A review on advanced catalytic co-pyrolysis of biomass and hydrogen-rich feedstock: Insights into synergistic effect, catalyst development and reaction mechanism

[Display omitted] •Catalytic co-pyrolysis of biomass and high-rich feedstock is reviewed.•Synergistic interaction between hydrogen donor feedstock and biomass are presented.•Effective catalysts for biomass deoxygenation and hydrogen transfer are compared.•Co-pyrolysis addresses waste management goal...

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Published inBioresource technology Vol. 310; p. 123457
Main Authors Ahmed, Mohamed H.M., Batalha, Nuno, Mahmudul, Hasan M.D., Perkins, Greg, Konarova, Muxina
Format Journal Article
LanguageEnglish
Published England Elsevier Ltd 01.08.2020
Subjects
Active sites
Biofuels
Biomass
Biomass deoxygenation
carbon
Catalysis
catalysts
Co-pyrolysis
commercialization
cost effectiveness
depolymerization
ethanol
feedstocks
fossil fuels
Hot Temperature
Hydrogen
Hydrogen transfer
lignocellulose
lubricants
methane
methanol
oils
oxygen
porous media
Pyrolysis
pyrolysis oils
reaction mechanisms
research and development
silica
solid wastes
synergism
technology
tires
waste utilization
Zeolite
zeolites
Biomass deoxygenation
Hydrogen transfer
Co-pyrolysis
Zeolite
Active sites
Online AccessGet full text
ISSN0960-8524
1873-2976
1873-2976
DOI10.1016/j.biortech.2020.123457

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Abstract [Display omitted] •Catalytic co-pyrolysis of biomass and high-rich feedstock is reviewed.•Synergistic interaction between hydrogen donor feedstock and biomass are presented.•Effective catalysts for biomass deoxygenation and hydrogen transfer are compared.•Co-pyrolysis addresses waste management goals by utilizing abundant waste feedstock. The depletion of fossil fuel reserves and the growing demand for alternative energy sources are the main drivers of biomass and carbonaceous waste utilization. Particularly, non-edible lignocellulosic biomass is the most attractive renewable feedstock due to its abundance. Pyrolysis of biomass produces highly oxygenated compounds with oxygen content >35 wt%. The cost-effective elimination of oxygen from the pyrolysis oil is the most challenging task impeding the commercialization of biomass to biofuel processes. The effective hydrogen/carbon ratio in biomass pyrolysis oil is low (0.3), requiring external hydrogen supply to produce hydrocarbon-rich oils. Exploiting hydrogen-rich feedstock particularly, solid waste (plastic, tyre and scum) and other low-cost feedstock (lubricant oil, methane, methanol, and ethanol) offer an eco-friendly solution to upgrade the produced bio-oil. Multi-functional catalysts that are capable of cleaving oxygen, promoting hydrogen transfer and depolymerisation must be developed to produce hydrocarbon-rich oil from biomass. This review compares catalytic co-pyrolysis studies based on zeolites, mesoporous silica and metal oxides. Furthermore, a wide range of catalyst modifications and the role of each feedstock were summarised to give a complete picture of the progress made on biomass co-pyrolysis research and development.
AbstractList [Display omitted] •Catalytic co-pyrolysis of biomass and high-rich feedstock is reviewed.•Synergistic interaction between hydrogen donor feedstock and biomass are presented.•Effective catalysts for biomass deoxygenation and hydrogen transfer are compared.•Co-pyrolysis addresses waste management goals by utilizing abundant waste feedstock. The depletion of fossil fuel reserves and the growing demand for alternative energy sources are the main drivers of biomass and carbonaceous waste utilization. Particularly, non-edible lignocellulosic biomass is the most attractive renewable feedstock due to its abundance. Pyrolysis of biomass produces highly oxygenated compounds with oxygen content >35 wt%. The cost-effective elimination of oxygen from the pyrolysis oil is the most challenging task impeding the commercialization of biomass to biofuel processes. The effective hydrogen/carbon ratio in biomass pyrolysis oil is low (0.3), requiring external hydrogen supply to produce hydrocarbon-rich oils. Exploiting hydrogen-rich feedstock particularly, solid waste (plastic, tyre and scum) and other low-cost feedstock (lubricant oil, methane, methanol, and ethanol) offer an eco-friendly solution to upgrade the produced bio-oil. Multi-functional catalysts that are capable of cleaving oxygen, promoting hydrogen transfer and depolymerisation must be developed to produce hydrocarbon-rich oil from biomass. This review compares catalytic co-pyrolysis studies based on zeolites, mesoporous silica and metal oxides. Furthermore, a wide range of catalyst modifications and the role of each feedstock were summarised to give a complete picture of the progress made on biomass co-pyrolysis research and development.
The depletion of fossil fuel reserves and the growing demand for alternative energy sources are the main drivers of biomass and carbonaceous waste utilization. Particularly, non-edible lignocellulosic biomass is the most attractive renewable feedstock due to its abundance. Pyrolysis of biomass produces highly oxygenated compounds with oxygen content >35 wt%. The cost-effective elimination of oxygen from the pyrolysis oil is the most challenging task impeding the commercialization of biomass to biofuel processes. The effective hydrogen/carbon ratio in biomass pyrolysis oil is low (0.3), requiring external hydrogen supply to produce hydrocarbon-rich oils. Exploiting hydrogen-rich feedstock particularly, solid waste (plastic, tyre and scum) and other low-cost feedstock (lubricant oil, methane, methanol, and ethanol) offer an eco-friendly solution to upgrade the produced bio-oil. Multi-functional catalysts that are capable of cleaving oxygen, promoting hydrogen transfer and depolymerisation must be developed to produce hydrocarbon-rich oil from biomass. This review compares catalytic co-pyrolysis studies based on zeolites, mesoporous silica and metal oxides. Furthermore, a wide range of catalyst modifications and the role of each feedstock were summarised to give a complete picture of the progress made on biomass co-pyrolysis research and development.
The depletion of fossil fuel reserves and the growing demand for alternative energy sources are the main drivers of biomass and carbonaceous waste utilization. Particularly, non-edible lignocellulosic biomass is the most attractive renewable feedstock due to its abundance. Pyrolysis of biomass produces highly oxygenated compounds with oxygen content >35 wt%. The cost-effective elimination of oxygen from the pyrolysis oil is the most challenging task impeding the commercialization of biomass to biofuel processes. The effective hydrogen/carbon ratio in biomass pyrolysis oil is low (0.3), requiring external hydrogen supply to produce hydrocarbon-rich oils. Exploiting hydrogen-rich feedstock particularly, solid waste (plastic, tyre and scum) and other low-cost feedstock (lubricant oil, methane, methanol, and ethanol) offer an eco-friendly solution to upgrade the produced bio-oil. Multi-functional catalysts that are capable of cleaving oxygen, promoting hydrogen transfer and depolymerisation must be developed to produce hydrocarbon-rich oil from biomass. This review compares catalytic co-pyrolysis studies based on zeolites, mesoporous silica and metal oxides. Furthermore, a wide range of catalyst modifications and the role of each feedstock were summarised to give a complete picture of the progress made on biomass co-pyrolysis research and development.
The depletion of fossil fuel reserves and the growing demand for alternative energy sources are the main drivers of biomass and carbonaceous waste utilization. Particularly, non-edible lignocellulosic biomass is the most attractive renewable feedstock due to its abundance. Pyrolysis of biomass produces highly oxygenated compounds with oxygen content >35 wt%. The cost-effective elimination of oxygen from the pyrolysis oil is the most challenging task impeding the commercialization of biomass to biofuel processes. The effective hydrogen/carbon ratio in biomass pyrolysis oil is low (0.3), requiring external hydrogen supply to produce hydrocarbon-rich oils. Exploiting hydrogen-rich feedstock particularly, solid waste (plastic, tyre and scum) and other low-cost feedstock (lubricant oil, methane, methanol, and ethanol) offer an eco-friendly solution to upgrade the produced bio-oil. Multi-functional catalysts that are capable of cleaving oxygen, promoting hydrogen transfer and depolymerisation must be developed to produce hydrocarbon-rich oil from biomass. This review compares catalytic co-pyrolysis studies based on zeolites, mesoporous silica and metal oxides. Furthermore, a wide range of catalyst modifications and the role of each feedstock were summarised to give a complete picture of the progress made on biomass co-pyrolysis research and development.The depletion of fossil fuel reserves and the growing demand for alternative energy sources are the main drivers of biomass and carbonaceous waste utilization. Particularly, non-edible lignocellulosic biomass is the most attractive renewable feedstock due to its abundance. Pyrolysis of biomass produces highly oxygenated compounds with oxygen content >35 wt%. The cost-effective elimination of oxygen from the pyrolysis oil is the most challenging task impeding the commercialization of biomass to biofuel processes. The effective hydrogen/carbon ratio in biomass pyrolysis oil is low (0.3), requiring external hydrogen supply to produce hydrocarbon-rich oils. Exploiting hydrogen-rich feedstock particularly, solid waste (plastic, tyre and scum) and other low-cost feedstock (lubricant oil, methane, methanol, and ethanol) offer an eco-friendly solution to upgrade the produced bio-oil. Multi-functional catalysts that are capable of cleaving oxygen, promoting hydrogen transfer and depolymerisation must be developed to produce hydrocarbon-rich oil from biomass. This review compares catalytic co-pyrolysis studies based on zeolites, mesoporous silica and metal oxides. Furthermore, a wide range of catalyst modifications and the role of each feedstock were summarised to give a complete picture of the progress made on biomass co-pyrolysis research and development.
ArticleNumber 123457
Author Konarova, Muxina
Ahmed, Mohamed H.M.
Batalha, Nuno
Perkins, Greg
Mahmudul, Hasan M.D.
Author_xml – sequence: 1
  givenname: Mohamed H.M.
  surname: Ahmed
  fullname: Ahmed, Mohamed H.M.
  organization: Australian Institute for Bioengineering and Nanotechnology, The University of Queensland, Brisbane 4072, Australia
– sequence: 2
  givenname: Nuno
  surname: Batalha
  fullname: Batalha, Nuno
  organization: School of Chemical Engineering, The University of Queensland, Brisbane 4072, Australia
– sequence: 3
  givenname: Hasan M.D.
  surname: Mahmudul
  fullname: Mahmudul, Hasan M.D.
  organization: Australian Institute for Bioengineering and Nanotechnology, The University of Queensland, Brisbane 4072, Australia
– sequence: 4
  givenname: Greg
  surname: Perkins
  fullname: Perkins, Greg
  organization: School of Chemical Engineering, The University of Queensland, Brisbane 4072, Australia
– sequence: 5
  givenname: Muxina
  surname: Konarova
  fullname: Konarova, Muxina
  email: m.konarova@uq.edu.au
  organization: Australian Institute for Bioengineering and Nanotechnology, The University of Queensland, Brisbane 4072, Australia
BackLink https://www.ncbi.nlm.nih.gov/pubmed/32371033$$D View this record in MEDLINE/PubMed
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Snippet [Display omitted] •Catalytic co-pyrolysis of biomass and high-rich feedstock is reviewed.•Synergistic interaction between hydrogen donor feedstock and biomass...
The depletion of fossil fuel reserves and the growing demand for alternative energy sources are the main drivers of biomass and carbonaceous waste utilization....
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SubjectTerms Active sites
Biofuels
Biomass
Biomass deoxygenation
carbon
Catalysis
catalysts
Co-pyrolysis
commercialization
cost effectiveness
depolymerization
ethanol
feedstocks
fossil fuels
Hot Temperature
Hydrogen
Hydrogen transfer
lignocellulose
lubricants
methane
methanol
oils
oxygen
porous media
Pyrolysis
pyrolysis oils
reaction mechanisms
research and development
silica
solid wastes
synergism
technology
tires
waste utilization
Zeolite
zeolites
Title A review on advanced catalytic co-pyrolysis of biomass and hydrogen-rich feedstock: Insights into synergistic effect, catalyst development and reaction mechanism
URI https://dx.doi.org/10.1016/j.biortech.2020.123457
https://www.ncbi.nlm.nih.gov/pubmed/32371033
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https://www.proquest.com/docview/2524252888
Volume 310
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