Photoexcitation of dimethyl sulfide and dimethyl disulfide in the vacuum ultraviolet region: Rydberg states and photofragment emissions
Photoabsorption cross sections and fluorescence excitation spectra of dimethyl sulfide (DMS) and dimethyl disulfide (DMDS) vapors have been studied in the 110–220 nm region using synchrotron radiation. For DMS, a new Rydberg series originating from the ns orbital is identified. A number of broad ban...
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| Published in | Chemical physics Vol. 130; no. 1-3; pp. 401 - 408 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
15.02.1989
Elsevier |
| Subjects | |
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| Abstract | Photoabsorption cross sections and fluorescence excitation spectra of dimethyl sulfide (DMS) and dimethyl disulfide (DMDS) vapors have been studied in the 110–220 nm region using synchrotron radiation. For DMS, a new Rydberg series originating from the ns orbital is identified. A number of broad bands from DMDS are assigned as Rydberg transitions. Emissions from DMS and DMDS are assigned as the CH3(A-X) band. For DMDS, another emission which is attributable to the S2(B-X) band appears in the excitation below 125 nm. Photodissociation processes forming the excited fragments are discussed. |
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| AbstractList | Photoabsorption cross sections and fluorescence excitation spectra of dimethyl sulfide (DMS) and dimethyl disulfide (DMDS) vapors have been studied in the 110–220 nm region using synchrotron radiation. For DMS, a new Rydberg series originating from the ns orbital is identified. A number of broad bands from DMDS are assigned as Rydberg transitions. Emissions from DMS and DMDS are assigned as the CH3(A-X) band. For DMDS, another emission which is attributable to the S2(B-X) band appears in the excitation below 125 nm. Photodissociation processes forming the excited fragments are discussed. |
| Author | Hiraya, Atsunari Shobatake, Kosuke Tokue, Ikuo |
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| Cites_doi | 10.1080/00268976600100811 10.1039/tf9706601987 10.1098/rspa.1950.0081 10.1016/0301-0104(83)80010-X 10.1016/0009-2614(81)85632-1 10.1016/0009-2614(86)87156-1 10.1139/p79-106 10.1063/1.1731956 10.1063/1.447685 10.1021/ja00769a001 10.1246/bcsj.48.33 10.1063/1.435173 10.1063/1.1680037 10.1063/1.1681633 10.1016/0301-0104(87)80212-4 10.1016/0301-0104(81)85101-4 10.1088/0022-3700/14/22/002 10.1021/j100547a013 10.1016/0009-2614(77)85117-8 10.1063/1.1727769 10.1063/1.1680457 10.1063/1.1696534 10.1016/0022-2852(69)90366-X |
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| Keywords | Fluorescence spectrum Organic disulfide Gaseous state Rydberg state Excitation spectrum Vibronic transition Photodissociation Experimental study Synchrotron radiation Vacuum ultraviolet spectrum Organic sulfide Organic compounds |
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| Title | Photoexcitation of dimethyl sulfide and dimethyl disulfide in the vacuum ultraviolet region: Rydberg states and photofragment emissions |
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