In Situ Synthesis of MnMgFe-LDH on Biochar for Electrochemical Detection and Removal of Cd2+ in Aqueous Solution
Herein, MnMgFe-layered double hydroxides/biochar (MnMgFe-LDHs/BC) composite was fabricated by immobilizing MnMgFe-LDHs on BC via the coprecipitation method, which was employed as an effective material for the detection and removal of Cd2+ from aqueous media. A lamellar structure of MnMgFe-LDHs with...
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| Published in | Molecules (Basel, Switzerland) Vol. 27; no. 22; p. 7875 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
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15.11.2022
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| Abstract | Herein, MnMgFe-layered double hydroxides/biochar (MnMgFe-LDHs/BC) composite was fabricated by immobilizing MnMgFe-LDHs on BC via the coprecipitation method, which was employed as an effective material for the detection and removal of Cd2+ from aqueous media. A lamellar structure of MnMgFe-LDHs with abundant surface-hydroxyl groups and various interlayer anions inside present a greater chance of trapping Cd2+. Meanwhile, the conductive BC with a porous structure provides numerous channels for the adsorption of Cd2+. Using the MnMgFe-LDHs/BC-based sensor, Cd2+ can be detected with a low limit of detection down to 0.03 ng/L. The feasibility of detecting Cd2+ in paddy water was also carried out, with satisfactory recoveries ranging from 97.3 to 102.3%. In addition, the MnMgFe-LDHs/BC material as an adsorbent was applied to remove Cd2+ from water with adsorption capacity of 118 mg/g, and the removal efficiency can reach 91%. These results suggest that the as-prepared MnMgFe-LDHs/BC can serve as a favorable platform for efficient determination and removal of Cd2+ in water. |
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| AbstractList | Herein, MnMgFe-layered double hydroxides/biochar (MnMgFe-LDHs/BC) composite was fabricated by immobilizing MnMgFe-LDHs on BC via the coprecipitation method, which was employed as an effective material for the detection and removal of Cd2+ from aqueous media. A lamellar structure of MnMgFe-LDHs with abundant surface-hydroxyl groups and various interlayer anions inside present a greater chance of trapping Cd2+. Meanwhile, the conductive BC with a porous structure provides numerous channels for the adsorption of Cd2+. Using the MnMgFe-LDHs/BC-based sensor, Cd2+ can be detected with a low limit of detection down to 0.03 ng/L. The feasibility of detecting Cd2+ in paddy water was also carried out, with satisfactory recoveries ranging from 97.3 to 102.3%. In addition, the MnMgFe-LDHs/BC material as an adsorbent was applied to remove Cd2+ from water with adsorption capacity of 118 mg/g, and the removal efficiency can reach 91%. These results suggest that the as-prepared MnMgFe-LDHs/BC can serve as a favorable platform for efficient determination and removal of Cd2+ in water. Herein, MnMgFe-layered double hydroxides/biochar (MnMgFe-LDHs/BC) composite was fabricated by immobilizing MnMgFe-LDHs on BC via the coprecipitation method, which was employed as an effective material for the detection and removal of Cd 2+ from aqueous media. A lamellar structure of MnMgFe-LDHs with abundant surface-hydroxyl groups and various interlayer anions inside present a greater chance of trapping Cd 2+ . Meanwhile, the conductive BC with a porous structure provides numerous channels for the adsorption of Cd 2+ . Using the MnMgFe-LDHs/BC-based sensor, Cd 2+ can be detected with a low limit of detection down to 0.03 ng/L. The feasibility of detecting Cd 2+ in paddy water was also carried out, with satisfactory recoveries ranging from 97.3 to 102.3%. In addition, the MnMgFe-LDHs/BC material as an adsorbent was applied to remove Cd 2+ from water with adsorption capacity of 118 mg/g, and the removal efficiency can reach 91%. These results suggest that the as-prepared MnMgFe-LDHs/BC can serve as a favorable platform for efficient determination and removal of Cd 2+ in water. Herein, MnMgFe-layered double hydroxides/biochar (MnMgFe-LDHs/BC) composite was fabricated by immobilizing MnMgFe-LDHs on BC via the coprecipitation method, which was employed as an effective material for the detection and removal of Cd2+ from aqueous media. A lamellar structure of MnMgFe-LDHs with abundant surface-hydroxyl groups and various interlayer anions inside present a greater chance of trapping Cd2+. Meanwhile, the conductive BC with a porous structure provides numerous channels for the adsorption of Cd2+. Using the MnMgFe-LDHs/BC-based sensor, Cd2+ can be detected with a low limit of detection down to 0.03 ng/L. The feasibility of detecting Cd2+ in paddy water was also carried out, with satisfactory recoveries ranging from 97.3 to 102.3%. In addition, the MnMgFe-LDHs/BC material as an adsorbent was applied to remove Cd2+ from water with adsorption capacity of 118 mg/g, and the removal efficiency can reach 91%. These results suggest that the as-prepared MnMgFe-LDHs/BC can serve as a favorable platform for efficient determination and removal of Cd2+ in water.Herein, MnMgFe-layered double hydroxides/biochar (MnMgFe-LDHs/BC) composite was fabricated by immobilizing MnMgFe-LDHs on BC via the coprecipitation method, which was employed as an effective material for the detection and removal of Cd2+ from aqueous media. A lamellar structure of MnMgFe-LDHs with abundant surface-hydroxyl groups and various interlayer anions inside present a greater chance of trapping Cd2+. Meanwhile, the conductive BC with a porous structure provides numerous channels for the adsorption of Cd2+. Using the MnMgFe-LDHs/BC-based sensor, Cd2+ can be detected with a low limit of detection down to 0.03 ng/L. The feasibility of detecting Cd2+ in paddy water was also carried out, with satisfactory recoveries ranging from 97.3 to 102.3%. In addition, the MnMgFe-LDHs/BC material as an adsorbent was applied to remove Cd2+ from water with adsorption capacity of 118 mg/g, and the removal efficiency can reach 91%. These results suggest that the as-prepared MnMgFe-LDHs/BC can serve as a favorable platform for efficient determination and removal of Cd2+ in water. |
| Author | Wang, Haocheng Yu, Yongfang Yang, Wenting Huang, Guoqin |
| AuthorAffiliation | Key Laboratory of Crop Physiology, Ecology and Genetic Breeding, Ministry of Education, Research Center on Ecological Sciences, Jiangxi Agricultural University, Nanchang 330045, China |
| AuthorAffiliation_xml | – name: Key Laboratory of Crop Physiology, Ecology and Genetic Breeding, Ministry of Education, Research Center on Ecological Sciences, Jiangxi Agricultural University, Nanchang 330045, China |
| Author_xml | – sequence: 1 givenname: Yongfang surname: Yu fullname: Yu, Yongfang – sequence: 2 givenname: Wenting orcidid: 0000-0001-9029-0344 surname: Yang fullname: Yang, Wenting – sequence: 3 givenname: Haocheng surname: Wang fullname: Wang, Haocheng – sequence: 4 givenname: Guoqin surname: Huang fullname: Huang, Guoqin |
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| SubjectTerms | Adsorption Aqueous solutions biochar cadmium electrochemical determination Electrodes layered double hydroxides Morphology Sensors Voltammetry |
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| Title | In Situ Synthesis of MnMgFe-LDH on Biochar for Electrochemical Detection and Removal of Cd2+ in Aqueous Solution |
| URI | https://www.proquest.com/docview/2739448762 https://www.proquest.com/docview/2740505837 https://pubmed.ncbi.nlm.nih.gov/PMC9696249 https://doaj.org/article/ad2cd33a4e774e8b804b3cb4c94b8758 |
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