A global optimization study on the devolatilisation kinetics of coal, biomass and waste fuels

Kinetic modeling of the pyrolysis of coal, biomass and waste fuels is presented using a power-law model in terms of multiple parallel reactions. The behaviour of the overall conversion rate of the pyrolysis products is derived from the summation of each reaction's conversion rate, while the exp...

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Published inFuel processing technology Vol. 90; no. 6; pp. 762 - 769
Main Authors Pantoleontos, G., Basinas, P., Skodras, G., Grammelis, P., Pintér, J.D., Topis, S., Sakellaropoulos, G.P.
Format Journal Article
LanguageEnglish
Published Amsterdam Elsevier B.V 01.06.2009
Elsevier
Subjects
Applied sciences
Combustion of heterogeneous mixtures. Incineration
Combustion. Flame
Energy
Energy. Thermal use of fuels
Exact sciences and technology
Exponential integral
Global Optimization Toolbox for Maple
Kinetic modeling
Pyrolysis
Theoretical studies. Data and constants. Metering
Pyrolysis
Global Optimization Toolbox for Maple
Kinetic modeling
Exponential integral
Conversion rate
Thermogravimetry
Biomass
Reaction rate
Modeling
Optimization
Combustible waste
Coal
Kinetics
Comparative study
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Abstract Kinetic modeling of the pyrolysis of coal, biomass and waste fuels is presented using a power-law model in terms of multiple parallel reactions. The behaviour of the overall conversion rate of the pyrolysis products is derived from the summation of each reaction's conversion rate, while the exponential integral for the computation of individual conversion is evaluated by Hastings rational approximation. Global optimization techniques and the Global Optimization Toolbox for Maple were used in order to minimize globally the sum of squares of errors. Comparison with literature results derived using local scope search methods supports the assumption that the problem is non-convex, thus necessitating the use of global optimization, which leads to a very good agreement between the computational and experimental values of the overall conversion rate vs. temperature derived from a non-isothermal thermogravimetric analyzer.
AbstractList Kinetic modeling of the pyrolysis of coal, biomass and waste fuels is presented using a power-law model in terms of multiple parallel reactions. The behaviour of the overall conversion rate of the pyrolysis products is derived from the summation of each reaction's conversion rate, while the exponential integral for the computation of individual conversion is evaluated by Hastings rational approximation. Global optimization techniques and the Global Optimization Toolbox for Maple were used in order to minimize globally the sum of squares of errors. Comparison with literature results derived using local scope search methods supports the assumption that the problem is non-convex, thus necessitating the use of global optimization, which leads to a very good agreement between the computational and experimental values of the overall conversion rate vs. temperature derived from a non-isothermal thermogravimetric analyzer.
Author Pantoleontos, G.
Basinas, P.
Topis, S.
Grammelis, P.
Sakellaropoulos, G.P.
Skodras, G.
Pintér, J.D.
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Issue 6
Keywords Pyrolysis
Global Optimization Toolbox for Maple
Kinetic modeling
Exponential integral
Conversion rate
Thermogravimetry
Biomass
Reaction rate
Modeling
Optimization
Combustible waste
Coal
Kinetics
Comparative study
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Snippet Kinetic modeling of the pyrolysis of coal, biomass and waste fuels is presented using a power-law model in terms of multiple parallel reactions. The behaviour...
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SubjectTerms Applied sciences
Combustion of heterogeneous mixtures. Incineration
Combustion. Flame
Energy
Energy. Thermal use of fuels
Exact sciences and technology
Exponential integral
Global Optimization Toolbox for Maple
Kinetic modeling
Pyrolysis
Theoretical studies. Data and constants. Metering
Title A global optimization study on the devolatilisation kinetics of coal, biomass and waste fuels
URI https://dx.doi.org/10.1016/j.fuproc.2009.03.011
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