A Method to Obtain Gas-PDMS Membrane Interaction Parameters for UNIQUAC Model
The recovery or capture of one or more components from gas mixture by membrane separation has become a research focus in recent years.This study investigates the gas-membrane solution equilibrium,for which Henry’s law is not applicable if the gas phase is a mixture.This problem can be solved by usin...
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| Published in | Chinese journal of chemical engineering Vol. 21; no. 5; pp. 485 - 493 |
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| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.05.2013
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1004-9541 2210-321X |
| DOI | 10.1016/S1004-9541(13)60513-3 |
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| Abstract | The recovery or capture of one or more components from gas mixture by membrane separation has become a research focus in recent years.This study investigates the gas-membrane solution equilibrium,for which Henry’s law is not applicable if the gas phase is a mixture.This problem can be solved by using UNIQUAC model to calculate the activity coefficient of gas dissolved in the membrane.A method was proposed in this study to obtain the gas-membrane interaction parameter for UNIQUAC model.By the experiments of gas permeation through polydimethylsiloxane PDMS membrane,the solubility coefficients of some gases（N2,CO2,CH4） were measured.Through non-linear fitting UNIQUAC model to the experimental results from this study and in literature（H2,O2,C3H8）,the gas-membrane interaction parameters for these gases were obtained.Based on these parameters,the activity coefficients of the dissolved gas were calculated by UNIQUAC model,and their values agree well with the experimental data.These results confirm the feasibility and effectiveness of the proposed method,which makes it possible to better predict gas-membrane solution equilibrium. |
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| AbstractList | The recovery or capture of one or more components from gas mixture by membrane separation has become a research focus in recent years.This study investigates the gas-membrane solution equilibrium,for which Henry’s law is not applicable if the gas phase is a mixture.This problem can be solved by using UNIQUAC model to calculate the activity coefficient of gas dissolved in the membrane.A method was proposed in this study to obtain the gas-membrane interaction parameter for UNIQUAC model.By the experiments of gas permeation through polydimethylsiloxane PDMS membrane,the solubility coefficients of some gases（N2,CO2,CH4） were measured.Through non-linear fitting UNIQUAC model to the experimental results from this study and in literature（H2,O2,C3H8）,the gas-membrane interaction parameters for these gases were obtained.Based on these parameters,the activity coefficients of the dissolved gas were calculated by UNIQUAC model,and their values agree well with the experimental data.These results confirm the feasibility and effectiveness of the proposed method,which makes it possible to better predict gas-membrane solution equilibrium. The recovery or capture of one or more components from gas mixture by membrane separation has become a research focus in recent years. This study investigates the gas-membrane solution equilibrium, for which Henry's law is not applicable if the gas phase is a mixture. This problem can be solved by using UNIQUAC model to calculate the activity coefficient of gas dissolved in the membrane. A method was proposed in this study to obtain the gas-membrane interaction parameter for UNIQUAC model. By the experiments of gas permeation through polydimethylsiloxane PDMS membrane, the solubility coefficients of some gases (N(2), CO(2), CH(4)) were measured. Through non-linear fitting UNIQUAC model to the experimental results from this study and in literature (H(2), O(2), C(3)H(8)), the gas-membrane interaction parameters for these gases were obtained. Based on these parameters, the activity coefficients of the dissolved gas were calculated by UNIQUAC model, and their values agree well with the experimental data. These results confirm the feasibility and effectiveness of the proposed method, which makes it possible to better predict gas-membrane solution equilibrium. The recovery or capture of one or more components from gas mixture by membrane separation has become a research focus in recent years. This study investigates the gas-membrane solution equilibrium, for which Henry's law is not applicable if the gas phase is a mixture. This problem can be solved by using UNIQUAC model to calculate the activity coefficient of gas dissolved in the membrane. A method was proposed in this study to obtain the gas-membrane interaction parameter for UNIQUAC model. By the experiments of gas permeation through polydimethylsiloxane PDMS membrane, the solubility coefficients of some gases (N2, CO2, CH4) were measured. Through non-linear fitting UNIQUAC model to the experimental results from this study and in literature (H2, O2, C3H8), the gas-membrane interaction parameters for these gases were obtained. Based on these parameters, the activity coefficients of the dissolved gas were calculated by UNIQUAC model, and their values agree well with the experimental data. These results confirm the feasibility and effectiveness of the proposed method, which makes it possible to better predict gas-membrane solution equilibrium. |
| Author | 林东杰 丁忠伟 刘丽英 马润宇 |
| AuthorAffiliation | College of Chemical Engineering, Beijing University of Chemical Technology, Beijing 100029, China Beijing Key Laboratory of Membrane Science and Technology, Beijing University of Chemical Technology, Beijing 100029, China |
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| Cites_doi | 10.1016/j.memsci.2008.08.019 10.1021/ie071493k 10.1016/j.cej.2005.09.014 10.1016/S0376-7388(98)00248-8 10.1016/j.polymer.2005.06.112 10.1016/S0376-7388(99)00193-3 10.1016/S1004-9541(08)60266-9 10.1016/j.memsci.2006.10.052 10.1016/j.memsci.2009.09.015 10.1016/0376-7388(96)00041-5 10.1016/j.memsci.2007.01.012 10.1016/j.memsci.2009.07.015 10.1016/0376-7388(95)00090-Y 10.1016/S1004-9541(11)60024-4 10.1016/S0376-7388(99)00252-5 10.1016/j.memsci.2010.02.008 10.1016/j.seppur.2010.11.010 10.1016/j.seppur.2011.02.033 10.1016/j.memsci.2009.06.047 10.1016/j.ces.2006.05.045 10.1021/ma991566e 10.1016/S0376-7388(02)00580-X 10.1016/S1004-9541(06)60138-9 10.1016/S0376-7388(01)00657-3 10.1016/S0376-7388(00)80786-3 10.1016/S1004-9541(09)60174-9 10.1016/S0376-7388(97)00150-6 |
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| Keywords | polydimethylsiloxane (PDMS) membrane UNIQUAC model solubility coefficient diffusion coefficient |
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| Notes | diffusion coefficient;solubility coefficient;polydimethylsiloxane（PDMS） membrane;UNIQUAC model LIN Dongjie 1,2,DING Zhongwei1,2,＊,LIU Liying1,2 and MA Runyu 1,2 1 College of Chemical Engineering,Beijing University of Chemical Technology,Beijing 100029,China 2 Beijing Key Laboratory of Membrane Science and Technology,Beijing University of Chemical Technology,Beijing 100029,China The recovery or capture of one or more components from gas mixture by membrane separation has become a research focus in recent years.This study investigates the gas-membrane solution equilibrium,for which Henry’s law is not applicable if the gas phase is a mixture.This problem can be solved by using UNIQUAC model to calculate the activity coefficient of gas dissolved in the membrane.A method was proposed in this study to obtain the gas-membrane interaction parameter for UNIQUAC model.By the experiments of gas permeation through polydimethylsiloxane PDMS membrane,the solubility coefficients of some gases（N2,CO2,CH4） were measured.Through non-linear fitting UNIQUAC model to the experimental results from this study and in literature（H2,O2,C3H8）,the gas-membrane interaction parameters for these gases were obtained.Based on these parameters,the activity coefficients of the dissolved gas were calculated by UNIQUAC model,and their values agree well with the experimental data.These results confirm the feasibility and effectiveness of the proposed method,which makes it possible to better predict gas-membrane solution equilibrium. 11-3270/TQ ObjectType-Article-2 SourceType-Scholarly Journals-1 ObjectType-Feature-1 content type line 23 ObjectType-Article-1 ObjectType-Feature-2 |
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| Snippet | The recovery or capture of one or more components from gas mixture by membrane separation has become a research focus in recent years.This study investigates... The recovery or capture of one or more components from gas mixture by membrane separation has become a research focus in recent years. This study investigates... |
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| SubjectTerms | Activity coefficients Chemical engineering diffusion coefficient Dissolution Feasibility Fittings Interaction parameters Mathematical models Membranes Nonlinearity PDMS膜 polydimethylsiloxane (PDMS) membrane Separation Solubility solubility coefficient UNIQUAC model UNIQUAC模型 天然气 气体混合物 溶液平衡 溶解度系数 相互作用参数 聚二甲基硅氧烷 |
| Title | A Method to Obtain Gas-PDMS Membrane Interaction Parameters for UNIQUAC Model |
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