The effects of salt concentration and foulant surface charge on hydrocarbon fouling of a poly(vinylidene fluoride) microfiltration membrane

The effects of inorganic salts and organic hydrocarbons on membrane fouling are often investigated independently. However, in many cases, these foulants are commonly found together, and such mixtures are rarely the subject of fouling studies. In this study, crude oil-in-water emulsions were formulat...

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Published inWater research (Oxford) Vol. 117; pp. 230 - 241
Main Authors He, Zhengwang, Kasemset, Sirirat, Kirschner, Alon Y., Cheng, Yu-Heng, Paul, Donald R., Freeman, Benny D.
Format Journal Article
LanguageEnglish
Published England Elsevier Ltd 15.06.2017
Subjects
DLVO model
Emulsions
Filtration
fluorides
fouling
Fouling propensity
Hydrocarbons
Ionic strength
Membrane fouling
Membranes, Artificial
microfiltration
Oil emulsion
oils
prediction
salt concentration
sodium chloride
surface interactions
Surface Properties
surface tension
Zeta potential
DLVO model
Fouling propensity
Zeta potential
Ionic strength
Membrane fouling
Oil emulsion
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Abstract The effects of inorganic salts and organic hydrocarbons on membrane fouling are often investigated independently. However, in many cases, these foulants are commonly found together, and such mixtures are rarely the subject of fouling studies. In this study, crude oil-in-water emulsions were formulated at three different added NaCl concentrations, 0, 10-3 and 10−1 M. Surface properties, such as surface tension and surface charge, of these emulsions and a poly(vinylidene fluoride) (PVDF) microfiltration (MF) membrane were characterized. The Derjaguin-Landau-Verwey-Overbeek (DLVO) model was utilized to simulate membrane-oil droplet and oil layer-oil droplet surface interactions. The DLVO model qualitatively predicted increasing fouling propensity with increasing emulsion salt concentration. The PVDF MF membrane was challenged with crude oil-in-water emulsions in constant permeate flux crossflow fouling tests to characterize the fouling propensity of the various emulsions, and the results were consistent with the model predictions. •Crude oil-in-water emulsions were formulated at various salt concentrations.•Foulant zeta potential decreased with increasing salt concentration.•DLVO model was used to simulate short-range interactions.•Model predictions of fouling propensity matched experimental observations.•Electrostatic interactions dominated van der Waals interactions in this study.
AbstractList The effects of inorganic salts and organic hydrocarbons on membrane fouling are often investigated independently. However, in many cases, these foulants are commonly found together, and such mixtures are rarely the subject of fouling studies. In this study, crude oil-in-water emulsions were formulated at three different added NaCl concentrations, 0, 10-3 and 10-1 M. Surface properties, such as surface tension and surface charge, of these emulsions and a poly(vinylidene fluoride) (PVDF) microfiltration (MF) membrane were characterized. The Derjaguin-Landau-Verwey-Overbeek (DLVO) model was utilized to simulate membrane-oil droplet and oil layer-oil droplet surface interactions. The DLVO model qualitatively predicted increasing fouling propensity with increasing emulsion salt concentration. The PVDF MF membrane was challenged with crude oil-in-water emulsions in constant permeate flux crossflow fouling tests to characterize the fouling propensity of the various emulsions, and the results were consistent with the model predictions.The effects of inorganic salts and organic hydrocarbons on membrane fouling are often investigated independently. However, in many cases, these foulants are commonly found together, and such mixtures are rarely the subject of fouling studies. In this study, crude oil-in-water emulsions were formulated at three different added NaCl concentrations, 0, 10-3 and 10-1 M. Surface properties, such as surface tension and surface charge, of these emulsions and a poly(vinylidene fluoride) (PVDF) microfiltration (MF) membrane were characterized. The Derjaguin-Landau-Verwey-Overbeek (DLVO) model was utilized to simulate membrane-oil droplet and oil layer-oil droplet surface interactions. The DLVO model qualitatively predicted increasing fouling propensity with increasing emulsion salt concentration. The PVDF MF membrane was challenged with crude oil-in-water emulsions in constant permeate flux crossflow fouling tests to characterize the fouling propensity of the various emulsions, and the results were consistent with the model predictions.
The effects of inorganic salts and organic hydrocarbons on membrane fouling are often investigated independently. However, in many cases, these foulants are commonly found together, and such mixtures are rarely the subject of fouling studies. In this study, crude oil-in-water emulsions were formulated at three different added NaCl concentrations, 0, 10−3 and 10−1 M. Surface properties, such as surface tension and surface charge, of these emulsions and a poly(vinylidene fluoride) (PVDF) microfiltration (MF) membrane were characterized. The Derjaguin-Landau-Verwey-Overbeek (DLVO) model was utilized to simulate membrane-oil droplet and oil layer-oil droplet surface interactions. The DLVO model qualitatively predicted increasing fouling propensity with increasing emulsion salt concentration. The PVDF MF membrane was challenged with crude oil-in-water emulsions in constant permeate flux crossflow fouling tests to characterize the fouling propensity of the various emulsions, and the results were consistent with the model predictions.
The effects of inorganic salts and organic hydrocarbons on membrane fouling are often investigated independently. However, in many cases, these foulants are commonly found together, and such mixtures are rarely the subject of fouling studies. In this study, crude oil-in-water emulsions were formulated at three different added NaCl concentrations, 0, 10 and 10 M. Surface properties, such as surface tension and surface charge, of these emulsions and a poly(vinylidene fluoride) (PVDF) microfiltration (MF) membrane were characterized. The Derjaguin-Landau-Verwey-Overbeek (DLVO) model was utilized to simulate membrane-oil droplet and oil layer-oil droplet surface interactions. The DLVO model qualitatively predicted increasing fouling propensity with increasing emulsion salt concentration. The PVDF MF membrane was challenged with crude oil-in-water emulsions in constant permeate flux crossflow fouling tests to characterize the fouling propensity of the various emulsions, and the results were consistent with the model predictions.
The effects of inorganic salts and organic hydrocarbons on membrane fouling are often investigated independently. However, in many cases, these foulants are commonly found together, and such mixtures are rarely the subject of fouling studies. In this study, crude oil-in-water emulsions were formulated at three different added NaCl concentrations, 0, 10-3 and 10−1 M. Surface properties, such as surface tension and surface charge, of these emulsions and a poly(vinylidene fluoride) (PVDF) microfiltration (MF) membrane were characterized. The Derjaguin-Landau-Verwey-Overbeek (DLVO) model was utilized to simulate membrane-oil droplet and oil layer-oil droplet surface interactions. The DLVO model qualitatively predicted increasing fouling propensity with increasing emulsion salt concentration. The PVDF MF membrane was challenged with crude oil-in-water emulsions in constant permeate flux crossflow fouling tests to characterize the fouling propensity of the various emulsions, and the results were consistent with the model predictions. •Crude oil-in-water emulsions were formulated at various salt concentrations.•Foulant zeta potential decreased with increasing salt concentration.•DLVO model was used to simulate short-range interactions.•Model predictions of fouling propensity matched experimental observations.•Electrostatic interactions dominated van der Waals interactions in this study.
Author He, Zhengwang
Kasemset, Sirirat
Kirschner, Alon Y.
Paul, Donald R.
Freeman, Benny D.
Cheng, Yu-Heng
Author_xml – sequence: 1
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  givenname: Alon Y.
  surname: Kirschner
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  surname: Freeman
  fullname: Freeman, Benny D.
  email: freeman@che.utexas.edu
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Keywords DLVO model
Fouling propensity
Zeta potential
Ionic strength
Membrane fouling
Oil emulsion
Language English
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Snippet The effects of inorganic salts and organic hydrocarbons on membrane fouling are often investigated independently. However, in many cases, these foulants are...
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SubjectTerms DLVO model
Emulsions
Filtration
fluorides
fouling
Fouling propensity
Hydrocarbons
Ionic strength
Membrane fouling
Membranes, Artificial
microfiltration
Oil emulsion
oils
prediction
salt concentration
sodium chloride
surface interactions
Surface Properties
surface tension
Zeta potential
Title The effects of salt concentration and foulant surface charge on hydrocarbon fouling of a poly(vinylidene fluoride) microfiltration membrane
URI https://dx.doi.org/10.1016/j.watres.2017.03.051
https://www.ncbi.nlm.nih.gov/pubmed/28412584
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https://www.proquest.com/docview/2000368427
Volume 117
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