A general approach to cobalt-based homobimetallic phosphide ultrathin nanosheets for highly efficient oxygen evolution in alkaline media
A general and effective approach was proposed to fabricate a new family of Co-based bimetallic phosphide ultrathin nanosheets (CoM-P-NS, M = Ni, Mn, Cu, Zn) with homogeneous composition and unique porous architecture using ultrathin metal–organic framework nanosheets (MOFNs) as precursors for the fi...
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| Published in | Energy & environmental science Vol. 10; no. 4; pp. 893 - 899 |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
01.04.2017
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| Subjects | |
| Online Access | Get full text |
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| Abstract | A general and effective approach was proposed to fabricate a new family of Co-based bimetallic phosphide ultrathin nanosheets (CoM-P-NS, M = Ni, Mn, Cu, Zn) with homogeneous composition and unique porous architecture using ultrathin metal–organic framework nanosheets (MOFNs) as precursors for the first time, which yielded synergistically active sites, mass transport and dynamic modulations for the oxygen evolution reaction (OER). The optimized samples showed remarkable oxygen evolution activity in alkaline electrolytes, outperforming both the commercial RuO
2
and Ir/C benchmarks and ranking the best among all the metal-phosphide electrocatalysts reported to date. |
|---|---|
| AbstractList | A general and effective approach was proposed to fabricate a new family of Co-based bimetallic phosphide ultrathin nanosheets (CoM-P-NS, M = Ni, Mn, Cu, Zn) with homogeneous composition and unique porous architecture using ultrathin metal–organic framework nanosheets (MOFNs) as precursors for the first time, which yielded synergistically active sites, mass transport and dynamic modulations for the oxygen evolution reaction (OER). The optimized samples showed remarkable oxygen evolution activity in alkaline electrolytes, outperforming both the commercial RuO
2
and Ir/C benchmarks and ranking the best among all the metal-phosphide electrocatalysts reported to date. A general and effective approach was proposed to fabricate a new family of Co-based bimetallic phosphide ultrathin nanosheets (CoM-P-NS, M = Ni, Mn, Cu, Zn) with homogeneous composition and unique porous architecture using ultrathin metal-organic framework nanosheets (MOFNs) as precursors for the first time, which yielded synergistically active sites, mass transport and dynamic modulations for the oxygen evolution reaction (OER). The optimized samples showed remarkable oxygen evolution activity in alkaline electrolytes, outperforming both the commercial RuO2 and Ir/C benchmarks and ranking the best among all the metal-phosphide electrocatalysts reported to date. |
| Author | Yuan, Zhongke Lin, Wensheng Xiao, Xiaofen Zhao, Shenlong Zhang, Qiang Wang, Shuangyin Dai, Liming Li, Jing Yu, Dingshan He, Chun-Ting |
| Author_xml | – sequence: 1 givenname: Xiaofen surname: Xiao fullname: Xiao, Xiaofen organization: Key Laboratory for Polymeric Composite and Functional Materials of Ministry of Education, Key Laboratory of High Performance Polymer-based Composites of Guangdong Province, School of Chemistry, Sun Yat-Sen University, Guangzhou 510275 – sequence: 2 givenname: Chun-Ting surname: He fullname: He, Chun-Ting organization: MOE Key Laboratory of Bioinorganic and Synthetic Chemistry, School of Chemistry, Sun Yat-Sen University, Guangzhou 510275, China – sequence: 3 givenname: Shenlong surname: Zhao fullname: Zhao, Shenlong organization: Laboratory for Nanosystem and Hierarchy Fabrication, National Center for Nanoscience and Technology, Beijing 100190, China – sequence: 4 givenname: Jing surname: Li fullname: Li, Jing organization: Key Laboratory for Polymeric Composite and Functional Materials of Ministry of Education, Key Laboratory of High Performance Polymer-based Composites of Guangdong Province, School of Chemistry, Sun Yat-Sen University, Guangzhou 510275 – sequence: 5 givenname: Wensheng surname: Lin fullname: Lin, Wensheng organization: Key Laboratory for Polymeric Composite and Functional Materials of Ministry of Education, Key Laboratory of High Performance Polymer-based Composites of Guangdong Province, School of Chemistry, Sun Yat-Sen University, Guangzhou 510275 – sequence: 6 givenname: Zhongke surname: Yuan fullname: Yuan, Zhongke organization: Key Laboratory for Polymeric Composite and Functional Materials of Ministry of Education, Key Laboratory of High Performance Polymer-based Composites of Guangdong Province, School of Chemistry, Sun Yat-Sen University, Guangzhou 510275 – sequence: 7 givenname: Qiang surname: Zhang fullname: Zhang, Qiang organization: Beijing Key Laboratory of Green Chemical, Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing, China – sequence: 8 givenname: Shuangyin surname: Wang fullname: Wang, Shuangyin organization: State Key Laboratory of Chem/Bio-Sensing and Chemometric, College of Chemistry and Chemical Engineering, Hunan University, Changsha, China – sequence: 9 givenname: Liming surname: Dai fullname: Dai, Liming organization: Department of Macromolecule Science and Engineering, Case Western Reserve University, Ohio, USA – sequence: 10 givenname: Dingshan surname: Yu fullname: Yu, Dingshan organization: Key Laboratory for Polymeric Composite and Functional Materials of Ministry of Education, Key Laboratory of High Performance Polymer-based Composites of Guangdong Province, School of Chemistry, Sun Yat-Sen University, Guangzhou 510275 |
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