Improved hydrogen evolution activity of layered double hydroxide by optimizing the electronic structure
[Display omitted] •P doping can weaken MO bonds by forming PO bonds.•The deposition of metal nanodots can destabilize water molecules.•This strategy can effectively improve Volmer and Heyrovsky process of HER catalysis.•The mechanism of enhanced HER activity is well explained. The layered double hyd...
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| Published in | Applied catalysis. B, Environmental Vol. 297; p. 120478 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
15.11.2021
Elsevier BV |
| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•P doping can weaken MO bonds by forming PO bonds.•The deposition of metal nanodots can destabilize water molecules.•This strategy can effectively improve Volmer and Heyrovsky process of HER catalysis.•The mechanism of enhanced HER activity is well explained.
The layered double hydroxides (LDHs) are considered to own great potential to serve as a catalyst for water electrolysis, while their extremely poor hydrogen evolution reaction (HER) activity limits their application. Herein, a general designing strategy to improve the HER activity of LDHs by P doping and deposition of metal nanodots (NDs) is proposed, which increases one order of magnitude higher than that of pristine LDHs. The obtained electrocatalyst, such as Cu NDs/P-FeCoLDH (CPFC-LDH), reaching a current density of 10 mA/cm2 with only 63 mV overpotential for HER in alkaline electrolyte. The adsorption energy of Hads and OH on catalyst is optimized by this strategy, which can weaken the interaction between the adsorbed Hads and electronegative oxygen in LDHs by formation of PO bonds. This work provides a strategy to develop LDHs materials with high catalytic activity for HER. |
|---|---|
| AbstractList | The layered double hydroxides (LDHs) are considered to own great potential to serve as a catalyst for water electrolysis, while their extremely poor hydrogen evolution reaction (HER) activity limits their application. Herein, a general designing strategy to improve the HER activity of LDHs by P doping and deposition of metal nanodots (NDs) is proposed, which increases one order of magnitude higher than that of pristine LDHs. The obtained electrocatalyst, such as Cu NDs/P-FeCoLDH (CPFC-LDH), reaching a current density of 10 mA/cm2 with only 63 mV overpotential for HER in alkaline electrolyte. The adsorption energy of Hads and OH on catalyst is optimized by this strategy, which can weaken the interaction between the adsorbed Hads and electronegative oxygen in LDHs by formation of P-O bonds. This work provides a strategy to develop LDHs materials with high catalytic activity for HER. [Display omitted] •P doping can weaken MO bonds by forming PO bonds.•The deposition of metal nanodots can destabilize water molecules.•This strategy can effectively improve Volmer and Heyrovsky process of HER catalysis.•The mechanism of enhanced HER activity is well explained. The layered double hydroxides (LDHs) are considered to own great potential to serve as a catalyst for water electrolysis, while their extremely poor hydrogen evolution reaction (HER) activity limits their application. Herein, a general designing strategy to improve the HER activity of LDHs by P doping and deposition of metal nanodots (NDs) is proposed, which increases one order of magnitude higher than that of pristine LDHs. The obtained electrocatalyst, such as Cu NDs/P-FeCoLDH (CPFC-LDH), reaching a current density of 10 mA/cm2 with only 63 mV overpotential for HER in alkaline electrolyte. The adsorption energy of Hads and OH on catalyst is optimized by this strategy, which can weaken the interaction between the adsorbed Hads and electronegative oxygen in LDHs by formation of PO bonds. This work provides a strategy to develop LDHs materials with high catalytic activity for HER. |
| ArticleNumber | 120478 |
| Author | Wang, Jiajia Dong, Haoran Feng, Haopeng Yu, Jiangfang Ni, Ting Tang, Lin Zhu, Xu Tang, Jing Liang, Chao Tang, Wangwang |
| Author_xml | – sequence: 1 givenname: Haopeng surname: Feng fullname: Feng, Haopeng organization: College of Environmental Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 2 givenname: Jiangfang surname: Yu fullname: Yu, Jiangfang organization: College of Environmental Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 3 givenname: Lin surname: Tang fullname: Tang, Lin email: tanglin@hnu.edu.cn organization: College of Environmental Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 4 givenname: Jiajia surname: Wang fullname: Wang, Jiajia organization: College of Environmental Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 5 givenname: Haoran surname: Dong fullname: Dong, Haoran organization: College of Environmental Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 6 givenname: Ting surname: Ni fullname: Ni, Ting organization: College of Environmental Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 7 givenname: Jing surname: Tang fullname: Tang, Jing organization: College of Environmental Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 8 givenname: Wangwang surname: Tang fullname: Tang, Wangwang organization: College of Environmental Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 9 givenname: Xu surname: Zhu fullname: Zhu, Xu organization: College of Environmental Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 10 givenname: Chao surname: Liang fullname: Liang, Chao organization: College of Environmental Science and Engineering, Hunan University, Changsha, 410082, China |
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•P doping can weaken MO bonds by forming PO bonds.•The deposition of metal nanodots can destabilize water molecules.•This strategy can... The layered double hydroxides (LDHs) are considered to own great potential to serve as a catalyst for water electrolysis, while their extremely poor hydrogen... |
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| SubjectTerms | Catalysts Catalytic activity Copper Destabilizing DFT calculation Electrocatalysts Electrolysis Electronegativity Electronic structure Hydrogen evolution reaction Hydrogen evolution reactions Hydroxides LDH |
| Title | Improved hydrogen evolution activity of layered double hydroxide by optimizing the electronic structure |
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