The influence of Ni stability, redox, and lattice oxygen capacity on catalytic hydrogen production via methane dry reforming in innovative metal oxide systems
Finding a robust catalytic system for hydrogen production via dry reforming of methane (DRM) remains a challenge. Herein, MNi0.9Zr1−xYxO3 (M = Ce, La, and La0.6Ce0.4; x = 0.00, 0.05, 0.07, and 0.09) catalyst was prepared by the sol–gel method, tested for DRM and characterized by surface area and por...
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| Published in | Energy science & engineering Vol. 11; no. 4; pp. 1436 - 1450 |
|---|---|
| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
John Wiley & Sons, Inc
01.04.2023
Wiley |
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| Online Access | Get full text |
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| Abstract | Finding a robust catalytic system for hydrogen production via dry reforming of methane (DRM) remains a challenge. Herein, MNi0.9Zr1−xYxO3 (M = Ce, La, and La0.6Ce0.4; x = 0.00, 0.05, 0.07, and 0.09) catalyst was prepared by the sol–gel method, tested for DRM and characterized by surface area and porosity, X‐ray diffraction, H2‐temperature programmed reduction, thermogravimetry, and transmission electron microscopy. In La0.6Ce0.4NiO3 catalyst, the substitution of Ni by 0.1% Zr results in a constant high catalytic activity (83% hydrogen yield at 800°C) due to the presence of reducible “NiO‐species interacted strongly with the support” (stable metallic Ni over reduced catalyst) and redox input by ceria phase for laying instant lattice oxygen during lag‐off period of CO2. Substitution of Ni by Zr and Y in the CeNiO3 catalyst system nurtures Ni3Y (providing highly stable metallic Ni for CH4 decomposition) and cerium yttrium oxide phases (providing strong redox input). CeNi0.9Zr0.01Y0.09O3 shows 85% H2 yield at 800°C.
The manuscript investigated the influence of Ni stability, redox, and lattice oxygen capacity on catalytic hydrogen production via methane dry reforming in innovative metal oxide systems. Herein, MNi0.9Zr1−xYxO3 (M = Ce, La, and La0.6Ce0.4; x = 0.00, 0.05 0.07, and 0.09) catalyst was prepared by sol–gel method, tested for dry reforming of methane. CeNi0.9Zr0.01Y0.09O3 shows 85% H2 yield at 800°C. |
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| AbstractList | Finding a robust catalytic system for hydrogen production via dry reforming of methane (DRM) remains a challenge. Herein, MNi0.9Zr1−xYxO3 (M = Ce, La, and La0.6Ce0.4; x = 0.00, 0.05, 0.07, and 0.09) catalyst was prepared by the sol–gel method, tested for DRM and characterized by surface area and porosity, X-ray diffraction, H2-temperature programmed reduction, thermogravimetry, and transmission electron microscopy. In La0.6Ce0.4NiO3 catalyst, the substitution of Ni by 0.1% Zr results in a constant high catalytic activity (83% hydrogen yield at 800°C) due to the presence of reducible “NiO-species interacted strongly with the support” (stable metallic Ni over reduced catalyst) and redox input by ceria phase for laying instant lattice oxygen during lag-off period of CO2. Substitution of Ni by Zr and Y in the CeNiO3 catalyst system nurtures Ni3Y (providing highly stable metallic Ni for CH4 decomposition) and cerium yttrium oxide phases (providing strong redox input). CeNi0.9Zr0.01Y0.09O3 shows 85% H2 yield at 800°C. Finding a robust catalytic system for hydrogen production via dry reforming of methane (DRM) remains a challenge. Herein, MNi0.9Zr1−xYxO3 (M = Ce, La, and La0.6Ce0.4; x = 0.00, 0.05, 0.07, and 0.09) catalyst was prepared by the sol–gel method, tested for DRM and characterized by surface area and porosity, X‐ray diffraction, H2‐temperature programmed reduction, thermogravimetry, and transmission electron microscopy. In La0.6Ce0.4NiO3 catalyst, the substitution of Ni by 0.1% Zr results in a constant high catalytic activity (83% hydrogen yield at 800°C) due to the presence of reducible “NiO‐species interacted strongly with the support” (stable metallic Ni over reduced catalyst) and redox input by ceria phase for laying instant lattice oxygen during lag‐off period of CO2. Substitution of Ni by Zr and Y in the CeNiO3 catalyst system nurtures Ni3Y (providing highly stable metallic Ni for CH4 decomposition) and cerium yttrium oxide phases (providing strong redox input). CeNi0.9Zr0.01Y0.09O3 shows 85% H2 yield at 800°C. The manuscript investigated the influence of Ni stability, redox, and lattice oxygen capacity on catalytic hydrogen production via methane dry reforming in innovative metal oxide systems. Herein, MNi0.9Zr1−xYxO3 (M = Ce, La, and La0.6Ce0.4; x = 0.00, 0.05 0.07, and 0.09) catalyst was prepared by sol–gel method, tested for dry reforming of methane. CeNi0.9Zr0.01Y0.09O3 shows 85% H2 yield at 800°C. Abstract Finding a robust catalytic system for hydrogen production via dry reforming of methane (DRM) remains a challenge. Herein, MNi0.9Zr1−xYxO3 (M = Ce, La, and La0.6Ce0.4; x = 0.00, 0.05, 0.07, and 0.09) catalyst was prepared by the sol–gel method, tested for DRM and characterized by surface area and porosity, X‐ray diffraction, H2‐temperature programmed reduction, thermogravimetry, and transmission electron microscopy. In La0.6Ce0.4NiO3 catalyst, the substitution of Ni by 0.1% Zr results in a constant high catalytic activity (83% hydrogen yield at 800°C) due to the presence of reducible “NiO‐species interacted strongly with the support” (stable metallic Ni over reduced catalyst) and redox input by ceria phase for laying instant lattice oxygen during lag‐off period of CO2. Substitution of Ni by Zr and Y in the CeNiO3 catalyst system nurtures Ni3Y (providing highly stable metallic Ni for CH4 decomposition) and cerium yttrium oxide phases (providing strong redox input). CeNi0.9Zr0.01Y0.09O3 shows 85% H2 yield at 800°C. Abstract Finding a robust catalytic system for hydrogen production via dry reforming of methane (DRM) remains a challenge. Herein, MNi 0.9 Zr 1 − x Y x O 3 (M = Ce, La, and La 0.6 Ce 0.4 ; x = 0.00, 0.05, 0.07, and 0.09) catalyst was prepared by the sol–gel method, tested for DRM and characterized by surface area and porosity, X‐ray diffraction, H 2 ‐temperature programmed reduction, thermogravimetry, and transmission electron microscopy. In La 0.6 Ce 0.4 NiO 3 catalyst, the substitution of Ni by 0.1% Zr results in a constant high catalytic activity (83% hydrogen yield at 800°C) due to the presence of reducible “NiO‐species interacted strongly with the support” (stable metallic Ni over reduced catalyst) and redox input by ceria phase for laying instant lattice oxygen during lag‐off period of CO 2 . Substitution of Ni by Zr and Y in the CeNiO 3 catalyst system nurtures Ni 3 Y (providing highly stable metallic Ni for CH 4 decomposition) and cerium yttrium oxide phases (providing strong redox input). CeNi 0.9 Zr 0.01 Y 0.09 O 3 shows 85% H 2 yield at 800°C. |
| Author | Abasaeed, Ahmed E. Bayahia, Hossein Sofiu, Mahmud L. Al‐Awadi, Abdulrhman S. Acharya, Kenit AL‐Otaibi, Raja Lafi Al‐Fatesh, Ahmed Sadeq Ibrahim, Ahmed A. Al‐Zahrani, Salma A. Kumar, Rawesh Osman, Ahmed I. Fakeeha, Anis H. |
| Author_xml | – sequence: 1 givenname: Ahmed E. surname: Abasaeed fullname: Abasaeed, Ahmed E. organization: King Saud University – sequence: 2 givenname: Mahmud L. surname: Sofiu fullname: Sofiu, Mahmud L. organization: King Saud University – sequence: 3 givenname: Kenit surname: Acharya fullname: Acharya, Kenit organization: Indus University – sequence: 4 givenname: Ahmed I. orcidid: 0000-0003-2788-7839 surname: Osman fullname: Osman, Ahmed I. email: aosmanahmed01@qub.ac.uk organization: Queen's University Belfast – sequence: 5 givenname: Anis H. surname: Fakeeha fullname: Fakeeha, Anis H. organization: Energy Research & Innovation Center (K.A.CARE) in Riyadh – sequence: 6 givenname: Raja Lafi surname: AL‐Otaibi fullname: AL‐Otaibi, Raja Lafi email: raletabi@kacst.edu.sa organization: King Abdulaziz City for Science and Technology – sequence: 7 givenname: Ahmed A. surname: Ibrahim fullname: Ibrahim, Ahmed A. organization: King Saud University – sequence: 8 givenname: Abdulrhman S. surname: Al‐Awadi fullname: Al‐Awadi, Abdulrhman S. organization: Energy Research & Innovation Center (K.A.CARE) in Riyadh – sequence: 9 givenname: Hossein orcidid: 0000-0002-1287-910X surname: Bayahia fullname: Bayahia, Hossein organization: Albaha University – sequence: 10 givenname: Salma A. surname: Al‐Zahrani fullname: Al‐Zahrani, Salma A. organization: University of Hail – sequence: 11 givenname: Rawesh surname: Kumar fullname: Kumar, Rawesh email: kr.rawesh@gmail.com organization: Indus University – sequence: 12 givenname: Ahmed Sadeq orcidid: 0000-0002-5521-5741 surname: Al‐Fatesh fullname: Al‐Fatesh, Ahmed Sadeq email: aalfatesh@ksu.edu.sa organization: King Saud University |
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| Snippet | Finding a robust catalytic system for hydrogen production via dry reforming of methane (DRM) remains a challenge. Herein, MNi0.9Zr1−xYxO3 (M = Ce, La, and... Abstract Finding a robust catalytic system for hydrogen production via dry reforming of methane (DRM) remains a challenge. Herein, MNi 0.9 Zr 1 − x Y x O 3 (M... Abstract Finding a robust catalytic system for hydrogen production via dry reforming of methane (DRM) remains a challenge. Herein, MNi0.9Zr1−xYxO3 (M = Ce, La,... |
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| SubjectTerms | Acids Carbon Carbon dioxide Catalysts Catalytic activity CeNi0.9Zr1−xYxO3 Cerium Cerium oxides dry reforming H2 yield Heat resistance Hydrogen Hydrogen production La0.6Ce0.4Ni0.9Zr1−xYxO3 catalyst system Metal oxides Metals Methane Oxidation Oxygen Porosity Reforming Sol-gel processes Stainless steel Substitutes Synthesis gas Thermogravimetry X-ray diffraction Yttrium Yttrium oxide Zirconium |
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| Title | The influence of Ni stability, redox, and lattice oxygen capacity on catalytic hydrogen production via methane dry reforming in innovative metal oxide systems |
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