology |
| Author_xml | – sequence: 1 givenname: Laura M surname: Salonen fullname: Salonen, Laura M – sequence: 2 givenname: Dana D surname: Medina fullname: Medina, Dana D – sequence: 3 givenname: Enrique surname: Carbó-Argibay fullname: Carbó-Argibay, Enrique – sequence: 4 givenname: Maarten G surname: Goesten fullname: Goesten, Maarten G – sequence: 5 givenname: Luís surname: Mafra fullname: Mafra, Luís – sequence: 6 givenname: Noelia surname: Guldris fullname: Guldris, Noelia – sequence: 7 givenname: Julian M surname: Rotter fullname: Rotter, Julian M – sequence: 8 givenname: Daniel G surname: Stroppa fullname: Stroppa, Daniel G – sequence: 9 givenname: Carlos surname: Rodríguez-Abreu fullname: Rodríguez-Abreu, Carlos |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/27257634$$D View this record in MEDLINE/PubMed |
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| Keywords | STORAGE HYDROGEN STACKING PYRENE STABILITY CONSTRUCTION AROMATIC RINGS CRYSTALLINE |
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article-title: Efficient Stacking on Protein Amide Fragments publication-title: CHEMMEDCHEM doi: 10.1002/cmdc.201200512 |
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| Snippet | A supramolecular strategy based on strong molecular dipole moments is presented to gain access to covalent organic framework structures with high crystallinity... A supramolecular strategy based on strongmolecular dipole moments is presented to gain access to covalent organic framework structures with high crystallinity... |
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| SubjectTerms | chemical compounds chemical reactions Chemistry Chemistry, Multidisciplinary Covalence crystal structure Crystallinity Dipole moment Gain Physical Sciences Porosity Science & Technology Stacking Strategy Walls |
| Title | A supramolecular strategy based on molecular dipole moments for high-quality covalent organic frameworks |
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