Water/AOT/IPM/alcohol reverse microemulsions: Influence of salts and nonionic surfactants on structure and percolation behavior

•Hydrogen bond interactions cause NaSal assist the percolation.•Brij-56 (TX-100) makes Peff decrease and droplets diameter increase, promoting the percolation.•Spans have little effect on percolation due mainly to their small headgroup.•Alcohol can decrease evidently the activation energy by enhanci...

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Published inThe Journal of chemical thermodynamics Vol. 72; pp. 1 - 8
Main Authors Liu, Jiexiang, Zhang, Xiaoguang, Zhang, Haijiao
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 01.05.2014
Subjects
Activation energy
AOT
Droplets
Dynamical systems
Dynamics
Microemulsions
Nonionic
Nonionic surfactants
Percolation
Salts
Sodium
Sodium chloride
Surfactants
Nonionic surfactants
Percolation
Salts
Activation energy
AOT
Online AccessGet full text

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Abstract •Hydrogen bond interactions cause NaSal assist the percolation.•Brij-56 (TX-100) makes Peff decrease and droplets diameter increase, promoting the percolation.•Spans have little effect on percolation due mainly to their small headgroup.•Alcohol can decrease evidently the activation energy by enhancing the interfacial flexibility. Influence of salts (sodium chloride, sodium salicylate and sodium cholate) and nonionic surfactants (Brij-56, TX-100, Span-20, Span-40 and Span-60) on structure and percolation behavior of water/AOT/IPM/propanol (butanol) systems were systematically investigated using conductivity and dynamic light scattering. Percolation behavior had a distinct change with different types of salts and nonionic surfactants. Addition of sodium chloride delayed the conductivity percolation, while sodium salicylate and sodium cholate assisted the percolation. Addition of Brij-56 and TX-100 promoted evidently the conductivity percolation, whereas Spans had little effect. Conductivity behavior was further discussed from the structural properties of nonionic surfactants and salts, and the surfactant packing parameter (P). Droplets sizes were measured using dynamic light scattering to underline the effect of nonionic surfactants on P. Furthermore, lnσ had a linear correlation with temperature in the range of (278.15 to 313.15)K. No percolation threshold induced by temperature was detected among all the studied systems. Moreover, the activation energy for conductivity was also estimated and discussed according to the Arrhenius-type equation.
AbstractList •Hydrogen bond interactions cause NaSal assist the percolation.•Brij-56 (TX-100) makes Peff decrease and droplets diameter increase, promoting the percolation.•Spans have little effect on percolation due mainly to their small headgroup.•Alcohol can decrease evidently the activation energy by enhancing the interfacial flexibility. Influence of salts (sodium chloride, sodium salicylate and sodium cholate) and nonionic surfactants (Brij-56, TX-100, Span-20, Span-40 and Span-60) on structure and percolation behavior of water/AOT/IPM/propanol (butanol) systems were systematically investigated using conductivity and dynamic light scattering. Percolation behavior had a distinct change with different types of salts and nonionic surfactants. Addition of sodium chloride delayed the conductivity percolation, while sodium salicylate and sodium cholate assisted the percolation. Addition of Brij-56 and TX-100 promoted evidently the conductivity percolation, whereas Spans had little effect. Conductivity behavior was further discussed from the structural properties of nonionic surfactants and salts, and the surfactant packing parameter (P). Droplets sizes were measured using dynamic light scattering to underline the effect of nonionic surfactants on P. Furthermore, lnσ had a linear correlation with temperature in the range of (278.15 to 313.15)K. No percolation threshold induced by temperature was detected among all the studied systems. Moreover, the activation energy for conductivity was also estimated and discussed according to the Arrhenius-type equation.
Influence of salts (sodium chloride, sodium salicylate and sodium cholate) and nonionic surfactants (Brij-56, TX-100, Span-20, Span-40 and Span-60) on structure and percolation behavior of water/AOT/IPM/propanol (butanol) systems were systematically investigated using conductivity and dynamic light scattering. Percolation behavior had a distinct change with different types of salts and nonionic surfactants. Addition of sodium chloride delayed the conductivity percolation, while sodium salicylate and sodium cholate assisted the percolation. Addition of Brij-56 and TX-100 promoted evidently the conductivity percolation, whereas Spans had little effect. Conductivity behavior was further discussed from the structural properties of nonionic surfactants and salts, and the surfactant packing parameter (P). Droplets sizes were measured using dynamic light scattering to underline the effect of nonionic surfactants on P. Furthermore, ln sigma had a linear correlation with temperature in the range of (278.15 to 313.15) K. No percolation threshold induced by temperature was detected among all the studied systems. Moreover, the activation energy for conductivity was also estimated and discussed according to the Arrhenius-type equation.
Author Zhang, Haijiao
Zhang, Xiaoguang
Liu, Jiexiang
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  organization: School of Chemical Engineering, Hebei University of Technology, Tianjin 300130, China
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Keywords Nonionic surfactants
Percolation
Salts
Activation energy
AOT
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Snippet •Hydrogen bond interactions cause NaSal assist the percolation.•Brij-56 (TX-100) makes Peff decrease and droplets diameter increase, promoting the...
Influence of salts (sodium chloride, sodium salicylate and sodium cholate) and nonionic surfactants (Brij-56, TX-100, Span-20, Span-40 and Span-60) on...
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SubjectTerms Activation energy
AOT
Droplets
Dynamical systems
Dynamics
Microemulsions
Nonionic
Nonionic surfactants
Percolation
Salts
Sodium
Sodium chloride
Surfactants
Title Water/AOT/IPM/alcohol reverse microemulsions: Influence of salts and nonionic surfactants on structure and percolation behavior
URI https://dx.doi.org/10.1016/j.jct.2013.12.026
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