Anisotropic localized surface plasmon resonance of vanadium dioxide rods in flexible thermochromic film towards multifunctionality

Plasmonic thermochromic films are promising for smart window applications. Hereby, we develop a flexible plasmonic thermochromic film towards multifunctionality. The double-layer film consists of a bottom layer of W/Mg co-doped vanadium dioxide (VO2) rods in a polyurethane acrylate matrix and a top...

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Published inSolar energy materials and solar cells Vol. 230; p. 111163
Main Authors Xu, Qiyang, Ke, Yujie, Feng, Chengchen, Chen, Cong, Wen, Zuohao, Wang, Haoran, Sun, Miaoyang, Liu, Xinghai, Liu, Hai, Magdassi, Shlomo, Li, Houbin, Huang, Chi, Long, Yi
Format Journal Article
LanguageEnglish
Published Amsterdam Elsevier B.V 15.09.2021
Elsevier BV
Subjects
Modulation
Plasmonics
Polyurethane
Polyurethane resins
Resonance
Rods
Silica
Silicon dioxide
Smart materials
Smart window
Solar energy
Solar modulation
Surface plasmon resonance
Thermal insulation
Thermal management
Thermochromics
Time domain analysis
Transition temperature
Transition temperatures
Vanadium
Vanadium dioxide
Vanadium oxides
VO2
Wettability
Windows (apertures)
Wettability
Solar modulation
Thermochromics
Smart window
VO2
Thermal management
Surface plasmon resonance
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Abstract Plasmonic thermochromic films are promising for smart window applications. Hereby, we develop a flexible plasmonic thermochromic film towards multifunctionality. The double-layer film consists of a bottom layer of W/Mg co-doped vanadium dioxide (VO2) rods in a polyurethane acrylate matrix and a top layer of hollow silica spheres (HSSs). Based on the finite-difference time-domain (FDTD) method, we demonstrate for the first time, a transverse and a longitudinal mode of VO2 localized surface plasmonic resonance (LSPR) in near- and mid-infrared bands, respectively, and only the transverse mode contributes to the solar energy modulation performance. The film shows a luminous transmittance of 46.2%, a solar energy modulation of 10.8%, and a critical transition temperature of 36.9 °C. The HSSs overcoating enhances the surface hydrophilicity and thermal insulation, which give rise to more favored functionalities for windows. [Display omitted] •The first identification of anisotropic LSPR on VO2 rods.•FDTD method proves only transverse mode of LSPR contributes to solar modulation.•Simultaneous improved flexibility, wettability, solar and thermal modulations.•The thermochromic film is promised for multifunctional smart windows.
AbstractList Plasmonic thermochromic films are promising for smart window applications. Hereby, we develop a flexible plasmonic thermochromic film towards multifunctionality. The double-layer film consists of a bottom layer of W/Mg co-doped vanadium dioxide (VO2) rods in a polyurethane acrylate matrix and a top layer of hollow silica spheres (HSSs). Based on the finite-difference time-domain (FDTD) method, we demonstrate for the first time, a transverse and a longitudinal mode of VO2 localized surface plasmonic resonance (LSPR) in near- and mid-infrared bands, respectively, and only the transverse mode contributes to the solar energy modulation performance. The film shows a luminous transmittance of 46.2%, a solar energy modulation of 10.8%, and a critical transition temperature of 36.9 °C. The HSSs overcoating enhances the surface hydrophilicity and thermal insulation, which give rise to more favored functionalities for windows.
Plasmonic thermochromic films are promising for smart window applications. Hereby, we develop a flexible plasmonic thermochromic film towards multifunctionality. The double-layer film consists of a bottom layer of W/Mg co-doped vanadium dioxide (VO2) rods in a polyurethane acrylate matrix and a top layer of hollow silica spheres (HSSs). Based on the finite-difference time-domain (FDTD) method, we demonstrate for the first time, a transverse and a longitudinal mode of VO2 localized surface plasmonic resonance (LSPR) in near- and mid-infrared bands, respectively, and only the transverse mode contributes to the solar energy modulation performance. The film shows a luminous transmittance of 46.2%, a solar energy modulation of 10.8%, and a critical transition temperature of 36.9 °C. The HSSs overcoating enhances the surface hydrophilicity and thermal insulation, which give rise to more favored functionalities for windows. [Display omitted] •The first identification of anisotropic LSPR on VO2 rods.•FDTD method proves only transverse mode of LSPR contributes to solar modulation.•Simultaneous improved flexibility, wettability, solar and thermal modulations.•The thermochromic film is promised for multifunctional smart windows.
ArticleNumber 111163
Author Li, Houbin
Wang, Haoran
Long, Yi
Chen, Cong
Liu, Xinghai
Sun, Miaoyang
Liu, Hai
Huang, Chi
Ke, Yujie
Feng, Chengchen
Xu, Qiyang
Magdassi, Shlomo
Wen, Zuohao
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  email: longyi@ntu.edu.sg
  organization: School of Information and Control Engineering, China University of Mining and Technology, Xuzhou, Jiangsu, 221116, PR China
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Keywords Wettability
Solar modulation
Thermochromics
Smart window
VO2
Thermal management
Surface plasmon resonance
Language English
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Snippet Plasmonic thermochromic films are promising for smart window applications. Hereby, we develop a flexible plasmonic thermochromic film towards...
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StartPage 111163
SubjectTerms Modulation
Plasmonics
Polyurethane
Polyurethane resins
Resonance
Rods
Silica
Silicon dioxide
Smart materials
Smart window
Solar energy
Solar modulation
Surface plasmon resonance
Thermal insulation
Thermal management
Thermochromics
Time domain analysis
Transition temperature
Transition temperatures
Vanadium
Vanadium dioxide
Vanadium oxides
VO2
Wettability
Windows (apertures)
Title Anisotropic localized surface plasmon resonance of vanadium dioxide rods in flexible thermochromic film towards multifunctionality
URI https://dx.doi.org/10.1016/j.solmat.2021.111163
https://www.proquest.com/docview/2581541425
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