Magnetically recoverable highly efficient visible-light-active g-C3N4/Fe3O4/Ag2WO4/AgBr nanocomposites for photocatalytic degradations of environmental pollutants
[Display omitted] •Magnetically recoverable g-C3N4/Fe3O4/Ag2WO4/AgBr photocatalyst is reported.•g-C3N4/Fe3O4/Ag2WO4/AgBr (30%) nanocomposite exhibited the highest activity.•Photocatalytic activity is 21-folds greater than g-C3N4 in RhB degradation.•The photocatalyst is magnetically separated after s...
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| Published in | Advanced powder technology : the international journal of the Society of Powder Technology, Japan Vol. 29; no. 1; pp. 94 - 105 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.01.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•Magnetically recoverable g-C3N4/Fe3O4/Ag2WO4/AgBr photocatalyst is reported.•g-C3N4/Fe3O4/Ag2WO4/AgBr (30%) nanocomposite exhibited the highest activity.•Photocatalytic activity is 21-folds greater than g-C3N4 in RhB degradation.•The photocatalyst is magnetically separated after successive runs.
Herein, magnetically recoverable g-C3N4/Fe3O4/Ag2WO4/AgBr (gCN/M/AgW/AgBr) nanocomposites, as greatly efficient visible-light-active photocatalysts, were fabricated by successive decoration of Fe3O4, Ag2WO4, and AgBr over g-C3N4 (gCN) and they were characterized by XRD, EDX, SEM, TEM, HRTEM, UV–vis DRS, FT-IR, PL, TG, and VSM analysis. Visible-light-induced photocatalytic performances were studied by degradations of RhB, MB, MO, and fuchsine pollutants. It was confirmed that the nanocomposites are effective in the reduction of e−/h+ recombination through the matched interactions between energy bands of gCN, Fe3O4, Ag2WO4, and AgBr semiconductors. The highest photocatalytic degradation efficiency was observed for the gCN/M/AgW/AgBr (30%) nanocomposite when it was refluxed for 30 min. Activity of this nanocomposite is almost 21, 41, 94, and 10-folds greater than those of the gCN toward the degradations of RhB, MB, MO, and fuchsine pollutants, respectively. Additionally, a mechanism for the superior photocatalytic performances was proposed using reactive species scavenging experiments and characterization results. |
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| AbstractList | [Display omitted]
•Magnetically recoverable g-C3N4/Fe3O4/Ag2WO4/AgBr photocatalyst is reported.•g-C3N4/Fe3O4/Ag2WO4/AgBr (30%) nanocomposite exhibited the highest activity.•Photocatalytic activity is 21-folds greater than g-C3N4 in RhB degradation.•The photocatalyst is magnetically separated after successive runs.
Herein, magnetically recoverable g-C3N4/Fe3O4/Ag2WO4/AgBr (gCN/M/AgW/AgBr) nanocomposites, as greatly efficient visible-light-active photocatalysts, were fabricated by successive decoration of Fe3O4, Ag2WO4, and AgBr over g-C3N4 (gCN) and they were characterized by XRD, EDX, SEM, TEM, HRTEM, UV–vis DRS, FT-IR, PL, TG, and VSM analysis. Visible-light-induced photocatalytic performances were studied by degradations of RhB, MB, MO, and fuchsine pollutants. It was confirmed that the nanocomposites are effective in the reduction of e−/h+ recombination through the matched interactions between energy bands of gCN, Fe3O4, Ag2WO4, and AgBr semiconductors. The highest photocatalytic degradation efficiency was observed for the gCN/M/AgW/AgBr (30%) nanocomposite when it was refluxed for 30 min. Activity of this nanocomposite is almost 21, 41, 94, and 10-folds greater than those of the gCN toward the degradations of RhB, MB, MO, and fuchsine pollutants, respectively. Additionally, a mechanism for the superior photocatalytic performances was proposed using reactive species scavenging experiments and characterization results. |
| Author | Habibi-Yangjeh, Aziz Mousavi, Mitra |
| Author_xml | – sequence: 1 givenname: Mitra surname: Mousavi fullname: Mousavi, Mitra – sequence: 2 givenname: Aziz surname: Habibi-Yangjeh fullname: Habibi-Yangjeh, Aziz email: ahabibi@uma.ac.ir |
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| Keywords | g-C3N4-based photocatalysts g-C3N4/Fe3O4/Ag2WO4/AgBr Magnetic nanocomposites Heterojunction |
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•Magnetically recoverable g-C3N4/Fe3O4/Ag2WO4/AgBr photocatalyst is reported.•g-C3N4/Fe3O4/Ag2WO4/AgBr (30%) nanocomposite exhibited the... |
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| Title | Magnetically recoverable highly efficient visible-light-active g-C3N4/Fe3O4/Ag2WO4/AgBr nanocomposites for photocatalytic degradations of environmental pollutants |
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