Sodium alginate reinforced polyacrylamide/xanthan gum double network ionic hydrogels for stress sensing and self-powered wearable device applications

Strong and ductile sodium alginate (SA) reinforced polyacrylamide (PAM)/xanthan gum (XG) double network ionic hydrogels were constructed for stress sensing and self-powered wearable device applications. In the designed network of PXS-Mn+/LiCl (short for PAM/XG/SA-Mn+/LiCl, where Mn+ stands for Fe3+,...

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Published inCarbohydrate polymers Vol. 309; p. 120678
Main Authors Li, Tuo, Wei, Huige, Zhang, Yingying, Wan, Tong, Cui, Dapeng, Zhao, Shixiang, Zhang, Teng, Ji, Yanxiu, Algadi, Hassan, Guo, Zhanhu, Chu, Liqiang, Cheng, Bowen
Format Journal Article
LanguageEnglish
Published England Elsevier Ltd 01.06.2023
Subjects
batteries
capacitors
Double network
electrical conductivity
electronics
energy
hydrogels
hydrophilicity
Ionic hydrogel
Macromolecular reinforcing agent
mechanical stress
polyacrylamide
Self-powered
sodium alginate
Stress-sensing
tensile strength
Wearable electronics
xanthan gum
Stress-sensing
Self-powered
Wearable electronics
Ionic hydrogel
Macromolecular reinforcing agent
Double network
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Abstract Strong and ductile sodium alginate (SA) reinforced polyacrylamide (PAM)/xanthan gum (XG) double network ionic hydrogels were constructed for stress sensing and self-powered wearable device applications. In the designed network of PXS-Mn+/LiCl (short for PAM/XG/SA-Mn+/LiCl, where Mn+ stands for Fe3+, Cu2+ or Zn2+), PAM acts as a flexible hydrophilic skeleton, and XG functions as a ductile second network. The macromolecule SA interacts with metal ion Mn+ to form a unique complex structure, significantly improving the mechanical strength of the hydrogel. The addition of inorganic salt LiCl endows the hydrogel with high electrical conductivity, and meanwhile reduces the freezing point and prevents water loss of the hydrogel. PXS-Mn+/LiCl exhibits excellent mechanical properties and ultra-high ductility (a fracture tensile strength up to 0.65 MPa and a fracture strain up to 1800%), and high stress-sensing performance (a high GF up to 4.56 and pressure sensitivity of 0.122). Moreover, a self-powered device with a dual-power-supply mode, i.e., PXS-Mn+/LiCl-based primary battery and TENG, and a capacitor as the energy storage component was constructed, which shows promising prospects for self-powered wearable electronics. [Display omitted]
AbstractList Strong and ductile sodium alginate (SA) reinforced polyacrylamide (PAM)/xanthan gum (XG) double network ionic hydrogels were constructed for stress sensing and self-powered wearable device applications. In the designed network of PXS-M /LiCl (short for PAM/XG/SA-M /LiCl, where M stands for Fe , Cu or Zn ), PAM acts as a flexible hydrophilic skeleton, and XG functions as a ductile second network. The macromolecule SA interacts with metal ion M to form a unique complex structure, significantly improving the mechanical strength of the hydrogel. The addition of inorganic salt LiCl endows the hydrogel with high electrical conductivity, and meanwhile reduces the freezing point and prevents water loss of the hydrogel. PXS-M /LiCl exhibits excellent mechanical properties and ultra-high ductility (a fracture tensile strength up to 0.65 MPa and a fracture strain up to 1800%), and high stress-sensing performance (a high GF up to 4.56 and pressure sensitivity of 0.122). Moreover, a self-powered device with a dual-power-supply mode, i.e., PXS-M /LiCl-based primary battery and TENG, and a capacitor as the energy storage component was constructed, which shows promising prospects for self-powered wearable electronics.
Strong and ductile sodium alginate (SA) reinforced polyacrylamide (PAM)/xanthan gum (XG) double network ionic hydrogels were constructed for stress sensing and self-powered wearable device applications. In the designed network of PXS-Mⁿ⁺/LiCl (short for PAM/XG/SA-Mⁿ⁺/LiCl, where Mⁿ⁺ stands for Fe³⁺, Cu²⁺ or Zn²⁺), PAM acts as a flexible hydrophilic skeleton, and XG functions as a ductile second network. The macromolecule SA interacts with metal ion Mⁿ⁺ to form a unique complex structure, significantly improving the mechanical strength of the hydrogel. The addition of inorganic salt LiCl endows the hydrogel with high electrical conductivity, and meanwhile reduces the freezing point and prevents water loss of the hydrogel. PXS-Mⁿ⁺/LiCl exhibits excellent mechanical properties and ultra-high ductility (a fracture tensile strength up to 0.65 MPa and a fracture strain up to 1800%), and high stress-sensing performance (a high GF up to 4.56 and pressure sensitivity of 0.122). Moreover, a self-powered device with a dual-power-supply mode, i.e., PXS-Mⁿ⁺/LiCl-based primary battery and TENG, and a capacitor as the energy storage component was constructed, which shows promising prospects for self-powered wearable electronics.
Strong and ductile sodium alginate (SA) reinforced polyacrylamide (PAM)/xanthan gum (XG) double network ionic hydrogels were constructed for stress sensing and self-powered wearable device applications. In the designed network of PXS-Mn+/LiCl (short for PAM/XG/SA-Mn+/LiCl, where Mn+ stands for Fe3+, Cu2+ or Zn2+), PAM acts as a flexible hydrophilic skeleton, and XG functions as a ductile second network. The macromolecule SA interacts with metal ion Mn+ to form a unique complex structure, significantly improving the mechanical strength of the hydrogel. The addition of inorganic salt LiCl endows the hydrogel with high electrical conductivity, and meanwhile reduces the freezing point and prevents water loss of the hydrogel. PXS-Mn+/LiCl exhibits excellent mechanical properties and ultra-high ductility (a fracture tensile strength up to 0.65 MPa and a fracture strain up to 1800%), and high stress-sensing performance (a high GF up to 4.56 and pressure sensitivity of 0.122). Moreover, a self-powered device with a dual-power-supply mode, i.e., PXS-Mn+/LiCl-based primary battery and TENG, and a capacitor as the energy storage component was constructed, which shows promising prospects for self-powered wearable electronics. [Display omitted]
Strong and ductile sodium alginate (SA) reinforced polyacrylamide (PAM)/xanthan gum (XG) double network ionic hydrogels were constructed for stress sensing and self-powered wearable device applications. In the designed network of PXS-Mn+/LiCl (short for PAM/XG/SA-Mn+/LiCl, where Mn+ stands for Fe3+, Cu2+ or Zn2+), PAM acts as a flexible hydrophilic skeleton, and XG functions as a ductile second network. The macromolecule SA interacts with metal ion Mn+ to form a unique complex structure, significantly improving the mechanical strength of the hydrogel. The addition of inorganic salt LiCl endows the hydrogel with high electrical conductivity, and meanwhile reduces the freezing point and prevents water loss of the hydrogel. PXS-Mn+/LiCl exhibits excellent mechanical properties and ultra-high ductility (a fracture tensile strength up to 0.65 MPa and a fracture strain up to 1800%), and high stress-sensing performance (a high GF up to 4.56 and pressure sensitivity of 0.122). Moreover, a self-powered device with a dual-power-supply mode, i.e., PXS-Mn+/LiCl-based primary battery and TENG, and a capacitor as the energy storage component was constructed, which shows promising prospects for self-powered wearable electronics.Strong and ductile sodium alginate (SA) reinforced polyacrylamide (PAM)/xanthan gum (XG) double network ionic hydrogels were constructed for stress sensing and self-powered wearable device applications. In the designed network of PXS-Mn+/LiCl (short for PAM/XG/SA-Mn+/LiCl, where Mn+ stands for Fe3+, Cu2+ or Zn2+), PAM acts as a flexible hydrophilic skeleton, and XG functions as a ductile second network. The macromolecule SA interacts with metal ion Mn+ to form a unique complex structure, significantly improving the mechanical strength of the hydrogel. The addition of inorganic salt LiCl endows the hydrogel with high electrical conductivity, and meanwhile reduces the freezing point and prevents water loss of the hydrogel. PXS-Mn+/LiCl exhibits excellent mechanical properties and ultra-high ductility (a fracture tensile strength up to 0.65 MPa and a fracture strain up to 1800%), and high stress-sensing performance (a high GF up to 4.56 and pressure sensitivity of 0.122). Moreover, a self-powered device with a dual-power-supply mode, i.e., PXS-Mn+/LiCl-based primary battery and TENG, and a capacitor as the energy storage component was constructed, which shows promising prospects for self-powered wearable electronics.
ArticleNumber 120678
Author Wei, Huige
Ji, Yanxiu
Chu, Liqiang
Cheng, Bowen
Zhang, Teng
Zhao, Shixiang
Algadi, Hassan
Zhang, Yingying
Cui, Dapeng
Wan, Tong
Guo, Zhanhu
Li, Tuo
Author_xml – sequence: 1
  givenname: Tuo
  surname: Li
  fullname: Li, Tuo
  organization: Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-utilization, College of Chemical Engineering and Materials Science, Tianjin University of Science and Technology, Tianjin 300457, China
– sequence: 2
  givenname: Huige
  surname: Wei
  fullname: Wei, Huige
  email: huigewei@tust.edu.cn
  organization: Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-utilization, College of Chemical Engineering and Materials Science, Tianjin University of Science and Technology, Tianjin 300457, China
– sequence: 3
  givenname: Yingying
  surname: Zhang
  fullname: Zhang, Yingying
  organization: Tianjin Chest Hospital, Tianjin 300222, China
– sequence: 4
  givenname: Tong
  surname: Wan
  fullname: Wan, Tong
  organization: Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-utilization, College of Chemical Engineering and Materials Science, Tianjin University of Science and Technology, Tianjin 300457, China
– sequence: 5
  givenname: Dapeng
  surname: Cui
  fullname: Cui, Dapeng
  organization: College of Light Industry Science and Engineering, Tianjin University of Science and Technology, Tianjin 300457, China
– sequence: 6
  givenname: Shixiang
  surname: Zhao
  fullname: Zhao, Shixiang
  organization: College of Electronic Information and Automation, Tianjin University of Science and Technology, Tianjin 300222, China
– sequence: 7
  givenname: Teng
  surname: Zhang
  fullname: Zhang, Teng
  organization: College of Electronic Information and Automation, Tianjin University of Science and Technology, Tianjin 300222, China
– sequence: 8
  givenname: Yanxiu
  surname: Ji
  fullname: Ji, Yanxiu
  organization: Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-utilization, College of Chemical Engineering and Materials Science, Tianjin University of Science and Technology, Tianjin 300457, China
– sequence: 9
  givenname: Hassan
  surname: Algadi
  fullname: Algadi, Hassan
  organization: Department of Electrical Engineering, Faculty of Engineering, Najran University, Najran 11001, Saudi Arabia
– sequence: 10
  givenname: Zhanhu
  surname: Guo
  fullname: Guo, Zhanhu
  organization: Mechanical and Construction Engineering, Faculty of Engineering and Environment, Northumbria University, Newcastle Upon Tyne NE1 8ST, UK
– sequence: 11
  givenname: Liqiang
  surname: Chu
  fullname: Chu, Liqiang
  email: chuliqiang@tust.edu.cn
  organization: Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-utilization, College of Chemical Engineering and Materials Science, Tianjin University of Science and Technology, Tianjin 300457, China
– sequence: 12
  givenname: Bowen
  surname: Cheng
  fullname: Cheng, Bowen
  email: bowenc15@tust.edu.cn
  organization: State Key Laboratory of Biobased Fiber Manufacturing Technology, Tianjin University of Science and Technology, Tianjin 300457, China
BackLink https://www.ncbi.nlm.nih.gov/pubmed/36906361$$D View this record in MEDLINE/PubMed
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10.1016/j.carbpol.2021.118207
10.1021/acsmaterialslett.1c00368
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Keywords Stress-sensing
Self-powered
Wearable electronics
Ionic hydrogel
Macromolecular reinforcing agent
Double network
Language English
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PublicationTitle Carbohydrate polymers
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Snippet Strong and ductile sodium alginate (SA) reinforced polyacrylamide (PAM)/xanthan gum (XG) double network ionic hydrogels were constructed for stress sensing and...
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SubjectTerms batteries
capacitors
Double network
electrical conductivity
electronics
energy
hydrogels
hydrophilicity
Ionic hydrogel
Macromolecular reinforcing agent
mechanical stress
polyacrylamide
Self-powered
sodium alginate
Stress-sensing
tensile strength
Wearable electronics
xanthan gum
Title Sodium alginate reinforced polyacrylamide/xanthan gum double network ionic hydrogels for stress sensing and self-powered wearable device applications
URI https://dx.doi.org/10.1016/j.carbpol.2023.120678
https://www.ncbi.nlm.nih.gov/pubmed/36906361
https://www.proquest.com/docview/2786098427
https://www.proquest.com/docview/2834221130
Volume 309
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