Capturing nitrosamines in aqueous solution by composited super-hydrophobic silicic xerogel

Super-hydrophobic silicic xerogel (SG) was prepared from methyltrimethoxysilane (MTMS) and dimethyldimethoxysilane (DMDMS), and the optimized MTMS to DMDMS molar ratio was determined to be 3/2. To fabricate new effective nitrosamines sorbent in tobacco extract solution, SG was modified by epitaxial...

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Published inMicroporous and mesoporous materials Vol. 227; pp. 161 - 168
Main Authors Li, Shuo Hao, Lin, Wei Gang, Huang, Bi Cheng, Wang, Lei-jun, Gu, Wen-bo, Wang, Wei-miao, Yang, Zheng Yu, Wang, Ying, Zhu, Jian Hua
Format Journal Article
LanguageEnglish
Published Elsevier Inc 01.06.2016
Subjects
Environment protection
Epitaxial growth of mesoporous silica
Liquid adsorption
Nitrosamines
Super-hydrophobic silicic xerogel
Nitrosamines
Liquid adsorption
Epitaxial growth of mesoporous silica
Environment protection
Super-hydrophobic silicic xerogel
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Abstract Super-hydrophobic silicic xerogel (SG) was prepared from methyltrimethoxysilane (MTMS) and dimethyldimethoxysilane (DMDMS), and the optimized MTMS to DMDMS molar ratio was determined to be 3/2. To fabricate new effective nitrosamines sorbent in tobacco extract solution, SG was modified by epitaxial growth of mesoporous silica to form the coated composite named as MSGx with a large surface area (152–208 m2 g-1) and pore volume (0.133–0.162 mLg−1), and the new sorbent could capture 54–59% of nitrosamines in tobacco solution, superior to zeolite and mesoporous silica. [Display omitted] •New powerful TSNA trapper in tobacco solution.•It can efficiently trap 60% of nitrosamines in tobacco solution.•Fabrication core–shell composite through epitaxial growth.•Tuning surface state of sorbent to accelerate liquid adsorption.•Control the carcinogen pollution at source.
AbstractList Super-hydrophobic silicic xerogel (SG) was prepared from methyltrimethoxysilane (MTMS) and dimethyldimethoxysilane (DMDMS), and the optimized MTMS to DMDMS molar ratio was determined to be 3/2. To fabricate new effective nitrosamines sorbent in tobacco extract solution, SG was modified by epitaxial growth of mesoporous silica to form the coated composite named as MSGx with a large surface area (152–208 m2 g-1) and pore volume (0.133–0.162 mLg−1), and the new sorbent could capture 54–59% of nitrosamines in tobacco solution, superior to zeolite and mesoporous silica. [Display omitted] •New powerful TSNA trapper in tobacco solution.•It can efficiently trap 60% of nitrosamines in tobacco solution.•Fabrication core–shell composite through epitaxial growth.•Tuning surface state of sorbent to accelerate liquid adsorption.•Control the carcinogen pollution at source.
Author Li, Shuo Hao
Wang, Wei-miao
Huang, Bi Cheng
Wang, Ying
Gu, Wen-bo
Zhu, Jian Hua
Wang, Lei-jun
Yang, Zheng Yu
Lin, Wei Gang
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  organization: Key Laboratory of Mesoscopic Chemistry of MOE, College of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210023, China
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crossref_primary_10_1016_j_micromeso_2016_09_031
crossref_primary_10_1007_s10924_020_02041_x
crossref_primary_10_1117_1_JPE_10_023508
crossref_primary_10_1016_j_cej_2017_04_064
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Keywords Nitrosamines
Liquid adsorption
Epitaxial growth of mesoporous silica
Environment protection
Super-hydrophobic silicic xerogel
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Snippet Super-hydrophobic silicic xerogel (SG) was prepared from methyltrimethoxysilane (MTMS) and dimethyldimethoxysilane (DMDMS), and the optimized MTMS to DMDMS...
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SubjectTerms Environment protection
Epitaxial growth of mesoporous silica
Liquid adsorption
Nitrosamines
Super-hydrophobic silicic xerogel
Title Capturing nitrosamines in aqueous solution by composited super-hydrophobic silicic xerogel
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