An imperative approach for fluorosis mitigation: Amending aqueous calcium to suppress hydroxyapatite dissolution in defluoridation
Drinking of fluoride (F−) contaminated water causes fluorosis and thus providing safe drinking water to the affected community remains a major challenge. Therefore, defluoridation without disturbing water quality is imperative. Hydroxyapatite (HAP) is proved to have a potential application for deflu...
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| Published in | Journal of environmental management Vol. 245; pp. 230 - 237 |
|---|---|
| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier Ltd
01.09.2019
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Drinking of fluoride (F−) contaminated water causes fluorosis and thus providing safe drinking water to the affected community remains a major challenge. Therefore, defluoridation without disturbing water quality is imperative. Hydroxyapatite (HAP) is proved to have a potential application for defluoridation; however, its dissolution during defluoridation is a concern for its implementation. Experiments conducted by suspending HAP in F− solution and deionized water without F− show that former had high residual pH and PO43− than the latter with Ca2+ being absent in the former. This indicates that Ca2+ had participated in defluoridation and promoted HAP dissolution when Ca2+ was unavailable. Hence, HAP dissolution seems to be a governing step for defluoridation. However, higher residual PO43− and pH affect drinking water quality, and its usage may pose additional health problems. Thus, Ca2+ deficient defluoridated water is unfit for drinking unless it is treated further. Hence, the present work proposes a novel method to overcome HAP dissolution by amending aqueous Ca2+ to F− water. The results show that amending Ca2+ efficiently prevents HAP dissolution and enhances defluoridation capacity as an added feature. Furthermore, speciation using MINEQL+ and FTIR of fluoride-calcium treated HAPs suggest the possibility of defluoridation by aqueous CaF+ adsorption onto HAP besides F− ion exchange with OH−.
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•HAP dissolution in defluoridation makes the treated water unfit for drinking.•Amending aqueous Ca2+ to F− water suppressed the HAP dissolution in defluoridation.•Aqueous Ca2+ amendment to F−-water provides Ca2+-enriched alkaline drinking-water.•Amending aqueous Ca2+ showed enhanced defluoridation capacity for HAP.•Deflouridation occurred by adsorption of aqueous CaF+ and ion-exchange. |
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| AbstractList | Drinking of fluoride (F−) contaminated water causes fluorosis and thus providing safe drinking water to the affected community remains a major challenge. Therefore, defluoridation without disturbing water quality is imperative. Hydroxyapatite (HAP) is proved to have a potential application for defluoridation; however, its dissolution during defluoridation is a concern for its implementation. Experiments conducted by suspending HAP in F− solution and deionized water without F− show that former had high residual pH and PO43− than the latter with Ca2+ being absent in the former. This indicates that Ca2+ had participated in defluoridation and promoted HAP dissolution when Ca2+ was unavailable. Hence, HAP dissolution seems to be a governing step for defluoridation. However, higher residual PO43− and pH affect drinking water quality, and its usage may pose additional health problems. Thus, Ca2+ deficient defluoridated water is unfit for drinking unless it is treated further. Hence, the present work proposes a novel method to overcome HAP dissolution by amending aqueous Ca2+ to F− water. The results show that amending Ca2+ efficiently prevents HAP dissolution and enhances defluoridation capacity as an added feature. Furthermore, speciation using MINEQL+ and FTIR of fluoride-calcium treated HAPs suggest the possibility of defluoridation by aqueous CaF+ adsorption onto HAP besides F− ion exchange with OH−.
[Display omitted]
•HAP dissolution in defluoridation makes the treated water unfit for drinking.•Amending aqueous Ca2+ to F− water suppressed the HAP dissolution in defluoridation.•Aqueous Ca2+ amendment to F−-water provides Ca2+-enriched alkaline drinking-water.•Amending aqueous Ca2+ showed enhanced defluoridation capacity for HAP.•Deflouridation occurred by adsorption of aqueous CaF+ and ion-exchange. Drinking of fluoride (F-) contaminated water causes fluorosis and thus providing safe drinking water to the affected community remains a major challenge. Therefore, defluoridation without disturbing water quality is imperative. Hydroxyapatite (HAP) is proved to have a potential application for defluoridation; however, its dissolution during defluoridation is a concern for its implementation. Experiments conducted by suspending HAP in F- solution and deionized water without F- show that former had high residual pH and PO43- than the latter with Ca2+ being absent in the former. This indicates that Ca2+ had participated in defluoridation and promoted HAP dissolution when Ca2+ was unavailable. Hence, HAP dissolution seems to be a governing step for defluoridation. However, higher residual PO43- and pH affect drinking water quality, and its usage may pose additional health problems. Thus, Ca2+ deficient defluoridated water is unfit for drinking unless it is treated further. Hence, the present work proposes a novel method to overcome HAP dissolution by amending aqueous Ca2+ to F- water. The results show that amending Ca2+ efficiently prevents HAP dissolution and enhances defluoridation capacity as an added feature. Furthermore, speciation using MINEQL+ and FTIR of fluoride-calcium treated HAPs suggest the possibility of defluoridation by aqueous CaF+ adsorption onto HAP besides F- ion exchange with OH-.Drinking of fluoride (F-) contaminated water causes fluorosis and thus providing safe drinking water to the affected community remains a major challenge. Therefore, defluoridation without disturbing water quality is imperative. Hydroxyapatite (HAP) is proved to have a potential application for defluoridation; however, its dissolution during defluoridation is a concern for its implementation. Experiments conducted by suspending HAP in F- solution and deionized water without F- show that former had high residual pH and PO43- than the latter with Ca2+ being absent in the former. This indicates that Ca2+ had participated in defluoridation and promoted HAP dissolution when Ca2+ was unavailable. Hence, HAP dissolution seems to be a governing step for defluoridation. However, higher residual PO43- and pH affect drinking water quality, and its usage may pose additional health problems. Thus, Ca2+ deficient defluoridated water is unfit for drinking unless it is treated further. Hence, the present work proposes a novel method to overcome HAP dissolution by amending aqueous Ca2+ to F- water. The results show that amending Ca2+ efficiently prevents HAP dissolution and enhances defluoridation capacity as an added feature. Furthermore, speciation using MINEQL+ and FTIR of fluoride-calcium treated HAPs suggest the possibility of defluoridation by aqueous CaF+ adsorption onto HAP besides F- ion exchange with OH-. Drinking of fluoride (F⁻) contaminated water causes fluorosis and thus providing safe drinking water to the affected community remains a major challenge. Therefore, defluoridation without disturbing water quality is imperative. Hydroxyapatite (HAP) is proved to have a potential application for defluoridation; however, its dissolution during defluoridation is a concern for its implementation. Experiments conducted by suspending HAP in F⁻ solution and deionized water without F⁻ show that former had high residual pH and PO43− than the latter with Ca²⁺ being absent in the former. This indicates that Ca²⁺ had participated in defluoridation and promoted HAP dissolution when Ca²⁺ was unavailable. Hence, HAP dissolution seems to be a governing step for defluoridation. However, higher residual PO43− and pH affect drinking water quality, and its usage may pose additional health problems. Thus, Ca²⁺ deficient defluoridated water is unfit for drinking unless it is treated further. Hence, the present work proposes a novel method to overcome HAP dissolution by amending aqueous Ca²⁺ to F⁻ water. The results show that amending Ca²⁺ efficiently prevents HAP dissolution and enhances defluoridation capacity as an added feature. Furthermore, speciation using MINEQL+ and FTIR of fluoride-calcium treated HAPs suggest the possibility of defluoridation by aqueous CaF⁺ adsorption onto HAP besides F⁻ ion exchange with OH⁻. Drinking of fluoride (F ) contaminated water causes fluorosis and thus providing safe drinking water to the affected community remains a major challenge. Therefore, defluoridation without disturbing water quality is imperative. Hydroxyapatite (HAP) is proved to have a potential application for defluoridation; however, its dissolution during defluoridation is a concern for its implementation. Experiments conducted by suspending HAP in F solution and deionized water without F show that former had high residual pH and PO than the latter with Ca being absent in the former. This indicates that Ca had participated in defluoridation and promoted HAP dissolution when Ca was unavailable. Hence, HAP dissolution seems to be a governing step for defluoridation. However, higher residual PO and pH affect drinking water quality, and its usage may pose additional health problems. Thus, Ca deficient defluoridated water is unfit for drinking unless it is treated further. Hence, the present work proposes a novel method to overcome HAP dissolution by amending aqueous Ca to F water. The results show that amending Ca efficiently prevents HAP dissolution and enhances defluoridation capacity as an added feature. Furthermore, speciation using MINEQL+ and FTIR of fluoride-calcium treated HAPs suggest the possibility of defluoridation by aqueous CaF adsorption onto HAP besides F ion exchange with OH . |
| Author | Chaudhari, Sanjeev Sankannavar, Ravi |
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| CitedBy_id | crossref_primary_10_1016_j_jece_2020_103704 crossref_primary_10_1016_j_jhazmat_2020_124694 crossref_primary_10_1016_j_seppur_2022_122497 crossref_primary_10_1016_j_jwpe_2023_103765 crossref_primary_10_3390_ma16093605 crossref_primary_10_1016_j_apgeochem_2022_105358 crossref_primary_10_1016_j_hazl_2021_100033 crossref_primary_10_1007_s43207_022_00225_w crossref_primary_10_1007_s11356_024_34452_x crossref_primary_10_1007_s12403_024_00625_9 crossref_primary_10_1016_j_reactfunctpolym_2021_105067 crossref_primary_10_17159_sajs_2024_12879 crossref_primary_10_1016_j_jenvman_2020_110415 crossref_primary_10_1016_j_envpol_2022_119882 crossref_primary_10_5004_dwt_2021_26814 |
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| Keywords | Calcium amendment Drinking water Hydroxyapatite dissolution Phosphate leaching Fluorosis reversal Fluoride removal |
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| Snippet | Drinking of fluoride (F−) contaminated water causes fluorosis and thus providing safe drinking water to the affected community remains a major challenge.... Drinking of fluoride (F ) contaminated water causes fluorosis and thus providing safe drinking water to the affected community remains a major challenge.... Drinking of fluoride (F-) contaminated water causes fluorosis and thus providing safe drinking water to the affected community remains a major challenge.... Drinking of fluoride (F⁻) contaminated water causes fluorosis and thus providing safe drinking water to the affected community remains a major challenge.... |
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| SubjectTerms | adsorption calcium Calcium amendment defluoridation drinking Drinking water Fluoride removal fluorides fluorosis Fluorosis reversal Fourier transform infrared spectroscopy hydroxyapatite Hydroxyapatite dissolution ion exchange Phosphate leaching water pollution water quality |
| Title | An imperative approach for fluorosis mitigation: Amending aqueous calcium to suppress hydroxyapatite dissolution in defluoridation |
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