Anchoring Co3O4 nanoparticles on MXene for efficient electrocatalytic oxygen evolution
[Display omitted] Rational design and controllable synthesis of efficient electrocatalysts for water oxidation is of significant importance for the development of promising energy conversion systems, in particular integrated photoelectrochemical water splitting devices. Cobalt oxide (Co3O4) nanostru...
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| Published in | Science bulletin (Beijing) Vol. 65; no. 6; pp. 460 - 466 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
30.03.2020
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
Rational design and controllable synthesis of efficient electrocatalysts for water oxidation is of significant importance for the development of promising energy conversion systems, in particular integrated photoelectrochemical water splitting devices. Cobalt oxide (Co3O4) nanostructures with mixed valences (II,III) have been regarded as promising electrocatalysts for the oxygen evolution reaction (OER). They are able to promote catalytic support of OER but with only modest activity. Here, we demonstrate that the OER performance of cubic Co3O4 electrocatalyst is obviously improved when they are anchored on delaminated two-dimensional (2D) Ti3C2 MXene nanosheets. Upon activation the overpotential of the hybrid catalyst delivers 300 mV at a current density of 10 mA cm−2 in basic solutions, which is remarkably lower than those of Ti3C2 MXene and Co3O4 nanocubes. The strong interfacial electrostatic interactions between two components contribute to the exceptional catalytic performance and stability. The enhanced OER activity and facile synthesis make these Co3O4 nanocubes-decorated ultrathin 2D Ti3C2 MXene nanosheets useful for constructing efficient and stable electrodes for high-performance electrochemical water splitting. |
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| AbstractList | [Display omitted]
Rational design and controllable synthesis of efficient electrocatalysts for water oxidation is of significant importance for the development of promising energy conversion systems, in particular integrated photoelectrochemical water splitting devices. Cobalt oxide (Co3O4) nanostructures with mixed valences (II,III) have been regarded as promising electrocatalysts for the oxygen evolution reaction (OER). They are able to promote catalytic support of OER but with only modest activity. Here, we demonstrate that the OER performance of cubic Co3O4 electrocatalyst is obviously improved when they are anchored on delaminated two-dimensional (2D) Ti3C2 MXene nanosheets. Upon activation the overpotential of the hybrid catalyst delivers 300 mV at a current density of 10 mA cm−2 in basic solutions, which is remarkably lower than those of Ti3C2 MXene and Co3O4 nanocubes. The strong interfacial electrostatic interactions between two components contribute to the exceptional catalytic performance and stability. The enhanced OER activity and facile synthesis make these Co3O4 nanocubes-decorated ultrathin 2D Ti3C2 MXene nanosheets useful for constructing efficient and stable electrodes for high-performance electrochemical water splitting. |
| Author | Lu, Yi Cao, Cancan Xiao, Weiping Yang, Xiaofei Fan, Deqi Chen, Zupeng |
| Author_xml | – sequence: 1 givenname: Yi surname: Lu fullname: Lu, Yi organization: Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, College of Science, Nanjing Forestry University, Nanjing 210037, China – sequence: 2 givenname: Deqi surname: Fan fullname: Fan, Deqi organization: Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, College of Science, Nanjing Forestry University, Nanjing 210037, China – sequence: 3 givenname: Zupeng surname: Chen fullname: Chen, Zupeng organization: Institute for Chemical and Bioengineering, Department of Chemistry and Applied Biosciences, ETH Zürich, CH-8093 Zürich, Switzerland – sequence: 4 givenname: Weiping surname: Xiao fullname: Xiao, Weiping email: wpxiao@njfu.edu.cn organization: Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, College of Science, Nanjing Forestry University, Nanjing 210037, China – sequence: 5 givenname: Cancan surname: Cao fullname: Cao, Cancan organization: Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, College of Science, Nanjing Forestry University, Nanjing 210037, China – sequence: 6 givenname: Xiaofei surname: Yang fullname: Yang, Xiaofei email: xiaofei.yang@njfu.edu.cn organization: Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, College of Science, Nanjing Forestry University, Nanjing 210037, China |
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| Keywords | Heterojunctions Electrocatalysis Water splitting Oxygen evolution reaction MXene Co3O4 |
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| Title | Anchoring Co3O4 nanoparticles on MXene for efficient electrocatalytic oxygen evolution |
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