In situ fabrication of 1D CdS nanorod/2D Ti3C2 MXene nanosheet Schottky heterojunction toward enhanced photocatalytic hydrogen evolution
[Display omitted] •1D CdS/2D Ti3C2 MXene Schottky heterojunction was successfully fabricated.•In situ constructed Schottky photocatalyst exhibits enhanced HER performance.•Ultrathin 2D MXene enhances light absorption and accelerates charge transport.•The specific Schottky interface is responsible fo...
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| Published in | Applied catalysis. B, Environmental Vol. 268; p. 118382 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
05.07.2020
Elsevier BV |
| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•1D CdS/2D Ti3C2 MXene Schottky heterojunction was successfully fabricated.•In situ constructed Schottky photocatalyst exhibits enhanced HER performance.•Ultrathin 2D MXene enhances light absorption and accelerates charge transport.•The specific Schottky interface is responsible for the improved HER activity.
Benefiting from excellent metallic conductivity, full-spectrum solar energy absorption and rich active sites on the surface, atomically thin two-dimensional transition metal carbide (2D MXene) shows great promise in improving solar-to-hydrogen efficiency and has drawn intense interest in the field of photocatalysis. However, controllable construction of ultrathin 2D MXene-based heterojunction photocatalysts still remains a significant challenge. Herein, one-dimensional (1D) CdS nanorod/2D MXene nanosheet heterojunctions with well-defined nanostructures and strong interfacial coupling are fabricated by in situ assembling solvothermally-generated CdS nanorods on ultrathin Ti3C2 MXene nanosheets. Due to their specific interface characteristics, 1D/2D Schottky heterojunction is capable of providing accelerated charge separation and a lower Schottky barrier for solar-driven hydrogen evolution from water splitting. As expected, the Schottky-based photocatalyst is 7-fold more active in the illuminated hydrogen evolution reaction (HER) than pristine CdS nanorods, implying the synergistic effects between n-type semiconductor CdS and highly conductive 2D Ti3C2 MXene nanosheets. |
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| AbstractList | [Display omitted]
•1D CdS/2D Ti3C2 MXene Schottky heterojunction was successfully fabricated.•In situ constructed Schottky photocatalyst exhibits enhanced HER performance.•Ultrathin 2D MXene enhances light absorption and accelerates charge transport.•The specific Schottky interface is responsible for the improved HER activity.
Benefiting from excellent metallic conductivity, full-spectrum solar energy absorption and rich active sites on the surface, atomically thin two-dimensional transition metal carbide (2D MXene) shows great promise in improving solar-to-hydrogen efficiency and has drawn intense interest in the field of photocatalysis. However, controllable construction of ultrathin 2D MXene-based heterojunction photocatalysts still remains a significant challenge. Herein, one-dimensional (1D) CdS nanorod/2D MXene nanosheet heterojunctions with well-defined nanostructures and strong interfacial coupling are fabricated by in situ assembling solvothermally-generated CdS nanorods on ultrathin Ti3C2 MXene nanosheets. Due to their specific interface characteristics, 1D/2D Schottky heterojunction is capable of providing accelerated charge separation and a lower Schottky barrier for solar-driven hydrogen evolution from water splitting. As expected, the Schottky-based photocatalyst is 7-fold more active in the illuminated hydrogen evolution reaction (HER) than pristine CdS nanorods, implying the synergistic effects between n-type semiconductor CdS and highly conductive 2D Ti3C2 MXene nanosheets. Benefiting from excellent metallic conductivity, full-spectrum solar energy absorption and rich active sites on the surface, atomically thin two-dimensional transition metal carbide (2D MXene) shows great promise in improving solar-to-hydrogen efficiency and has drawn intense interest in the field of photocatalysis. However, controllable construction of ultrathin 2D MXene-based heterojunction photocatalysts still remains a significant challenge. Herein, one-dimensional (1D) CdS nanorod/2D MXene nanosheet heterojunctions with well-defined nanostructures and strong interfacial coupling are fabricated by in situ assembling solvothermally-generated CdS nanorods on ultrathin Ti3C2 MXene nanosheets. Due to their specific interface characteristics, 1D/2D Schottky heterojunction is capable of providing accelerated charge separation and a lower Schottky barrier for solar-driven hydrogen evolution from water splitting. As expected, the Schottky-based photocatalyst is 7-fold more active in the illuminated hydrogen evolution reaction (HER) than pristine CdS nanorods, implying the synergistic effects between n-type semiconductor CdS and highly conductive 2D Ti3C2 MXene nanosheets. |
| ArticleNumber | 118382 |
| Author | Yang, Xiaofei Tian, Lin Liu, Qinqin Chen, Zupeng Xu, Haotian Tang, Hua Zou, Zhaoyong Xiao, Rong Zhao, Chengxiao Lin, Zixia |
| Author_xml | – sequence: 1 givenname: Rong surname: Xiao fullname: Xiao, Rong organization: School of Materials Science and Engineering, Jiangsu University, Zhenjiang, 212013, PR China – sequence: 2 givenname: Chengxiao surname: Zhao fullname: Zhao, Chengxiao organization: College of Science, Institute of Materials Physics and Chemistry, Nanjing Forestry University, Nanjing, 210037, PR China – sequence: 3 givenname: Zhaoyong surname: Zou fullname: Zou, Zhaoyong organization: State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, PR China – sequence: 4 givenname: Zupeng orcidid: 0000-0002-7351-3240 surname: Chen fullname: Chen, Zupeng organization: Institute for Chemical and Bioengineering, Department of Chemistry and Applied Biosciences, ETH Zürich, 8093 Zürich, Switzerland – sequence: 5 givenname: Lin surname: Tian fullname: Tian, Lin organization: School of Materials Science and Engineering, Jiangsu University, Zhenjiang, 212013, PR China – sequence: 6 givenname: Haotian surname: Xu fullname: Xu, Haotian organization: School of Materials Science and Engineering, Jiangsu University, Zhenjiang, 212013, PR China – sequence: 7 givenname: Hua surname: Tang fullname: Tang, Hua organization: School of Materials Science and Engineering, Jiangsu University, Zhenjiang, 212013, PR China – sequence: 8 givenname: Qinqin surname: Liu fullname: Liu, Qinqin email: qqliu@ujs.edu.cn organization: School of Materials Science and Engineering, Jiangsu University, Zhenjiang, 212013, PR China – sequence: 9 givenname: Zixia surname: Lin fullname: Lin, Zixia organization: Testing Center, Yangzhou University, Yangzhou 225009, PR China – sequence: 10 givenname: Xiaofei orcidid: 0000-0003-1972-4562 surname: Yang fullname: Yang, Xiaofei email: xiaofei.yang@njfu.edu.cn organization: School of Materials Science and Engineering, Jiangsu University, Zhenjiang, 212013, PR China |
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| Snippet | [Display omitted]
•1D CdS/2D Ti3C2 MXene Schottky heterojunction was successfully fabricated.•In situ constructed Schottky photocatalyst exhibits enhanced HER... Benefiting from excellent metallic conductivity, full-spectrum solar energy absorption and rich active sites on the surface, atomically thin two-dimensional... |
| SourceID | proquest crossref elsevier |
| SourceType | Aggregation Database Enrichment Source Index Database Publisher |
| StartPage | 118382 |
| SubjectTerms | CdS Energy absorption Evolution Fabrication Heterojunctions Hydrogen Hydrogen evolution reactions Metal carbides MXene MXenes N-type semiconductors Nanorods Nanosheets Nanostructure Photocatalysis Photocatalysts Photocatalytic hydrogen evolution Schottky heterojunction Solar energy Synergistic effect Transition metals Water splitting |
| Title | In situ fabrication of 1D CdS nanorod/2D Ti3C2 MXene nanosheet Schottky heterojunction toward enhanced photocatalytic hydrogen evolution |
| URI | https://dx.doi.org/10.1016/j.apcatb.2019.118382 https://www.proquest.com/docview/2435541252 |
| Volume | 268 |
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