Aging mechanism of microplastics with UV irradiation and its effects on the adsorption of heavy metals
[Display omitted] •PS were aged by air, pure water and seawater under UV irradiation.•Changes in chemical/physical properties of PS were examined by FTIR, XPS, XRD and SEM.•Aging mechanisms of PS in water environment is different from that in air.•Aging can significantly improve the adsorption of he...
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| Published in | Journal of hazardous materials Vol. 393; p. 122515 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Netherlands
Elsevier B.V
05.07.2020
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•PS were aged by air, pure water and seawater under UV irradiation.•Changes in chemical/physical properties of PS were examined by FTIR, XPS, XRD and SEM.•Aging mechanisms of PS in water environment is different from that in air.•Aging can significantly improve the adsorption of heavy metals by PS.
Microplastics are formed by the degradation of plastic wastes under the action of physicochemical mechanisms in environment, and they are becoming a new type of pollutant that is attractings global attention. However, research on the aging characteristics and mechanism of microplastics is limited. The aging mechanism of Polystyrene (PS) with UV irradiation under different conditions (air, pure water and seawater) and the effect of aging on heavy metal adsorption were studied. The results show that PS have different characteristics with UV irradiation under different conditions, and the aging of PS is the most obvious in air. Based on the 2D-COS analysis, different aging mechanisms were identified under different aging conditions, aging sequence of aged PS functional groups in air and water were clearly definited. An isothermal adsorption model shows that aging can significantly increase the adsorption of heavy metals by PS. The adsorption of heavy metals is also affected by different aging methods. Over all, a 2D-COS analysis was an effective method for understanding the aging process of PS. These results further clarify the aging mechanism of PS, and provides a theoretical basis for the assessment of environmental behavior and ecological risk when microplastics and heavy metals coexist. |
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| AbstractList | Microplastics are formed by the degradation of plastic wastes under the action of physicochemical mechanisms in environment, and they are becoming a new type of pollutant that is attractings global attention. However, research on the aging characteristics and mechanism of microplastics is limited. The aging mechanism of Polystyrene (PS) with UV irradiation under different conditions (air, pure water and seawater) and the effect of aging on heavy metal adsorption were studied. The results show that PS have different characteristics with UV irradiation under different conditions, and the aging of PS is the most obvious in air. Based on the 2D-COS analysis, different aging mechanisms were identified under different aging conditions, aging sequence of aged PS functional groups in air and water were clearly definited. An isothermal adsorption model shows that aging can significantly increase the adsorption of heavy metals by PS. The adsorption of heavy metals is also affected by different aging methods. Over all, a 2D-COS analysis was an effective method for understanding the aging process of PS. These results further clarify the aging mechanism of PS, and provides a theoretical basis for the assessment of environmental behavior and ecological risk when microplastics and heavy metals coexist. [Display omitted] •PS were aged by air, pure water and seawater under UV irradiation.•Changes in chemical/physical properties of PS were examined by FTIR, XPS, XRD and SEM.•Aging mechanisms of PS in water environment is different from that in air.•Aging can significantly improve the adsorption of heavy metals by PS. Microplastics are formed by the degradation of plastic wastes under the action of physicochemical mechanisms in environment, and they are becoming a new type of pollutant that is attractings global attention. However, research on the aging characteristics and mechanism of microplastics is limited. The aging mechanism of Polystyrene (PS) with UV irradiation under different conditions (air, pure water and seawater) and the effect of aging on heavy metal adsorption were studied. The results show that PS have different characteristics with UV irradiation under different conditions, and the aging of PS is the most obvious in air. Based on the 2D-COS analysis, different aging mechanisms were identified under different aging conditions, aging sequence of aged PS functional groups in air and water were clearly definited. An isothermal adsorption model shows that aging can significantly increase the adsorption of heavy metals by PS. The adsorption of heavy metals is also affected by different aging methods. Over all, a 2D-COS analysis was an effective method for understanding the aging process of PS. These results further clarify the aging mechanism of PS, and provides a theoretical basis for the assessment of environmental behavior and ecological risk when microplastics and heavy metals coexist. Microplastics are formed by the degradation of plastic wastes under the action of physicochemical mechanisms in environment, and they are becoming a new type of pollutant that is attractings global attention. However, research on the aging characteristics and mechanism of microplastics is limited. The aging mechanism of Polystyrene (PS) with UV irradiation under different conditions (air, pure water and seawater) and the effect of aging on heavy metal adsorption were studied. The results show that PS have different characteristics with UV irradiation under different conditions, and the aging of PS is the most obvious in air. Based on the 2D-COS analysis, different aging mechanisms were identified under different aging conditions, aging sequence of aged PS functional groups in air and water were clearly definited. An isothermal adsorption model shows that aging can significantly increase the adsorption of heavy metals by PS. The adsorption of heavy metals is also affected by different aging methods. Over all, a 2D-COS analysis was an effective method for understanding the aging process of PS. These results further clarify the aging mechanism of PS, and provides a theoretical basis for the assessment of environmental behavior and ecological risk when microplastics and heavy metals coexist.Microplastics are formed by the degradation of plastic wastes under the action of physicochemical mechanisms in environment, and they are becoming a new type of pollutant that is attractings global attention. However, research on the aging characteristics and mechanism of microplastics is limited. The aging mechanism of Polystyrene (PS) with UV irradiation under different conditions (air, pure water and seawater) and the effect of aging on heavy metal adsorption were studied. The results show that PS have different characteristics with UV irradiation under different conditions, and the aging of PS is the most obvious in air. Based on the 2D-COS analysis, different aging mechanisms were identified under different aging conditions, aging sequence of aged PS functional groups in air and water were clearly definited. An isothermal adsorption model shows that aging can significantly increase the adsorption of heavy metals by PS. The adsorption of heavy metals is also affected by different aging methods. Over all, a 2D-COS analysis was an effective method for understanding the aging process of PS. These results further clarify the aging mechanism of PS, and provides a theoretical basis for the assessment of environmental behavior and ecological risk when microplastics and heavy metals coexist. |
| ArticleNumber | 122515 |
| Author | Yu, Xiaoqin Mao, Ruofan Wu, Renren Yang, Xiaomei Lang, Mengfan Guo, Xuetao |
| Author_xml | – sequence: 1 givenname: Ruofan surname: Mao fullname: Mao, Ruofan organization: College of Natural Resources and Environment, Northwest A&F University, Yangling, Shaanxi, 712100, China – sequence: 2 givenname: Mengfan surname: Lang fullname: Lang, Mengfan organization: College of Natural Resources and Environment, Northwest A&F University, Yangling, Shaanxi, 712100, China – sequence: 3 givenname: Xiaoqin surname: Yu fullname: Yu, Xiaoqin organization: College of Natural Resources and Environment, Northwest A&F University, Yangling, Shaanxi, 712100, China – sequence: 4 givenname: Renren surname: Wu fullname: Wu, Renren email: wurenren@scies.org organization: State Environmental Protection Key Laboratory of Water Environmental Simulation and Pollution Control, South China Institute of Environmental Sciences, MEE, Guangzhou 510655, PR China – sequence: 5 givenname: Xiaomei surname: Yang fullname: Yang, Xiaomei organization: College of Natural Resources and Environment, Northwest A&F University, Yangling, Shaanxi, 712100, China – sequence: 6 givenname: Xuetao surname: Guo fullname: Guo, Xuetao email: guoxuetao2005@nwafu.edu.cn organization: College of Natural Resources and Environment, Northwest A&F University, Yangling, Shaanxi, 712100, China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32197203$$D View this record in MEDLINE/PubMed |
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| Copyright | 2020 Elsevier B.V. Copyright © 2020 Elsevier B.V. All rights reserved. |
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| Keywords | Microplastics UV irradiation 2D-COS Adsorption Heavy metal |
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•PS were aged by air, pure water and seawater under UV irradiation.•Changes in chemical/physical properties of PS were examined by FTIR, XPS,... Microplastics are formed by the degradation of plastic wastes under the action of physicochemical mechanisms in environment, and they are becoming a new type... |
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| SubjectTerms | 2D-COS Adsorption Heavy metal heavy metals Microplastics moieties pollutants polystyrenes risk seawater ultraviolet radiation UV irradiation wastes |
| Title | Aging mechanism of microplastics with UV irradiation and its effects on the adsorption of heavy metals |
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