A novel electrochemically switched ion exchange system for phenol recovery and regeneration of NaOH from sodium phenolate wastewater
•Separation of the phenol and desalination could be achieved simultaneously.•Production of NaOH with this ESIX system could be realized.•The FeHCF coated electrode could work repeatedly in the series operation.•The ESIX system exhibited a very low energy consumption. An electrochemically switched io...
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| Published in | Separation and Purification Technology Vol. 248; p. 117125 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English Japanese |
| Published |
Elsevier B.V
01.10.2020
Elsevier BV |
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| Abstract | •Separation of the phenol and desalination could be achieved simultaneously.•Production of NaOH with this ESIX system could be realized.•The FeHCF coated electrode could work repeatedly in the series operation.•The ESIX system exhibited a very low energy consumption.
An electrochemically switched ion exchange (ESIX) system was proposed as a novel electrochemical method for the treatment of high concentration phenolic sodium salty wastewater, in which a ferric ferricyanide (FeHCF) coated electrode with rigid open framework can control the insertion/extraction of sodium (Na+) ions by switching the redox state of FeHCF. It is found that this ESIX system can not only remove the phenol and desalinate the phenol-containing wastewater simultaneously, but also regenerate the FeHCF coated electrode and produce sodium hydroxide (NaOH). In the series operation, more than 79% of phenol could be removed with energy consumption of 9.677 × 10−3 kWh mol−1, and meanwhile NaOH solution with a pH of 12.84 was generated with energy consumption of 2.083 × 10−3 kWh mol−1 during the recovery process of Na+ ions. It is expected that such an ESIX system can be applied for the treatment of phenol-containing high salinity wastewater. |
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| AbstractList | •Separation of the phenol and desalination could be achieved simultaneously.•Production of NaOH with this ESIX system could be realized.•The FeHCF coated electrode could work repeatedly in the series operation.•The ESIX system exhibited a very low energy consumption.
An electrochemically switched ion exchange (ESIX) system was proposed as a novel electrochemical method for the treatment of high concentration phenolic sodium salty wastewater, in which a ferric ferricyanide (FeHCF) coated electrode with rigid open framework can control the insertion/extraction of sodium (Na+) ions by switching the redox state of FeHCF. It is found that this ESIX system can not only remove the phenol and desalinate the phenol-containing wastewater simultaneously, but also regenerate the FeHCF coated electrode and produce sodium hydroxide (NaOH). In the series operation, more than 79% of phenol could be removed with energy consumption of 9.677 × 10−3 kWh mol−1, and meanwhile NaOH solution with a pH of 12.84 was generated with energy consumption of 2.083 × 10−3 kWh mol−1 during the recovery process of Na+ ions. It is expected that such an ESIX system can be applied for the treatment of phenol-containing high salinity wastewater. |
| ArticleNumber | 117125 |
| Author | Niu, Junjian Guan, Guoqing Hao, Xiaogang Wang, Zhongde Zhang, Xiang Abudula, Abuliti |
| Author_xml | – sequence: 1 givenname: Xiang surname: Zhang fullname: Zhang, Xiang organization: Department of Chemical Engineering, Taiyuan University of Technology, Taiyuan 030024, China – sequence: 2 givenname: Junjian surname: Niu fullname: Niu, Junjian organization: Department of Chemical Engineering, Taiyuan University of Technology, Taiyuan 030024, China – sequence: 3 givenname: Xiaogang surname: Hao fullname: Hao, Xiaogang organization: Department of Chemical Engineering, Taiyuan University of Technology, Taiyuan 030024, China – sequence: 4 givenname: Zhongde surname: Wang fullname: Wang, Zhongde email: wangzhongde@tyut.edu.cn organization: Department of Chemical Engineering, Taiyuan University of Technology, Taiyuan 030024, China – sequence: 5 givenname: Guoqing surname: Guan fullname: Guan, Guoqing organization: North Japan Research Institute for Sustainable Energy (NJRISE), Hirosaki University, 2-1-3, Matsubara, Aomori 030-0813, Japan – sequence: 6 givenname: Abuliti surname: Abudula fullname: Abudula, Abuliti organization: North Japan Research Institute for Sustainable Energy (NJRISE), Hirosaki University, 2-1-3, Matsubara, Aomori 030-0813, Japan |
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| CitedBy_id | crossref_primary_10_1016_j_envres_2023_117005 crossref_primary_10_3390_polym12112496 crossref_primary_10_3390_separations10070370 crossref_primary_10_1021_acsami_1c10464 crossref_primary_10_1016_j_dwt_2024_100091 crossref_primary_10_1016_j_jece_2022_109163 crossref_primary_10_1016_j_seppur_2022_120845 crossref_primary_10_1080_21655979_2021_1946631 crossref_primary_10_1016_j_cej_2021_130807 crossref_primary_10_1016_j_scitotenv_2020_143901 crossref_primary_10_1002_slct_202104074 crossref_primary_10_1016_j_jclepro_2024_142234 |
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| Keywords | Electrochemically switched ion exchange Energy consumption Phenol High salinity wastewater |
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A doi: 10.1039/C5TA03181H |
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| Snippet | •Separation of the phenol and desalination could be achieved simultaneously.•Production of NaOH with this ESIX system could be realized.•The FeHCF coated... |
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| SubjectTerms | Electrochemically switched ion exchange Energy consumption High salinity wastewater Phenol |
| Title | A novel electrochemically switched ion exchange system for phenol recovery and regeneration of NaOH from sodium phenolate wastewater |
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