Novel nanowire self-assembled hierarchical CeO2 microspheres for low temperature toluene catalytic combustion
[Display omitted] •The hierarchical microsphere CeO2 (CeO2-HS) is prepared.•The CeO2-HS is self-assembled by many ceria nanowires.•The CeO2-HS exhibits the outstanding activity toward toluene catalytic oxidation.•Surface oxygen vacancies control the reaction rate. The catalytic oxidation of toluene...
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| Published in | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 331; pp. 425 - 434 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.01.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•The hierarchical microsphere CeO2 (CeO2-HS) is prepared.•The CeO2-HS is self-assembled by many ceria nanowires.•The CeO2-HS exhibits the outstanding activity toward toluene catalytic oxidation.•Surface oxygen vacancies control the reaction rate.
The catalytic oxidation of toluene has been investigated over pure CeO2 hierarchical catalyst for the first time. The novel CeO2 catalyst was prepared by a hydrothermal-driven assembly method. The structure of CeO2 catalyst was consisted of nanowire self-assembled hierarchical microspheres. The new hierarchical CeO2 catalyst showed much better catalytic activity than analogous nonporous catalyst by traditional hydrothermal method. The hierarchical CeO2 catalyst could reach more than 90% toluene conversion even as low as 210°C (T90) under a high space velocity of 60,000mL/(g·h). The high catalytic activities could be attributed to the large surface areas, in addition, the hierarchical porous structures provide more contents of surface oxygen vacancies for the dissociation of gaseous O2 on the surface. |
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| AbstractList | [Display omitted]
•The hierarchical microsphere CeO2 (CeO2-HS) is prepared.•The CeO2-HS is self-assembled by many ceria nanowires.•The CeO2-HS exhibits the outstanding activity toward toluene catalytic oxidation.•Surface oxygen vacancies control the reaction rate.
The catalytic oxidation of toluene has been investigated over pure CeO2 hierarchical catalyst for the first time. The novel CeO2 catalyst was prepared by a hydrothermal-driven assembly method. The structure of CeO2 catalyst was consisted of nanowire self-assembled hierarchical microspheres. The new hierarchical CeO2 catalyst showed much better catalytic activity than analogous nonporous catalyst by traditional hydrothermal method. The hierarchical CeO2 catalyst could reach more than 90% toluene conversion even as low as 210°C (T90) under a high space velocity of 60,000mL/(g·h). The high catalytic activities could be attributed to the large surface areas, in addition, the hierarchical porous structures provide more contents of surface oxygen vacancies for the dissociation of gaseous O2 on the surface. |
| Author | Hu, Fangyun Chen, Jianjun Peng, Yue Li, Kezhi Song, Hua Li, Junhua |
| Author_xml | – sequence: 1 givenname: Fangyun surname: Hu fullname: Hu, Fangyun organization: School of Environment, Tsinghua University, Beijing 100084, China – sequence: 2 givenname: Jianjun surname: Chen fullname: Chen, Jianjun email: chenjianjun@tsinghua.edu.cn organization: School of Environment, Tsinghua University, Beijing 100084, China – sequence: 3 givenname: Yue surname: Peng fullname: Peng, Yue organization: School of Environment, Tsinghua University, Beijing 100084, China – sequence: 4 givenname: Hua surname: Song fullname: Song, Hua organization: School of Environment, Tsinghua University, Beijing 100084, China – sequence: 5 givenname: Kezhi surname: Li fullname: Li, Kezhi organization: School of Environment, Tsinghua University, Beijing 100084, China – sequence: 6 givenname: Junhua orcidid: 0000-0003-3630-8712 surname: Li fullname: Li, Junhua email: lijunhua@tsinghua.edu.cn organization: School of Environment, Tsinghua University, Beijing 100084, China |
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•The hierarchical microsphere CeO2 (CeO2-HS) is prepared.•The CeO2-HS is self-assembled by many ceria nanowires.•The CeO2-HS exhibits the... |
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| SubjectTerms | CeO2 Hierarchical structure Surface oxygen vacancies Toluene catalytic combustion |
| Title | Novel nanowire self-assembled hierarchical CeO2 microspheres for low temperature toluene catalytic combustion |
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