Molecular-sized fluorescent nanodiamonds
Doping of carbon nanoparticles with impurity atoms is central to their application 1 , 2 . However, doping has proven elusive for very small carbon nanoparticles because of their limited availability and a lack of fundamental understanding of impurity stability in such nanostructures 3 . Here, we sh...
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| Published in | Nature nanotechnology Vol. 9; no. 1; pp. 54 - 58 |
|---|---|
| Main Authors | , , , , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
01.01.2014
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Doping of carbon nanoparticles with impurity atoms is central to their application
1
,
2
. However, doping has proven elusive for very small carbon nanoparticles because of their limited availability and a lack of fundamental understanding of impurity stability in such nanostructures
3
. Here, we show that isolated diamond nanoparticles as small as 1.6 nm, comprising only ∼400 carbon atoms, are capable of housing stable photoluminescent colour centres, namely the silicon vacancy (SiV)
4
,
5
. Surprisingly, fluorescence from SiVs is stable over time, and few or only single colour centres are found per nanocrystal. We also observe size-dependent SiV emission supported by quantum-chemical simulation of SiV energy levels in small nanodiamonds. Our work opens the way to investigating the physics and chemistry of molecular-sized cubic carbon clusters and promises the application of ultrasmall non-perturbative fluorescent nanoparticles as markers in microscopy and sensing.
Diamond nanoparticles containing only about 400 atoms emit bright fluorescence due to silicon vacancy defects. |
|---|---|
| AbstractList | Doping of carbon nanoparticles with impurity atoms is central to their application. However, doping has proven elusive for very small carbon nanoparticles because of their limited availability and a lack of fundamental understanding of impurity stability in such nanostructures. Here, we show that isolated diamond nanoparticles as small as 1.6 nm, comprising only ∼400 carbon atoms, are capable of housing stable photoluminescent colour centres, namely the silicon vacancy (SiV). Surprisingly, fluorescence from SiVs is stable over time, and few or only single colour centres are found per nanocrystal. We also observe size-dependent SiV emission supported by quantum-chemical simulation of SiV energy levels in small nanodiamonds. Our work opens the way to investigating the physics and chemistry of molecular-sized cubic carbon clusters and promises the application of ultrasmall non-perturbative fluorescent nanoparticles as markers in microscopy and sensing. Doping of carbon nanoparticles with impurity atoms is central to their application 1 , 2 . However, doping has proven elusive for very small carbon nanoparticles because of their limited availability and a lack of fundamental understanding of impurity stability in such nanostructures 3 . Here, we show that isolated diamond nanoparticles as small as 1.6 nm, comprising only ∼400 carbon atoms, are capable of housing stable photoluminescent colour centres, namely the silicon vacancy (SiV) 4 , 5 . Surprisingly, fluorescence from SiVs is stable over time, and few or only single colour centres are found per nanocrystal. We also observe size-dependent SiV emission supported by quantum-chemical simulation of SiV energy levels in small nanodiamonds. Our work opens the way to investigating the physics and chemistry of molecular-sized cubic carbon clusters and promises the application of ultrasmall non-perturbative fluorescent nanoparticles as markers in microscopy and sensing. Diamond nanoparticles containing only about 400 atoms emit bright fluorescence due to silicon vacancy defects. Doping of carbon nanoparticles with impurity atoms is central to their application. However, doping has proven elusive for very small carbon nanoparticles because of their limited availability and a lack of fundamental understanding of impurity stability in such nanostructures. Here, we show that isolated diamond nanoparticles as small as 1.6 nm, comprising only 400 carbon atoms, are capable of housing stable photoluminescent colour centres, namely the silicon vacancy (SiV). Surprisingly, fluorescence from SiVs is stable over time, and few or only single colour centres are found per nanocrystal. We also observe size-dependent SiV emission supported by quantum-chemical simulation of SiV energy levels in small nanodiamonds. Our work opens the way to investigating the physics and chemistry of molecular-sized cubic carbon clusters and promises the application of ultrasmall non-perturbative fluorescent nanoparticles as markers in microscopy and sensing. |
| Author | Vlasov, Igor I. Vörös, Márton Shiryaev, Andrey A. Kaiser, Ute Jelezko, Fedor Konov, Vitaly I. Gali, Adam Sildos, Ilmo Steinert, Steffen Fisenko, Anatolii V. Wrachtrup, Jörg Antonov, Denis Semjonova, Lubov F. Lee, Sang-Yun Lebedev, Oleg I. Biskupek, Johannes Hemmer, Philip. R. Rendler, Torsten |
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| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/24317283$$D View this record in MEDLINE/PubMed |
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| Snippet | Doping of carbon nanoparticles with impurity atoms is central to their application
1
,
2
. However, doping has proven elusive for very small carbon... Doping of carbon nanoparticles with impurity atoms is central to their application. However, doping has proven elusive for very small carbon nanoparticles... |
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| SubjectTerms | 639/624/399/1096 Carbon Chemistry Color centers Defects Diamonds Doping Electrons Emissions Fluorescence Impurities letter Materials Science Microscopy Nanoparticles Nanostructure Nanotechnology Nanotechnology and Microengineering Optics Physics Quantum chemistry Quantum dots Silicon |
| Title | Molecular-sized fluorescent nanodiamonds |
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