Pure hydrogen generation in a fluidized-bed membrane reactor: Experimental findings
A pilot-scale fluidized-bed membrane reactor was tested for the production of hydrogen. The prototype reactor operated under steam methane reforming (SMR) and autothermal reforming (ATR) conditions, without membranes and with membranes of different total areas. Heat was added either externally or vi...
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| Published in | Chemical engineering science Vol. 63; no. 10; pp. 2752 - 2762 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
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Oxford
Elsevier Ltd
01.05.2008
Elsevier |
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| Abstract | A pilot-scale fluidized-bed membrane reactor was tested for the production of hydrogen. The prototype reactor operated under steam methane reforming (SMR) and autothermal reforming (ATR) conditions, without membranes and with membranes of different total areas. Heat was added either externally or via direct air addition. Hydrogen permeate purity of up to 99.995+% as well as a pure-H2-to-natural-gas yield of 2.07 were achieved with only half of the full complement of membrane panels active under SMR conditions. A permeate-H2-to reactor natural gas feed molar ratio >3 was achieved when all of the membrane panels were installed under SMR conditions. Experimental tests investigated the influence of such parameters as reactor pressure, hydrogen permeate pressure (vacuum vs atmospheric pressure), air top/bottom split, feed flowrate and membrane area. Reactor performance was strongly dependent on the active membrane surface area. |
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| AbstractList | A pilot-scale fluidized-bed membrane reactor was tested for the production of hydrogen. The prototype reactor operated under steam methane reforming (SMR) and autothermal reforming (ATR) conditions, without membranes and with membranes of different total areas. Heat was added either externally or via direct air addition. Hydrogen permeate purity of up to 99.995+% as well as a pure-H2-to-natural-gas yield of 2.07 were achieved with only half of the full complement of membrane panels active under SMR conditions. A permeate-H2-to reactor natural gas feed molar ratio >3 was achieved when all of the membrane panels were installed under SMR conditions. Experimental tests investigated the influence of such parameters as reactor pressure, hydrogen permeate pressure (vacuum vs atmospheric pressure), air top/bottom split, feed flowrate and membrane area. Reactor performance was strongly dependent on the active membrane surface area. |
| Author | Mahecha-Botero, Andrés Lim, C. Jim Grace, John R. Shirasaki, Yoshinori Comyn, Nicholas Boyd, Tony Yasuda, Isamu Gulamhusein, Ali |
| Author_xml | – sequence: 1 givenname: Andrés surname: Mahecha-Botero fullname: Mahecha-Botero, Andrés email: andresm@chml.ubc.ca, andresmb@gmail.com organization: Department of Chemical and Biological Engineering, University of British Columbia, 2360 East Mall, Vancouver, Canada V6T 1Z3 – sequence: 2 givenname: Tony surname: Boyd fullname: Boyd, Tony organization: Membrane Reactor Technologies (MRT) Ltd., 200 Granville Street, Suite 1800, Vancouver, BC, Canada V6C 1S4 – sequence: 3 givenname: Ali surname: Gulamhusein fullname: Gulamhusein, Ali organization: Membrane Reactor Technologies (MRT) Ltd., 200 Granville Street, Suite 1800, Vancouver, BC, Canada V6C 1S4 – sequence: 4 givenname: Nicholas surname: Comyn fullname: Comyn, Nicholas organization: Membrane Reactor Technologies (MRT) Ltd., 200 Granville Street, Suite 1800, Vancouver, BC, Canada V6C 1S4 – sequence: 5 givenname: C. Jim surname: Lim fullname: Lim, C. Jim organization: Department of Chemical and Biological Engineering, University of British Columbia, 2360 East Mall, Vancouver, Canada V6T 1Z3 – sequence: 6 givenname: John R. surname: Grace fullname: Grace, John R. organization: Department of Chemical and Biological Engineering, University of British Columbia, 2360 East Mall, Vancouver, Canada V6T 1Z3 – sequence: 7 givenname: Yoshinori surname: Shirasaki fullname: Shirasaki, Yoshinori organization: Tokyo Gas Co., Ltd. Hydrogen System Team, Technology Research Institute, 1-7-7, Suehiro-cho, Tsurumi-ku, Yokohama-city, Kanagawa 230-0045 Japan – sequence: 8 givenname: Isamu surname: Yasuda fullname: Yasuda, Isamu organization: Tokyo Gas Co., Ltd. Hydrogen System Team, Technology Research Institute, 1-7-7, Suehiro-cho, Tsurumi-ku, Yokohama-city, Kanagawa 230-0045 Japan |
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| Keywords | Membranes Multiphase reactors Powder technology Prototype fluidized-bed membrane reactor Fuel Steam methane reforming Autothermic reactor Atmospheric pressure Purity Reforming Fluidization Water vapor Membrane reactor Surface area Steam methane reforming;Membranes;Multiphase reactors;Powder technology Natural gas Hydrogen production Fluidized bed |
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| Snippet | A pilot-scale fluidized-bed membrane reactor was tested for the production of hydrogen. The prototype reactor operated under steam methane reforming (SMR) and... |
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| SubjectTerms | Applied sciences Chemical engineering Exact sciences and technology Fluidization Fuel Membranes Multiphase reactors Powder technology Prototype fluidized-bed membrane reactor Reactors Steam methane reforming |
| Title | Pure hydrogen generation in a fluidized-bed membrane reactor: Experimental findings |
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