Inorganic, Organic, and Perovskite Halides with Nanotechnology for High–Light Yield X- and γ-ray Scintillators

Trends in scintillators that are used in many applications, such as medical imaging, security, oil-logging, high energy physics and non-destructive inspections are reviewed. First, we address traditional inorganic and organic scintillators with respect of limitation in the scintillation light yields...

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Bibliographic Details
Published inCrystals (Basel) Vol. 9; no. 2; p. 88
Main Authors Maddalena, Francesco, Tjahjana, Liliana, Xie, Aozhen, Arramel, Zeng, Shuwen, Wang, Hong, Coquet, Philippe, Drozdowski, Winicjusz, Dujardin, Christophe, Dang, Cuong, Birowosuto, Muhammad
Format Journal Article
LanguageEnglish
Published Basel MDPI AG 01.02.2019
MDPI
Subjects
Absorption cross sections
Atoms & subatomic particles
Cerium
Chemical Sciences
Collaboration
Conversion
Crystal growth
Energy dissipation
Engineering Sciences
High temperature
inorganic
Lead compounds
Low temperature
Medical imaging
Metal halides
Nanocrystals
Nanotechnology
organic
perovskite
Perovskites
Photoluminescence
Photons
Physics
Quantum dots
R&D
Research & development
Scintillation
Scintillation counters
scintillator
Sensors
Single crystals
Tomography
X ray absorption
X-ray
X-rays
γ-ray
perovskite
X-ray
inorganic
organic
scintillator
γ-ray
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Abstract Trends in scintillators that are used in many applications, such as medical imaging, security, oil-logging, high energy physics and non-destructive inspections are reviewed. First, we address traditional inorganic and organic scintillators with respect of limitation in the scintillation light yields and lifetimes. The combination of high–light yield and fast response can be found in Ce 3 + , Pr 3 + and Nd 3 + lanthanide-doped scintillators while the maximum light yield conversion of 100,000 photons/MeV can be found in Eu 3 + doped SrI 2 . However, the fabrication of those lanthanide-doped scintillators is inefficient and expensive as it requires high-temperature furnaces. A self-grown single crystal using solution processes is already introduced in perovskite photovoltaic technology and it can be the key for low-cost scintillators. A novel class of materials in scintillation includes lead halide perovskites. These materials were explored decades ago due to the large X-ray absorption cross section. However, lately lead halide perovskites have become a focus of interest due to recently reported very high photoluminescence quantum yield and light yield conversion at low temperatures. In principle, 150,000–300,000 photons/MeV light yields can be proportional to the small energy bandgap of these materials, which is below 2 eV. Finally, we discuss the extraction efficiency improvements through the fabrication of the nanostructure in scintillators, which can be implemented in perovskite materials. The recent technology involving quantum dots and nanocrystals may also improve light conversion in perovskite scintillators.
AbstractList Trends in scintillators that are used in many applications, such as medical imaging, security, oil-logging, high energy physics and non-destructive inspections are reviewed. First, we address traditional inorganic and organic scintillators with respect of limitation in the scintillation light yields and lifetimes. The combination of high–light yield and fast response can be found in Ce 3 + , Pr 3 + and Nd 3 + lanthanide-doped scintillators while the maximum light yield conversion of 100,000 photons/MeV can be found in Eu 3 + doped SrI 2 . However, the fabrication of those lanthanide-doped scintillators is inefficient and expensive as it requires high-temperature furnaces. A self-grown single crystal using solution processes is already introduced in perovskite photovoltaic technology and it can be the key for low-cost scintillators. A novel class of materials in scintillation includes lead halide perovskites. These materials were explored decades ago due to the large X-ray absorption cross section. However, lately lead halide perovskites have become a focus of interest due to recently reported very high photoluminescence quantum yield and light yield conversion at low temperatures. In principle, 150,000–300,000 photons/MeV light yields can be proportional to the small energy bandgap of these materials, which is below 2 eV. Finally, we discuss the extraction efficiency improvements through the fabrication of the nanostructure in scintillators, which can be implemented in perovskite materials. The recent technology involving quantum dots and nanocrystals may also improve light conversion in perovskite scintillators.
Trends in scintillators that are used in many applications, such as medical imaging, security, oil-logging, high energy physics and non-destructive inspections are reviewed. First, we address traditional inorganic and organic scintillators with respect of limitation in the scintillation light yields and lifetimes. The combination of high⁻light yield and fast response can be found in Ce 3 + , Pr 3 + and Nd 3 + lanthanide-doped scintillators while the maximum light yield conversion of 100,000 photons/MeV can be found in Eu 3 + doped SrI 2 . However, the fabrication of those lanthanide-doped scintillators is inefficient and expensive as it requires high-temperature furnaces. A self-grown single crystal using solution processes is already introduced in perovskite photovoltaic technology and it can be the key for low-cost scintillators. A novel class of materials in scintillation includes lead halide perovskites. These materials were explored decades ago due to the large X-ray absorption cross section. However, lately lead halide perovskites have become a focus of interest due to recently reported very high photoluminescence quantum yield and light yield conversion at low temperatures. In principle, 150,000⁻300,000 photons/MeV light yields can be proportional to the small energy bandgap of these materials, which is below 2 eV. Finally, we discuss the extraction efficiency improvements through the fabrication of the nanostructure in scintillators, which can be implemented in perovskite materials. The recent technology involving quantum dots and nanocrystals may also improve light conversion in perovskite scintillators.
Trends in scintillators that are used in many applications, such as medical imaging, security, oil-logging, high energy physics and non-destructive inspections are reviewed. First, we address traditional inorganic and organic scintillators with respect of limitation in the scintillation light yields and lifetimes. The combination of high–light yield and fast response can be found in Ce3+, Pr3+and Nd3+lanthanide-doped scintillators while the maximum light yield conversion of 100,000 photons/MeV can be found in Eu3+doped SrI2. However, the fabrication of those lanthanide-doped scintillators is inefficient and expensive as it requires high-temperature furnaces. A self-grown single crystal using solution processes is already introduced in perovskite photovoltaic technology and it can be the key for low-cost scintillators. A novel class of materials in scintillation includes lead halide perovskites. These materials were explored decades ago due to the large X-ray absorption cross section. However, lately lead halide perovskites have become a focus of interest due to recently reported very high photoluminescence quantum yield and light yield conversion at low temperatures. In principle, 150,000–300,000 photons/MeV light yields can be proportional to the small energy bandgap of these materials, which is below 2 eV. Finally, we discuss the extraction efficiency improvements through the fabrication of the nanostructure in scintillators, which can be implemented in perovskite materials. The recent technology involving quantum dots and nanocrystals may also improve light conversion in perovskite scintillators.
Trends in scintillators that are used in many applications, such as medical imaging, security, oil-logging, high energy physics and non-destructive inspections are reviewed. First, we address traditional inorganic and organic scintillators with respect of limitation in the scintillation light yields and lifetimes. The combination of high–light yield and fast response can be found in Ce3+ , Pr3+ and Nd3+ lanthanide-doped scintillators while the maximum light yield conversion of 100,000 photons/MeV can be found in Eu3+ doped SrI2 . However, the fabrication of those lanthanide-doped scintillators is inefficient and expensive as it requires high-temperature furnaces. A self-grown single crystal using solution processes is already introduced in perovskite photovoltaic technology and it can be the key for low-cost scintillators. A novel class of materials in scintillation includes lead halide perovskites. These materials were explored decades ago due to the large X-ray absorption cross section. However, lately lead halide perovskites have become a focus of interest due to recently reported very high photoluminescence quantum yield and light yield conversion at low temperatures. In principle, 150,000–300,000 photons/MeV light yields can be proportional to the small energy bandgap of these materials, which is below 2 eV. Finally, we discuss the extraction efficiency improvements through the fabrication of the nanostructure in scintillators, which can be implemented in perovskite materials. The recent technology involving quantum dots and nanocrystals may also improve light conversion in perovskite scintillators
Author Dujardin, Christophe
Maddalena, Francesco
Tjahjana, Liliana
Dang, Cuong
Arramel
Wang, Hong
Coquet, Philippe
Birowosuto, Muhammad
Xie, Aozhen
Drozdowski, Winicjusz
Zeng, Shuwen
Author_xml – sequence: 1
  givenname: Francesco
  orcidid: 0000-0001-6246-8870
  surname: Maddalena
  fullname: Maddalena, Francesco
– sequence: 2
  givenname: Liliana
  orcidid: 0000-0003-0015-5582
  surname: Tjahjana
  fullname: Tjahjana, Liliana
– sequence: 3
  givenname: Aozhen
  orcidid: 0000-0003-3510-7177
  surname: Xie
  fullname: Xie, Aozhen
– sequence: 4
  orcidid: 0000-0003-4125-6099
  surname: Arramel
  fullname: Arramel
– sequence: 5
  givenname: Shuwen
  orcidid: 0000-0003-2188-7213
  surname: Zeng
  fullname: Zeng, Shuwen
– sequence: 6
  givenname: Hong
  surname: Wang
  fullname: Wang, Hong
– sequence: 7
  givenname: Philippe
  surname: Coquet
  fullname: Coquet, Philippe
– sequence: 8
  givenname: Winicjusz
  orcidid: 0000-0002-6207-4801
  surname: Drozdowski
  fullname: Drozdowski, Winicjusz
– sequence: 9
  givenname: Christophe
  surname: Dujardin
  fullname: Dujardin, Christophe
– sequence: 10
  givenname: Cuong
  orcidid: 0000-0001-6183-4082
  surname: Dang
  fullname: Dang, Cuong
– sequence: 11
  givenname: Muhammad
  orcidid: 0000-0002-9997-6841
  surname: Birowosuto
  fullname: Birowosuto, Muhammad
BackLink https://univ-lyon1.hal.science/hal-02285858$$DView record in HAL
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Snippet Trends in scintillators that are used in many applications, such as medical imaging, security, oil-logging, high energy physics and non-destructive inspections...
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StartPage 88
SubjectTerms Absorption cross sections
Atoms & subatomic particles
Cerium
Chemical Sciences
Collaboration
Conversion
Crystal growth
Energy dissipation
Engineering Sciences
High temperature
inorganic
Lead compounds
Low temperature
Medical imaging
Metal halides
Nanocrystals
Nanotechnology
organic
perovskite
Perovskites
Photoluminescence
Photons
Physics
Quantum dots
R&D
Research & development
Scintillation
Scintillation counters
scintillator
Sensors
Single crystals
Tomography
X ray absorption
X-ray
X-rays
γ-ray
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Title Inorganic, Organic, and Perovskite Halides with Nanotechnology for High–Light Yield X- and γ-ray Scintillators
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Volume 9
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