Ordered structures of two sulfur containing donor molecules on the Au(111) surface

We report experiments by low energy electron diffraction (LEED) and scanning tunneling microscopy (STM) on ordered structures of two sulfur-containing π-conjugated molecules on the Au(111)-surface, namely tetrabenzothianthrene (TBTA) and tetrathiotetracene (TTT). These molecules are candidates for d...

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Published inSurface science Vol. 606; no. 23-24; pp. 1855 - 1863
Main Authors Fiedler, Benjamin, Rojo-Wiechel, Elena, Klassen, Johann, Simon, Julia, Beck, Johannes, Sokolowski, Moritz
Format Journal Article
LanguageEnglish
Published Kidlington Elsevier B.V 01.12.2012
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Abstract We report experiments by low energy electron diffraction (LEED) and scanning tunneling microscopy (STM) on ordered structures of two sulfur-containing π-conjugated molecules on the Au(111)-surface, namely tetrabenzothianthrene (TBTA) and tetrathiotetracene (TTT). These molecules are candidates for donors in charge transfer salts. On Au(111) both molecules form long-range ordered structures that are commensurate to the top-most surface layer. For TBTA, the reconstruction of the Au(111) surface is maintained, whereas it is lifted by TTT. Both molecules lie flat on the surface. For TBTA, the structure indicates that the molecule is planarized upon adsorption. ► Tetrabenzothianthrene and tetrathiotetracene form long-range ordered commensurate structures on the Au(111) surface ► For TBTA, the reconstruction of the Au(111) surface is maintained. ► The reconstruction is lifted by TTT. ► Both molecules adsorb intact and in a planar configuration. ► For TBTA, the structure indicates that the molecule is planarized upon adsorption.
AbstractList We report experiments by low energy electron diffraction (LEED) and scanning tunneling microscopy (STM) on ordered structures of two sulfur-containing π-conjugated molecules on the Au(111)-surface, namely tetrabenzothianthrene (TBTA) and tetrathiotetracene (TTT). These molecules are candidates for donors in charge transfer salts. On Au(111) both molecules form long-range ordered structures that are commensurate to the top-most surface layer. For TBTA, the reconstruction of the Au(111) surface is maintained, whereas it is lifted by TTT. Both molecules lie flat on the surface. For TBTA, the structure indicates that the molecule is planarized upon adsorption. ► Tetrabenzothianthrene and tetrathiotetracene form long-range ordered commensurate structures on the Au(111) surface ► For TBTA, the reconstruction of the Au(111) surface is maintained. ► The reconstruction is lifted by TTT. ► Both molecules adsorb intact and in a planar configuration. ► For TBTA, the structure indicates that the molecule is planarized upon adsorption.
Author Simon, Julia
Beck, Johannes
Rojo-Wiechel, Elena
Klassen, Johann
Fiedler, Benjamin
Sokolowski, Moritz
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Keywords Au
Organic molecules
Thin organic films
STM
SPA-LEED
Ordered structures
Thin films
Scanning tunneling microscopy
Donors
LEED
Sulfur
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Snippet We report experiments by low energy electron diffraction (LEED) and scanning tunneling microscopy (STM) on ordered structures of two sulfur-containing...
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SubjectTerms Condensed matter: electronic structure, electrical, magnetic, and optical properties
Condensed matter: structure, mechanical and thermal properties
Cross-disciplinary physics: materials science; rheology
Exact sciences and technology
Ordered structures
Organic molecules
Physics
SPA-LEED
STM
Thin organic films
Title Ordered structures of two sulfur containing donor molecules on the Au(111) surface
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