Improving urban drainage systems to mitigate PPCPs pollution in surface water: A watershed perspective

Parabens are preservatives widely used in pharmaceutical and personal care products (PPCPs). This study investigated urban water pollution by parabens from a watershed perspective. Water and sediment samples were collected from one of the most polluted urban streams in China. Six parabens and five p...

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Published inJournal of hazardous materials Vol. 411; p. 125047
Main Authors Zhao, Xue, Zheng, Yi, Hu, Shiyao, Qiu, Wenhui, Jiang, Jiping, Gao, Chuanzi, Xiong, Jianzhi, Lu, Haiyan, Quan, Feng
Format Journal Article
LanguageEnglish
Published Netherlands Elsevier B.V 05.06.2021
Subjects
China
Combined sewage overflows
drainage
Drainage system
dry season
metabolites
Parabens
PPCPs
rain
rivers
sediments
sewage
stormwater
surface water
Urban river
wastewater treatment
water pollution
watersheds
wet season
China
Drainage system
PPCPs
Combined sewage overflows
Urban river
Parabens
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Abstract Parabens are preservatives widely used in pharmaceutical and personal care products (PPCPs). This study investigated urban water pollution by parabens from a watershed perspective. Water and sediment samples were collected from one of the most polluted urban streams in China. Six parabens and five paraben metabolites were frequently detected in the samples, whereas the overall pollution level was intermediate according to a global comparison. The spatial distributions of the chemical concentrations along the river are influenced by multiple factors, and WWTPs appear to be a major factor. In general, the target pollutants were detected at higher concentrations in the dry season than in the wet season, but extraordinary concentration peaks in water were observed downstream of wastewater treatment plants (WWTPs), indicating a dominant contribution from combined sewage overflows (CSOs) during rainfall events. In a representative WWTP-influenced reach, CSOs account for its 97.3% of ∑parabens input and 96.9% of ∑metabolites input in a typical rainfall event. Converting the existing combined sewer systems to separate stormwater drainage systems could reduce the inputs of ∑parabens and ∑metabolites by 86.9–84.5%, respectively. This study highlights the role of urban drainage systems in preventing surface water pollution by PPCPs. Urban drainage systems play a critical role in controlling pollution by parabens and their metabolites in urban surface water. [Display omitted] •Transport of parabens in urban surface water was investigated at a watershed scale.•The occurrence of five paraben metabolites in Chinese rivers was first reported.•CSOs contributed over 95% of the chemicals input to the river in the rainfall event.•The new drainage systems avoid CSOs and may reduce over 80% of the chemicals input.
AbstractList Parabens are preservatives widely used in pharmaceutical and personal care products (PPCPs). This study investigated urban water pollution by parabens from a watershed perspective. Water and sediment samples were collected from one of the most polluted urban streams in China. Six parabens and five paraben metabolites were frequently detected in the samples, whereas the overall pollution level was intermediate according to a global comparison. The spatial distributions of the chemical concentrations along the river are influenced by multiple factors, and WWTPs appear to be a major factor. In general, the target pollutants were detected at higher concentrations in the dry season than in the wet season, but extraordinary concentration peaks in water were observed downstream of wastewater treatment plants (WWTPs), indicating a dominant contribution from combined sewage overflows (CSOs) during rainfall events. In a representative WWTP-influenced reach, CSOs account for its 97.3% of ∑parabens input and 96.9% of ∑metabolites input in a typical rainfall event. Converting the existing combined sewer systems to separate stormwater drainage systems could reduce the inputs of ∑parabens and ∑metabolites by 86.9–84.5%, respectively. This study highlights the role of urban drainage systems in preventing surface water pollution by PPCPs.Urban drainage systems play a critical role in controlling pollution by parabens and their metabolites in urban surface water.
Parabens are preservatives widely used in pharmaceutical and personal care products (PPCPs). This study investigated urban water pollution by parabens from a watershed perspective. Water and sediment samples were collected from one of the most polluted urban streams in China. Six parabens and five paraben metabolites were frequently detected in the samples, whereas the overall pollution level was intermediate according to a global comparison. The spatial distributions of the chemical concentrations along the river are influenced by multiple factors, and WWTPs appear to be a major factor. In general, the target pollutants were detected at higher concentrations in the dry season than in the wet season, but extraordinary concentration peaks in water were observed downstream of wastewater treatment plants (WWTPs), indicating a dominant contribution from combined sewage overflows (CSOs) during rainfall events. In a representative WWTP-influenced reach, CSOs account for its 97.3% of ∑parabens input and 96.9% of ∑metabolites input in a typical rainfall event. Converting the existing combined sewer systems to separate stormwater drainage systems could reduce the inputs of ∑parabens and ∑metabolites by 86.9–84.5%, respectively. This study highlights the role of urban drainage systems in preventing surface water pollution by PPCPs. Urban drainage systems play a critical role in controlling pollution by parabens and their metabolites in urban surface water. [Display omitted] •Transport of parabens in urban surface water was investigated at a watershed scale.•The occurrence of five paraben metabolites in Chinese rivers was first reported.•CSOs contributed over 95% of the chemicals input to the river in the rainfall event.•The new drainage systems avoid CSOs and may reduce over 80% of the chemicals input.
Parabens are preservatives widely used in pharmaceutical and personal care products (PPCPs). This study investigated urban water pollution by parabens from a watershed perspective. Water and sediment samples were collected from one of the most polluted urban streams in China. Six parabens and five paraben metabolites were frequently detected in the samples, whereas the overall pollution level was intermediate according to a global comparison. The spatial distributions of the chemical concentrations along the river are influenced by multiple factors, and WWTPs appear to be a major factor. In general, the target pollutants were detected at higher concentrations in the dry season than in the wet season, but extraordinary concentration peaks in water were observed downstream of wastewater treatment plants (WWTPs), indicating a dominant contribution from combined sewage overflows (CSOs) during rainfall events. In a representative WWTP-influenced reach, CSOs account for its 97.3% of ∑parabens input and 96.9% of ∑metabolites input in a typical rainfall event. Converting the existing combined sewer systems to separate stormwater drainage systems could reduce the inputs of ∑parabens and ∑metabolites by 86.9-84.5%, respectively. This study highlights the role of urban drainage systems in preventing surface water pollution by PPCPs. CAPSULE: Urban drainage systems play a critical role in controlling pollution by parabens and their metabolites in urban surface water.Parabens are preservatives widely used in pharmaceutical and personal care products (PPCPs). This study investigated urban water pollution by parabens from a watershed perspective. Water and sediment samples were collected from one of the most polluted urban streams in China. Six parabens and five paraben metabolites were frequently detected in the samples, whereas the overall pollution level was intermediate according to a global comparison. The spatial distributions of the chemical concentrations along the river are influenced by multiple factors, and WWTPs appear to be a major factor. In general, the target pollutants were detected at higher concentrations in the dry season than in the wet season, but extraordinary concentration peaks in water were observed downstream of wastewater treatment plants (WWTPs), indicating a dominant contribution from combined sewage overflows (CSOs) during rainfall events. In a representative WWTP-influenced reach, CSOs account for its 97.3% of ∑parabens input and 96.9% of ∑metabolites input in a typical rainfall event. Converting the existing combined sewer systems to separate stormwater drainage systems could reduce the inputs of ∑parabens and ∑metabolites by 86.9-84.5%, respectively. This study highlights the role of urban drainage systems in preventing surface water pollution by PPCPs. CAPSULE: Urban drainage systems play a critical role in controlling pollution by parabens and their metabolites in urban surface water.
Parabens are preservatives widely used in pharmaceutical and personal care products (PPCPs). This study investigated urban water pollution by parabens from a watershed perspective. Water and sediment samples were collected from one of the most polluted urban streams in China. Six parabens and five paraben metabolites were frequently detected in the samples, whereas the overall pollution level was intermediate according to a global comparison. The spatial distributions of the chemical concentrations along the river are influenced by multiple factors, and WWTPs appear to be a major factor. In general, the target pollutants were detected at higher concentrations in the dry season than in the wet season, but extraordinary concentration peaks in water were observed downstream of wastewater treatment plants (WWTPs), indicating a dominant contribution from combined sewage overflows (CSOs) during rainfall events. In a representative WWTP-influenced reach, CSOs account for its 97.3% of ∑parabens input and 96.9% of ∑metabolites input in a typical rainfall event. Converting the existing combined sewer systems to separate stormwater drainage systems could reduce the inputs of ∑parabens and ∑metabolites by 86.9-84.5%, respectively. This study highlights the role of urban drainage systems in preventing surface water pollution by PPCPs. CAPSULE: Urban drainage systems play a critical role in controlling pollution by parabens and their metabolites in urban surface water.
ArticleNumber 125047
Author Quan, Feng
Hu, Shiyao
Zhao, Xue
Xiong, Jianzhi
Gao, Chuanzi
Zheng, Yi
Lu, Haiyan
Jiang, Jiping
Qiu, Wenhui
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Keywords Drainage system
PPCPs
Combined sewage overflows
Urban river
Parabens
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Snippet Parabens are preservatives widely used in pharmaceutical and personal care products (PPCPs). This study investigated urban water pollution by parabens from a...
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SubjectTerms China
Combined sewage overflows
drainage
Drainage system
dry season
metabolites
Parabens
PPCPs
rain
rivers
sediments
sewage
stormwater
surface water
Urban river
wastewater treatment
water pollution
watersheds
wet season
Title Improving urban drainage systems to mitigate PPCPs pollution in surface water: A watershed perspective
URI https://dx.doi.org/10.1016/j.jhazmat.2021.125047
https://www.ncbi.nlm.nih.gov/pubmed/33453662
https://www.proquest.com/docview/2478597704
https://www.proquest.com/docview/2524276768
Volume 411
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